Over the last sixty years, classical information theory has revolutionized the understanding of the nature of information, and how it can be quantified and manipulated. Quantum information processing extends these lessons to quantum systems, where the properties of intrinsic uncertainty and entanglement fundamentally defy classical explanation. This growing field has many potential applications, including computing, cryptography, communication, and metrology. As inherently mobile quantum particles, photons are likely to play an important role in any mature large-scale quantum information processing system. However, the available methods for producing and detecting complex multi-photon states place practical limits on the feasibility of sophisticated optical quantum information processing experiments. In a typical quantum information protocol, a source first produces an interesting or useful quantum state (or set of states), perhaps involving superposition or entanglement. Then, some manipulations are performed on this state, perhaps involving quantum logic gates which further manipulate or entangle the intial state. Finally, the state must be detected, obtaining some desired measurement result, e.g., for secure communication or computationally efficient factoring. The work presented here concerns the first and last stages of this process as they relate to photons: sources and detectors. Our work on sources is based on the need for optimized non-classical states of light delivered at high rates, particularly of single photons in a pure quantum state. We seek to better understand the properties of spontaneous parameteric downconversion (SPDC) sources of photon pairs, and in doing so, produce such an optimized source. We report an SPDC source which produces pure heralded single photons with little or no spectral filtering, allowing a significant rate enhancement. Our work on detectors is based on the need to reliably measure single-photon states. We have focused on optimizing the detection efficiency of visible light photon counters (VLPCs), a single-photon detection technology that is also capable of resolving photon number states. We report a record-breaking quantum efficiency of 91 +/- 3% observed with our detection system. Both sources and detectors are independently interesting physical systems worthy of study, but together they promise to enable entire new classes and applications of information based on quantum mechanics.
Over the last sixty years, classical information theory has revolutionized the understanding of the nature of information, and how it can be quantified and manipulated. Quantum information processing extends these lessons to quantum systems, where the properties of intrinsic uncertainty and entanglement fundamentally defy classical explanation. This growing field has many potential applications, including computing, cryptography, communication, and metrology. As inherently mobile quantum particles, photons are likely to play an important role in any mature large-scale quantum information processing system. However, the available methods for producing and detecting complex multi-photon states place practical limits on the feasibility of sophisticated optical quantum information processing experiments. In a typical quantum information protocol, a source first produces an interesting or useful quantum state (or set of states), perhaps involving superposition or entanglement. Then, some manipulations are performed on this state, perhaps involving quantum logic gates which further manipulate or entangle the intial state. Finally, the state must be detected, obtaining some desired measurement result, e.g., for secure communication or computationally efficient factoring. The work presented here concerns the first and last stages of this process as they relate to photons: sources and detectors. Our work on sources is based on the need for optimized non-classical states of light delivered at high rates, particularly of single photons in a pure quantum state. We seek to better understand the properties of spontaneous parameteric downconversion (SPDC) sources of photon pairs, and in doing so, produce such an optimized source. We report an SPDC source which produces pure heralded single photons with little or no spectral filtering, allowing a significant rate enhancement. Our work on detectors is based on the need to reliably measure single-photon states. We have focused on optimizing the detection efficiency of visible light photon counters (VLPCs), a single-photon detection technology that is also capable of resolving photon number states. We report a record-breaking quantum efficiency of 91 +/- 3% observed with our detection system. Both sources and detectors are independently interesting physical systems worthy of study, but together they promise to enable entire new classes and applications of information based on quantum mechanics.
Over a century after the modern prediction of the existence of individual particles of light by Albert Einstein, a reliable source of this simple quantum state of one photon does not exist. While common light sources such as a light bulb, LED, or laser can produce a pulse of light with an average of one photon, there is (currently) no way of knowing the number of photons in that pulse without first absorbing (and thereby destroying) them. Spontaneous parametric down-conversion, a process in which one high-energy photon splits into two lower-energy photons, allows us to prepare a single-photon state by detecting one of the photons, which then heralds the existence of its twin. This process has been the workhorse of quantum optics, allowing demonstrations of a myriad of quantum processes and protocols, such as entanglement, cryptography, superdense coding, teleportation, and simple quantum computing demonstrations. All of these processes would benefit from better engineering of the underlying down-conversion process, but despite significant effort (both theoretical and experimental), optimization of this process is ongoing. The focus of this work is to optimize certain aspects of a down-conversion source, and then use this tool in novel experiments not otherwise feasible. Specifically, the goal is to optimize the heralding efficiency of the down-conversion photons, i.e., the probability that if one photon is detected, the other photon is also detected. This source is then applied to two experiments (a single-photon source, and a quantum cryptography implementation), and the detailed theory of an additional application (a source of Fock states and path-entangled states, called N00N states) is discussed, along with some other possible applications.
Light is composed of photons, but only recently has it become relatively common, albeit still challenging, to manipulate single or few photons. This special issue presents state-of-the-art theory and experiment concerning the production of few-photon states of light, processing the states, and performing highly sensitive low-noise detection at the single-photon level. In many cases, the connection between photon manipulation and quantum information science is apparent. Few-photon sources have applications for quantum cryptography and optical quantum computing. Photon processing can involve producing entangled states of light as resources for quantum information processing, performing optical gates for example by interferometry, and realizing quantum memory to store information and synchronize gate operations. Ultimately the photons are carriers of information, and this information is acquired by detectors, which have to be reliable, highly sensitive, fast and operate with low noise. Many of these photon generation, processing and detection issues are exemplified in the papers presented here. This special issue thus serves as a compendium of recent results in the area of few-photon optics, covering the development of new sources, the characterization and improvement of detection schemes, and the analysis and proposal of processing protocols. We trust that this issue will serve as a valuable resource for the community for years to come.
Single photons - discrete wavepackets of light - are one of the most fundamental entities in physics. In recent years, the ability to consistently create and manipulate both single photons and pairs of photons has facilitated everything from tests of quantum theory to the implementation of quantum-enhanced precision measurements. These activities all fall within the scope of the rapidly-growing field of quantum information - the exploitation of the properties of quantum states (and specifically their capability to exist in superpositions) to accomplish tasks that would not be possible with classical objects. One stated goal of research in quantum information is to build a device consisting of a network of quantum logic gates that can evaluate quantum algorithms. The photonic implementation of individual logic gates has already been demonstrated. However, partly due to standard methods of preparing single photons, current schemes have severe limitations in terms of scaling up from a single logic gate to multiple concatenated operations. Until now it has not been proven that single photons can be generated in pure and indistinguishable quantum states, something upon which the successful operation of optical quantum logic gates relies. This thesis presents an experimental demonstration of simultaneous generation of almost identical single photons in highly pure states from two independent sources based on parametric downconversion. This is a process of photon pair generation during the passage of a light beam through a nonlinear crystal; one photon from the resulting pair is detected to herald the other. The work herein describes, refines, and implements a technique that minimises the strong quantum correlations usually present within each pair by spectral engineering of the source. This allows the heralded single photons to be in pure states, a property that is confirmed by observing a high-visibility two-photon interference effect without spectral filtering.
This thesis presents experimental progress towards highly efficient generation of cavity- enhanced, narrow-band multiphotons using spontaneous parametric downconversion. It also suggests theoretical proposals for new applications of multiphoton sources in quantum information technology. Photons prepared in Fock states, with a well-defined number of particles, are the essence of the quantum nature of light, and their unique nonclassical properties help us to develop quantum information technology. The generation of Fock states has been most commonly achieved by using spontaneous parametric down-conversion (SPDC) through the χ(2) nonlinearity in bulk crystals. During the SPDC process the nonlinear crystal emits photon-number correlated modes, and a photon-number- resolving measurement in one mode heralds the preparation of the other mode in a Fock state. The fidelity and the success rate of Fock state generation is limited by the multimode nature of SPDC emission. In this thesis, I will investigate the use of cavity-enhanced SPDC modes for higher fidelity photon pair generation, in which the well defined mode of the cavity is enhanced and results in the narrow-band source of the heralded single-photons with up to 80% heralding efficiency. The heralding efficiency is defined as the ratio between number of coincidences and single events on the heralding mode. The photon-number-resolving ability of high-quantum-efficiency transition edge sensors is used for the heralding and detection. We further discuss the feasibility of Fock state generation with higher photon numbers upon improving the data acquisition and analysis techniques. We also demonstrate and implement an interferometry scheme that exploit the phase of the photon and is capable of reading boundless bits of digital information using a single photon. This thesis also introduces new theoretical proposals for using Fock states to obtain quantum advantages for various quantum information applications, here to increase the efficiency in reading out information stored in a classical digital memory and to discriminate optical phases with lower error rates than is feasible with classical protocols.
This dissertation explores the role of optimized resources in facilitating efficient optical quantum information processing and sensing. Three key applications are considered: quantum interferometry, detector characterization, and multi-photon processing. For each application, we examine the underlying quantum resource states and quantum technology resources. Careful attention is paid to how these resources can be optimized to maximize the efficiency of the overarching application in terms of resources consumed, whether photonic, temporal, or infrastructural. Such optimization is an important step in fully realizing the potential of quantum science as it emerges from the laboratory and into the mainstream. For quantum interferometry, we investigate the traditional trade-offs between two-photon quantum interference and single-photon classical interference in terms of measurement resolution and resilience against optical loss and background. We show how we can overcome these trade-offs by replacing conventional single photons with highly non-degenerate energy-entangled photons, which are more optimized for achieving high information content on a per-photon basis. In combination with a specialized dual-wavelength interferometer, our high per-photon information efficiency allows us to achieve nanometer-scale resolution in a matter of seconds with only O(10^4) photon pairs. We then show how this entanglement-enhanced quantum sensing modality can allow for new studies in challenging regimes, such as characterizing lossy thin films or detecting distant vibrations. Then, for detector characterization, we consider the instrumental role of photon detectors in various optical quantum science protocols. As these protocols expand into spectral bands with growing technological applications, such as the mid-infrared, there is a developing need to characterize suitable detectors, with their efficiencies being one of the most important metrics. Typical methods for efficiency characterization, whether classical or quantum, can face the challenge of being infrastructure-intensive, with some requiring resources such as independent reference standards or large bulk-optics apparatuses. To help realize a resource-efficient characterization system for mid-infrared detectors, we have developed a compact and portable solution involving highly non-degenerate photon pairs produced by a fiber-coupled waveguide device. We evaluate the performance of early prototypes and identify next steps for improved device engineering. Lastly, for multi-photon processing, we focus on the single-photon source, given its key role in preparing the required photonic states. From a scalability perspective, efficient single-photon generation is essential for performing many large-scale multi-photon protocols within useful timescales. To meet this requirement, we explore how multiplexing techniques allow us to pair heralded single photons with photon routing, storage, and counting technologies to realize an efficient single-photon source. We then discuss our efforts to implement and integrate optimized versions of these technologies to address limitations faced by earlier implementations with regard to preparing pure single photons at a high rate. This discussion includes an in-depth analysis of our work related to realizing an efficient photon-number-resolving detector.
Two important challenges in quantum photonics are to generate useful states with high fidelity, and to detect them and verify their properties. Particularly valuable states are single photons and entangled photon pairs in well-defined optical modes, as they can be used in many quantum information protocols or used to build up more complex states. For sources, we employ integrated nonlinear optics (waveguides in lithium niobite and potassium titanyl phosphate) to maximize brightness and go beyond what is possible in bulk optics, showing simultaneously high state fidelity, heralding efficiency, and spectral purity across three experiments: first we show record heralding efficiency in a fully-fibered heralded single-photon source, and use it to probe the tradeoff between spectral purity and heralding efficiency in non-engineered sources. With an engineered source, we then herald up to 50 photons in a nonclassical state. The last source is for polarization-entangled photon pairs, with brightness of 3.5 million pairs/s·mW, fidelity to a Bell state of 96%, heralding efficiency of 43%, and HOM interference visibility of 82%. Once a complex state is constructed, it must also be verified. For this we employ a time-multiplexed detector consisting of a fibre loop and a single-photon detector. Surprisingly, we are able to extract information even in the saturation regime of the detector. We use the click statistics of the time-multiplexed detector to verify the non-classicality of quantum light, and we use its extremely high dynamic range (123 dB) to measure a macroscopic power level with a single-photon detector. Eliminating calibrated attenuators with this approach will allow direct standardization of quantum and classical optical power levels.