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Waveguide Sources of Photon Pairs

Rolf T. Horn

Published May 4, 2011• 2 citations
OpenAlex

Abstract

This thesis describes various methods for producing photon pairs from waveguides. It covers relevant topics such as waveguide coupling and phase matching, along with the relevant measurement techniques used to infer photon pair production. A new proposal to solve the phase matching problem is described along with two conceptual methods for generating entangled photon pairs. Photon pairs are also experimentally demonstrated from a third novel structure called a Bragg Reflection Waveguide (BRW). \n \nThe new proposal to solve the phase matching problem is called Directional Quasi-Phase Matching (DQPM). It is a technique that exploits the directional dependence of the non-linear susceptiblity ($\\chi^{(2)}$) tensor. It is aimed at those materials that do not allow birefringent phase-matching or periodic poling. In particular, it focuses on waveguides in which the interplay between the propagation direction, electric field polarizations and the nonlinearity can change the strength and sign of the nonlinear interaction periodically to achieve quasi-phasematching. \n \nOne of the new conceptual methods for generating entangled photon pairs involves a new technique that sandwiches two waveguides from two differently oriented but similar crystals together. The idea stems from the design of a Michelson interferometer which interferes the paths over which two unique photon pair processes can occur, thereby creating entanglement in any pair of photons created in the interferometer. By forcing or sandwiching the two waveguides together, the physical space that exists in the standard Micheleson type interferometer is made non-existent, and the interferometer is effectively squashed. The result is that the two unique photon pair processes actually occupy the same physical path. This benefits the stability of the interferometer in addition to miniaturizing it. The technical challenges involved in sandwiching the two waveguides are briefly discussed. \n \nThe main result of this thesis is the observation of photon pairs from the BRW. By analyzing the time correlation between two single photon detection events, spontaneous parametric down conversion (SPDC) of a picosecond pulsed ti:sapph laser is demonstrated. The process is mediated by a ridge BRW. The results show evidence for type-0, type-I and type-II phase matching of pump light at 783nm, 786nm and 789nm to down converted light that is strongly degenerate at 1566nm, 1572nm, and 1578nm respectively. The inferred efficiency of the BRW was 9.8$\\cdot$10$^{-9}$ photon pairs per pump photon. This contrasts with the predicted type-0 efficiency of 2.65$\\cdot$10$^{-11}$. This data is presented for the first time in such waveguides, and represents significant advances towards the integration of sources of quantum information into the existing telecommunications infrastructure.

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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Mar 29, 2013•0 citations
This thesis describes various methods for producing photon pairs from waveguides. It covers relevant topics such as waveguide coupling and phase matching, along with the relevant measurement techniques used to infer photon pair production. A new proposal to solve the phase matching problem is described along with two conceptual methods for generating entangled photon pairs. Photon pairs are also experimentally demonstrated from a third novel structure called a Bragg Reflection Waveguide (BRW). \n \nThe new proposal to solve the phase matching problem is called Directional Quasi-Phase Matching (DQPM). It is a technique that exploits the directional dependence of the non-linear susceptiblity (chi(2)\\chi^{(2)}chi(2)) tensor. It is aimed at those materials that do not allow birefringent phase-matching or periodic poling. In particular, it focuses on waveguides in which the interplay between the propagation direction, electric field polarizations and the nonlinearity can change the strength and sign of the nonlinear interaction periodically to achieve quasi-phasematching. \n \nOne of the new conceptual methods for generating entangled photon pairs involves a new technique that sandwiches two waveguides from two differently oriented but similar crystals together. The idea stems from the design of a Michelson interferometer which interferes the paths over which two unique photon pair processes can occur, thereby creating entanglement in any pair of photons created in the interferometer. By forcing or sandwiching the two waveguides together, the physical space that exists in the standard Micheleson type interferometer is made non-existent, and the interferometer is effectively squashed. The result is that the two unique photon pair processes actually occupy the same physical path. This benefits the stability of the interferometer in addition to miniaturizing it. The technical challenges involved in sandwiching the two waveguides are briefly discussed. \n \nThe main result of this thesis is the observation of photon pairs from the BRW. By analyzing the time correlation between two single photon detection events, spontaneous parametric down conversion (SPDC) of a picosecond pulsed ti:sapph laser is demonstrated. The process is mediated by a ridge BRW. The results show evidence for type-0, type-I and type-II phase matching of pump light at 783nm, 786nm and 789nm to down converted light that is strongly degenerate at 1566nm, 1572nm, and 1578nm respectively. The inferred efficiency of the BRW was 9.8cdot\\cdotcdot10−9^{-9}−9 photon pairs per pump photon. This contrasts with the predicted type-0 efficiency of 2.65cdot\\cdotcdot10−11^{-11}−11. This data is presented for the first time in such waveguides, and represents significant advances towards the integration of sources of quantum information into the existing telecommunications infrastructure.
In this thesis, I overcome the challenges and fill the gaps in knowledge for the design and analysis of photonic crystal slab waveguides (PCSWs) as spontaneous parametric down-conversion (SPDC) sources of photon-pairs, as well as to investigate their potential for engineering the properties of the photon-pair quantum state. I have developed the required formalism for analyzing both the quantum process of SPDC and its classical counterpart of second-harmonic generation (SHG). In studying SHG, I verified my formalism through comparing its results with direct nonlinear simulations. In these formulations, special attention was given to treating lossy modes, as they prove to be an inherent part of the SPDC designs in PCSWs. Moreover, I have found a practical set of PCSW designs, phase-matched for three-wave-mixing processes, while demonstrating that PCSWs can offer a strong control over the phase-matching configuration. This includes reaching phase-matching between modes of different propagation directions, reaching simultaneous phase-matching between multiple processes, and controlling the group velocity of the modes at the point of phase-matching. These capabilities proved to be the key to discovering the unique strength of PCSWs for the SPDC application. Through the use of various phase-matching configurations, I showed how compact SPDC sources can be designed using PCSWs that are capable of creating entanglement and tuning its extent in different degrees of freedom, with specific examples for path and spectral degrees of entanglement, all in a fully integrated way and directly at the generation step. This work also includes my experimental results on characterizing lithium niobate nanostructured ridge waveguides, demonstrating phase-matched SHG. Finally, I propose the concept of atom-mediated SPDC, for interfacing a single-emitter source with a photon-pair source, relying on the bandgap evanescent modes of a periodic waveguide.
We report the observation of polarization entangled photon pairs generated by means of type-II spontaneous parametric down-conversion (SPDC) within an Al x Ga 1-x As Bragg reflection waveguide (BRW).Even though SPDC in BRW had been observed before, the photons detected were not entangled in the polarization degree of freedom.As a necessary previous step, we also characterized the phasematching properties of the waveguides designed by means of the nonlinear process of second-harmonic generation (SHG).
Entanglement is the hallmark of quantum mechanics. Quantum entanglement -- putting two or more identical particles into a non-factorable state -- has been leveraged for applications ranging from quantum computation and encryption to high-precision metrology. Entanglement is a practical engineering resource and a tool for sidestepping certain limitations of classical measurement and communication. Engineered nonlinear optical waveguides are an enabling technology for generating entangled photon pairs and manipulating the state of single photons. This dissertation reports on: i) frequency conversion of single photons from the mid-infrared to 843nm as a tool for incorporating quantum memories in quantum networks, ii) the design, fabrication, and test of a prototype broadband source of polarization and frequency entangled photons; and iii) a roadmap for further investigations of this source, including applications in quantum interferometry and high-precision optical metrology. \n \nThe devices presented herein are quasi-phase-matched lithium niobate waveguides. Lithium niobate is a second-order nonlinear optical material and can mediate optical energy conversion to different wavelengths. This nonlinear effect is the basis of both quantum frequency conversion and entangled photon generation, and is enhanced by i) confining light in waveguides to increase conversion efficiency, and ii) quasi-phase matching, a technique for engineering the second-order nonlinear response by locally altering the direction of a material's polarization vector. Waveguides are formed by diffusing titanium into a lithium niobate wafer. Quasi-phase matching is achieved by electric field poling, with multiple stages of process development and optimization to fabricate the delicate structures necessary for broadband entangled photon generation. \n \nThe results presented herein update and optimize past fabrication techniques, demonstrate novel optical devices, and propose future avenues for device development. Quantum frequency conversion from 1848nm to 843nm is demonstrated for the first time, with >75% single-photon conversion efficiency. A new electric field poling methodology is presented, combining elements from multiple historical techniques with a new fast-feedback control system. This poling technique is used to fabricate the first chirped-and-apodized Type-II quasi-phase-matched structures in titanium-diffused lithium niobate waveguides, culminating in a measured phasematching spectrum that is predominantly Gaussian (R^2 = 0.80), nearly eight times broader than the unchirped spectrum, and agrees well with simulations.
AlGaAs Bragg reflection waveguides are promising systems for the generation of single and entangled photons through the process of spontaneous parametric down-conversion (SPDC) [1]. We use a type II SPDC process where the downconverted photons are orthogonally polarized. The produced photons are inherently polarization-entangled eliminating the need for any additional entanglement setup. The material AlGaAs is our preferred choice as a nonlinear medium because it features a high nonlinear coefficient allowing for room temperature operation and has the advantage of being a non-birefringent material. Further, the material platform allows for the direct integration of a pump laser into the same chip.
This thesis deals with the production of entangled photons using spontaneous parametric down-conversion (SPDC). We start with a short overview of some important theoretical concepts. First we provide a brief reminder of the theory of entanglement. We then discuss how the state of quantum systems can be determined using quantum state tomography. We also explain SPDC, the physical process which we use to produce entangled photons. Finally, we give an overview of the methods which have been used to produce entangled photons in the past, both for two- and three-photon entanglement. \n \nThe first experiment is the design of an efficient source of entangled photon pairs based on a polarizing Sagnac interferometer configuration. With this configuration, we can use quasi-phasematched materials which allow for higher efficiencies than standard bulk nonlinear materials. The source is pumped by a low-power continuous-wave laser diode, and produces degenerate photon pairs at 809nm. It has a spectral brightness of 87,500 pairs/(s mW nm), and the fidelity of the produced quantum states with a Bell state is 98.9%. The source is used for experiments in quantum key distribution, cluster state quantum computing, remote state preparation, state discrimination, and entanglement-enhanced classical communication. \n \nThe second experiment discussed in this thesis is the generation of photon triplets using cascaded SPDC. In this experiment, a primary SPDC source is pumped with a low-power, continuous-wave laser diode, producing photon pairs. Single photons from these pairs serve as the pump for a second down-conversion, resulting in photon triplets. This is the first demonstration of the direct production of photon triplets, and the first observation of SPDC at the single photon level. This method could potentially be used to produce entangled photon triplets without post-selection, and as a source of triggered Bell pairs.
We demonstrate efficient photon pair generation for quantum communication using an all-semiconductor approach. In an AlGaAs Bragg-reflection waveguide we employ spontaneous parametric down-conversion to produce photon pairs at telecommunication wavelengths. The various phase-matching solutions present in our device can be used to create timebin or polarization entanglement. This approach can to lead to a fully integrated photon pair source with the pump laser, active and passive optical devices all on a single semiconductor chip.