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Direct generation of three-photon entanglement using cascaded downconversion

Deny R. Hamel

Published Dec 6, 2013• 0 citations
OpenAlex

Abstract

High quality entangled photon sources are a key requirement for many promising quantum optical technologies. However, the production of multi-photon entangled states with good fidelity is challenging. Current sources of multi-photon entanglement require the use of post-selection, which limits their usefulness for some applications. It has been an open challenge to create a source capable of directly producing three-photon entanglement. An important step in this direction was achieved with the demonstration of photon triplets produced by a new process called cascaded downconversion, but these previous measurements were not sufficient to show whether these photons were in an entangled state and only had detection rates of five triplets per hour. In this thesis, we show the first demonstration of a direct source of three-photon entanglement. Our source is based on cascaded downconversion, and we verify that it produces genuine tripartite entanglement in two degrees of freedom: energy-time and polarization. \n \nThe energy-time entanglement is similar to a three-particle generalization of an Einstein-Podolski-Rosen state; the three photons are created simultaneously, yet the sum of their energies is well defined, which is an indication of energy-time entanglement. To prove it, we use time-bandwidth inequalities which check for genuine tripartite entanglement. Our measurements show that the state violates the inequalities with what constitute, to the best of our knowledge, the strongest violation of time-bandwidth inequalities in a tripartite continuous-variable system to date. \n \nWe create polarization entanglement by modifying our experimental setup so that two downconversion processes producing orthogonally polarized triplets interfere to create Greenberger-Horne-Zeilinger states. By using highly efficient superconducting nanowire single photon detectors, we improve the detected triplet rate by 2 orders of magnitude to 660 triplets per hour. We characterize the state using quantum state tomography, and find a fidelity of 86\\% with the ideal state, beating the previous best value for a three-photon entangled state fidelity measured by tomography. We also use the state to perform two tests of local realism. We violate the Mermin and Svetlichny inequalities by 10 and 5 standard deviations respectively, the latter being the strongest violation to date. Finally, we show that, unlike previous sources of tree-photon entanglement, our source can be used as a source of heralded Bell pairs. We demonstrate this by measuring a CHSH inequality with the heralded Bell pairs, and by reconstructing their state using quantum state tomography.

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High quality entangled photon sources are a key requirement for many promising quantum optical technologies. However, the production of multi-photon entangled states with good fidelity is challenging. Current sources of multi-photon entanglement require the use of post-selection, which limits their usefulness for some applications. It has been an open challenge to create a source capable of directly producing three-photon entanglement. An important step in this direction was achieved with the demonstration of photon triplets produced by a new process called cascaded downconversion, but these previous measurements were not sufficient to show whether these photons were in an entangled state and only had detection rates of five triplets per hour. In this thesis, we show the first demonstration of a direct source of three-photon entanglement. Our source is based on cascaded downconversion, and we verify that it produces genuine tripartite entanglement in two degrees of freedom: energy-time and polarization. \n \nThe energy-time entanglement is similar to a three-particle generalization of an Einstein-Podolski-Rosen state; the three photons are created simultaneously, yet the sum of their energies is well defined, which is an indication of energy-time entanglement. To prove it, we use time-bandwidth inequalities which check for genuine tripartite entanglement. Our measurements show that the state violates the inequalities with what constitute, to the best of our knowledge, the strongest violation of time-bandwidth inequalities in a tripartite continuous-variable system to date. \n \nWe create polarization entanglement by modifying our experimental setup so that two downconversion processes producing orthogonally polarized triplets interfere to create Greenberger-Horne-Zeilinger states. By using highly efficient superconducting nanowire single photon detectors, we improve the detected triplet rate by 2 orders of magnitude to 660 triplets per hour. We characterize the state using quantum state tomography, and find a fidelity of 86\% with the ideal state, beating the previous best value for a three-photon entangled state fidelity measured by tomography. We also use the state to perform two tests of local realism. We violate the Mermin and Svetlichny inequalities by 10 and 5 standard deviations respectively, the latter being the strongest violation to date. Finally, we show that, unlike previous sources of tree-photon entanglement, our source can be used as a source of heralded Bell pairs. We demonstrate this by measuring a CHSH inequality with the heralded Bell pairs, and by reconstructing their state using quantum state tomography.
Stable sources of entangled photons are important requirements for quantum communications. In recent years, cascaded down-conversion has been demonstrated as an effective method of directly producing three-photon entanglement. However, to produce polarization entanglement these sources have until now relied on intricate active phase stabilization schemes, thus limiting their robustness and usability. In this paper, we present a completely phase-stable source of three-photon entanglement in the polarization degree of freedom. With this source, which is based on a cascade of two pair sources based on Sagnac configurations, we produce states with over 96% fidelity with an ideal Greenberger-Horne-Zeilinger state. Moreover, we demonstrate the stability of the source over several days without any ongoing optimization. We expect this source to be a useful tool for applications requiring multiphoton entanglement, such as quantum secret sharing and producing heralded entangled photon pairs.
This thesis deals with the production of entangled photons using spontaneous parametric down-conversion (SPDC). We start with a short overview of some important theoretical concepts. First we provide a brief reminder of the theory of entanglement. We then discuss how the state of quantum systems can be determined using quantum state tomography. We also explain SPDC, the physical process which we use to produce entangled photons. Finally, we give an overview of the methods which have been used to produce entangled photons in the past, both for two- and three-photon entanglement. \n \nThe first experiment is the design of an efficient source of entangled photon pairs based on a polarizing Sagnac interferometer configuration. With this configuration, we can use quasi-phasematched materials which allow for higher efficiencies than standard bulk nonlinear materials. The source is pumped by a low-power continuous-wave laser diode, and produces degenerate photon pairs at 809nm. It has a spectral brightness of 87,500 pairs/(s mW nm), and the fidelity of the produced quantum states with a Bell state is 98.9%. The source is used for experiments in quantum key distribution, cluster state quantum computing, remote state preparation, state discrimination, and entanglement-enhanced classical communication. \n \nThe second experiment discussed in this thesis is the generation of photon triplets using cascaded SPDC. In this experiment, a primary SPDC source is pumped with a low-power, continuous-wave laser diode, producing photon pairs. Single photons from these pairs serve as the pump for a second down-conversion, resulting in photon triplets. This is the first demonstration of the direct production of photon triplets, and the first observation of SPDC at the single photon level. This method could potentially be used to produce entangled photon triplets without post-selection, and as a source of triggered Bell pairs.
Non-classical states of light are of fundamental importance for emerging quantum technologies. All optics experiments producing multi-qubit entangled states have until now relied on outcome post-selection, a procedure where only the measurement results corresponding to the desired state are considered. This method severely limits the usefulness of the resulting entangled states. fiere, we show the direct production of polarization- entangled photon triplets by cascading two entangled down-conversion processes[1]. First, a Sagnac source [2] produces non-degenerate entangled photon pairs at 776 nm and 842 nm in a Bell state. The 776 nm photon is sent through a polarizing Mach-Zehnder interferometer with a down-conversion crystal in each arm. If it is down-converted, a photon pair is created in modes 2 and 3 with a polarization state depending on the pump photon. The quantum stete describing the photon triplets is:
We lay down a general scheme to quantify the amount of genuine tripartite entanglement present in the spatial and energy-time degrees of freedom of entangled photon triplets using a resource-based measure known as the tripartite entanglement of formation. Quantifying genuine tripartite entanglement relative to a number of maximally entangled three-qubit Greenberger-Horne-Zeilinger (GHZ) states called gebits, the tripartite entanglement of formation serves as a basis of comparison between different tripartite entangled states of differing dimension. Demonstrating genuine tripartite entanglement is doubly challenging because it is not enough to show that each party is inseparable from the other two (which is sufficient only for pure states). Instead, one must rule out all mixtures of all combinations of biseparable states from describing the tripartite state. To meet this challenge, we use entropic measures of the statistics of tripartite systems to simultaneously bound the correlations each party has with the other two, and in so doing place a lower limit to the tripartite entanglement of formation. Even though our measure never over-estimates the entanglement present, we estimate the effectiveness of our technique by determining the exact tripartite entanglement of a triple-gaussian triphoton wavefunction with the same correlations as seen in photon triplets generated in third-order spontaneous parametric down-conversion (SPDC). Between these two efforts, we show that a substantial amount of tripartite entanglement exists in both the spatial and energy-time degrees of freedom of these systems, and propose an experiment that can measure them.
Cascaded down conversion has been demonstrated as an effective method of directly producing three-photon entanglement. Until now, these sources have relied on intricate active phase stabilization schemes. In this work, we present a completely phase-stable source of three-photon entanglement in the polarization degree of freedom. We produce states with over 96% fidelity with an ideal Greenberger-Horn-Zeilinger state. Moreover, we demonstrate the stability of the source over several days without any ongoing optimization.