Motivated by correlated decay processes producing gain, loss, and lasing in driven semiconductor quantum dots [Phys. Rev. Lett. 113, 036801 (2014); Science 347, 285 (2015); Phys. Rev. Lett. 114, 196802 (2015)], we develop a theoretical technique by using Keldysh diagrammatic perturbation theory to derive a Lindblad master equation that goes beyond the usual second-order perturbation theory. We demonstrate the method on the driven dissipative Rabi model, including terms up to fourth order in the interaction between the qubit and both the resonator and environment. This results in a large class of Lindblad dissipators and associated rates which go beyond the terms that have previously been proposed to describe similar systems. All of the additional terms contribute to the system behavior at the same order of perturbation theory. We then apply these results to analyze the phonon-assisted steady-state gain of a microwave field driving a double quantum dot in a resonator. We show that resonator gain and loss are substantially affected by dephasing-assisted dissipative processes in the quantum-dot system. These additional processes, which go beyond recently proposed polaronic theories, are in good quantitative agreement with experimental observations.
We present a unified many-body perturbation theory for open quantum systems that treats dissipation, correlations, and external driving on equal footing. Using a Keldysh-Lindblad formalism, we introduce a diagrammatic treatment of dissipative interaction lines representing quasiparticle flows and fluctuations. Two new Feynman rules render the evaluation of dissipative diagrams compact and systematically improvable, while preserving the Keldysh and anti-Hermitian symmetries of the closed-system theory. Consequently, the structure of the Kadanoff-Baym equations remains unchanged, enabling existing numerical methods to be directly applied. To illustrate this, we derive dissipative versions of the second Born and GW approximations and identify the physical content of the self-energy components. Moreover, we demonstrate that time-linear approximations to the full Kadanoff-Baym equations retain their closed-form structure and can be efficiently used to simulate relaxation and decoherence dynamics. The impact of dissipation-induced correlations is illustrated in the driven Haldane model, where quasiparticles exhibit nontrivial stabilization and acquire lifetimes that far exceed those of the bare system. This framework establishes a general route toward first-principles modeling of correlated, driven, and dissipative quantum materials.
Driven-dissipative qubit-resonator dynamics, which are the basis of most dispersive superconducting qubit measurement schemes, are often modeled with Lindblad master equations built from subsystem local jump operators, even when the qubit and resonator are appreciably hybridized. In this work we revisit this setting using a microscopic Bloch-Redfield approach, where dissipation is constructed in the eigenbasis of the coupled qubit-resonator Hamiltonian with a complete, frequency dependent, open system description of the transmission line environment. Here, we show that the Lindblad and Bloch-Redfield decay rates can be quantitatively different in the absence of driving, while in the driven case we demonstrate that the time-independent Redfield dissipator and its time-dependent generalization can show qualitatively different behaviors as a function of driving strength. Finally, we investigate the effects of driving in structured spectral densities, recovering the suppression of measurement-induced relaxation in the presence of a so called Purcell filter.
The extraordinary quantum properties of nonequilibrium systems governed by dissipative dynamics have become a focal point in contemporary scientific inquiry. The nonequilibrium Green's functions (NEGF) theory provides a versatile method for addressing driven nondissipative systems, utilizing the powerful diagrammatic technique to incorporate correlation effects. We here present a second-quantization approach to the dissipative NEGF theory, reformulating Keldysh ideas to accommodate Lindbladian dynamics and extending the Kadanoff-Baym equations accordingly. Generalizing diagrammatic perturbation theory for many-body Lindblad operators, the formalism enables correlated and dissipative real-time simulations for the exploration of transient and steady-state changes in the electronic, transport, and optical properties of materials.
We construct Feynman rules for Lindblad master equations in the operator language of quantum optics: a fixed algebra of elementary operator moves and closed-form propagators for perturbation theory about an exactly solvable, in most cases Gaussian, generator. The expansion separates into a kinematic part (the shift algebra on the Wick-ordered eigenoperators
Omn=:(c†)mcn:, from which the vertex table for a specified interaction is assembled) and a dynamical part that enters only through the resolvent of the unperturbed generator, diagonal and additive for any stable, diagonalizable Gaussian
L0, including thermal and squeezed reservoirs and correlated decay, and equally available for a two-level emitter, driven or undriven. In the driven Kerr cavity the loop expansion is the semiclassical expansion and the series is asymptotic. In a strongly driven two-level atom, dressed lines replace a series of finite radius by one accurate deep into saturation, one line per Mollow component. For Kerr rings and chains the cost is polynomial in the number of sites at fixed perturbative order. On a three-site ring the diagrams recover the non-Gaussian part of the three-photon correlation that the Gaussian cumulant closure lacks; carried to tenth order they give the smallest
g(3) error of the methods compared for
U≤0.25κ at a cost below that of a fourth-order closure, and third- and fourth-order closures are more accurate at moderate coupling. The same rules, extended to the counting-field-tilted generator, give the photon-counting cumulants of a disordered eight-site chain beyond direct diagonalization; quantum-jump trajectories at three couplings agree with them to within
1.6 standard errors, within one at the strongest coupling, where they place the third cumulant six standard errors above the Gaussian value.
We develop a recursive perturbative expansion for the time-convolutionless generator of an open quantum system in a generalized Lindblad form. This formulation provides a systematic approach to derive the generator at arbitrary order while preserving a Lindblad-like structure, without imposing assumptions on the system or environment beyond an initially uncorrelated state. The generator is written, at all orders, in a canonical form, which also corresponds to the minimal dissipation condition, which uniquely specifies the decomposition of the generator into Hamiltonian and dissipative contributions. To validate the method and show its effectiveness in addressing non-Markovian dynamics and strong-coupling effects, we compute the generator explicitly up to fourth order.