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Journal of Theoretical and Computational Chemistry

Theoretical study of Zeno and anti-Zeno effects on photodissociation dynamics: A model approach

Bikram Nath, Chandan Kumar Mondal

Published Nov 3, 2016• 2 citations
Publisher

Abstract

Zeno and anti-Zeno effects in the evolution of the multi-photonic dissociation dynamics of the diatomic molecule HBr[Formula: see text] owing to repeated measurements demand if the system in the initial state have been studied. The effects have been calculated numerically for the case of vibrational population transfer and dissociation dynamics of HBr[Formula: see text] taking it as a model. We use time-dependent Fourier grid Hamiltonian (TDFGH) method as a mathematical tool in presence of intense radiation field as perturbation. The effects have been explored through a probable mechanism of population transfer from the ground vibrational state to the different upper vibrational states which ultimately go to the dissociation continuum. The results show significant differences in the mechanism of population transfer and the significant role of time interval of measurement ([Formula: see text] in Zeno and anti-Zeno effects. In case of survival probability of ground vibrational states, there is Zeno effect when the frequency of the laser to which the molecule is submitted is near the vibrational [Formula: see text] to [Formula: see text] resonance, while there is anti-Zeno effect if it is far from this resonance.

DOI
10.1142/s021963361650070x

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American Journal of Modern Physics•Jan 1, 2018•0 citations
Zeno and anti-Zeno effects in the evolution of the multi-photonic dissociation dynamics of the diatomic molecule HBr[Formula: see text] owing to repeated measurements demand if the system in the initial state have been studied. The effects have been calculated numerically for the case of vibrational population transfer and dissociation dynamics of HBr[Formula: see text] taking it as a model. We use time-dependent Fourier grid Hamiltonian (TDFGH) method as a mathematical tool in presence of intense radiation field as perturbation. The effects have been explored through a probable mechanism of population transfer from the ground vibrational state to the different upper vibrational states which ultimately go to the dissociation continuum. The results show significant differences in the mechanism of population transfer and the significant role of time interval of measurement ([Formula: see text] in Zeno and anti-Zeno effects. In case of survival probability of ground vibrational states, there is Zeno effect when the frequency of the laser to which the molecule is submitted is near the vibrational [Formula: see text] to [Formula: see text] resonance, while there is anti-Zeno effect if it is far from this resonance.
We have proposed the mathematical formulations of quantum Zeno and anti-Zeno effects at non-zero temperature on vibrational population transfer and dissociation of a diatomic system. The proposed formulation has been tested for diatomic systems HBr+ and HI using time-dependent Fourier grid Hamiltonian method. The effect of temperature on the dynamics is incorporated through the population distribution at different vibrational states following Boltzmann distribution formula. It has been found that with increase in temperature Zeno effect increases and anti-Zeno effect decreases in case of survival probability on ground vibrational state. In case of dissociation, with increase in temperature Zeno effect increases while anti-Zeno effect remains almost same.
We have proposed a methodology that uses secondary electromagnetic field to overcome the effect of measurement on quantum dynamics. Our aim is also to find out some characteristics of the used secondary (recovery) field. We have applied the methodology to reduce the quantum Zeno effect (ZE), a consequence of repeated measurements in survival probability of ground vibrational state. As the model systems, we choose HBr[Formula: see text] and HI. The study is done with variation in frequency, pulse shape and other parameters of the secondary field. In all cases, suitable secondary field for which the Zeno effect is minimum is found near 0 [Formula: see text] 1 vibrational transition frequency. Suitable time gap between the measurement and the application of secondary field depends on the shape of the secondary field. When the secondary field is optimized, the recovery is more than 90% which almost nullify the Zeno effect.
We examine the appearance of Zeno and anti-Zeno effects (Misra and Sudarshan 1977 J. Math. Phys. 18 756; Kofman and Kurizki 2000 Nature 405 546; Kofman and Kurizki 1996 Phys. Rev. A 54 3750; Facchi et al 2001 Phys. Rev. Lett. 86 2699) in the entanglement dynamics of two qubits off-resonantly coupled to the same lossy cavity when the unitary evolution of the system is interrupted by repeated projective measurements. We describe in detail these quantum effects by comparing the measurement-induced coarse-grained dynamics to the entanglement evolution in the absence of measurements in several scenarios (Francica et al 2009 Phys. Rev. A 79 032310). In particular, we examine the strong and weak coupling regimes, the role of the relative coupling strengths between the two qubits and the reservoir and the effect of the detuning from the main cavity frequency. We show that the anti-Zeno effect can occur in the entanglement dynamics when the qubit frequencies are detuned from the main reservoir frequency. Furthermore, we find that Zeno and anti-Zeno effects can even appear sequentially many times as a function of the interval between the measurements. Finally, we show that, in the off-resonant regime, we can preserve the entanglement using the quantum Zeno effect more efficiently than in the resonant limit (Maniscalco et al 2008 Phys. Rev. Lett. 100 090503), even if, in this case, no sub-radiant state exists.
Quantum Zeno and anti-Zeno effects on pure dephasing are studied using exactly solvable microscopic models. The crossover between these two opposite effects is investigated. The case of a single two-level system undergoing dephasing is already different from the previously studied population-decay problem, even without taking into account any back action from the environment. For many two-level systems interacting with a common environment, multiple transitions between Zeno and anti-Zeno regimes are predicted. Finally, if the system-environment coupling strength is not weak, we show that the nontrivial evolution of the environment between measurements can considerably alter the quantum Zeno and anti-Zeno effects. This is qualitatively different from population-decay models where the environment state is reset to equilibrium after each measurement.
The quantum-Zeno and anti-Zeno effects (QZE/AZE) are known for a long time, in a quantum system with coupled levels, the measurement of a particular level population can lead to either acceleration (i.e. AZE) or retardation (i.e. QZE) of its population transfer to other levels. Here we consider how one can control the population flow from a coupled quantum state by measurement at a particular time, and what system parameters are responsible for that. We propose a framework for analysis of quantum Zeno dynamics based on time-dependent density matrix perturbation theory. This framework allows us to clearly separate state populations from their coherences and to predict appearance of either QZE or AZE. We illustrate our analysis on two model systems: 1) two coupled levels and 2) a level coupled to a continuum. In both cases dynamics of quantum coherences play a crucial role, and perturbative considerations allow us to predict the effect of projective measurements. In addition, we have extended our consideration to a closely related coherent control scenario, a unitary transformation flipping a sign of a state in a coherent superposition describing the system wavefunction.
Quantum Zeno effect can be applied to quantum information processing，and can reveal the nature of quantum measurement. In addition, it has also many potential applications. This suggests that studying the quantum Zeno effect has great theoretical and experimental significance. In this work, the system of a two-level atom interacting with a single mode field is considered and the dynamics of the system subjected to successive projection measurements is studied, and the quantum Zeno effect is presented. Moreover, the influence of the quantum Zeno effect on atomic population inversion is discussed. Based on Schrödinger equation, the survival probability of the initial state of the two-level atom subjected to frequently repeated measurements can be obtained. The survival probability depends on the time interval between measurements. It is seen that the exponential decay of the system under slowly frequent measurements is presented instead of the naturally oscillatory process. For slowly repeated measurements the atomic population inversion and the survival probability of initial state decline rapidly at the early time and then both of them become unchanged. As the time intervals of the measurements are sufficiently short, the quantum Zeno effect occurs. These results have also shown how the measurement can inhibit the atomic population inversion.