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Optica

Toward quantum plasmonic networks

Matthew Holtfrerich, Mohammadjavad Dowran, Roderick B. Davidson, Benjamin J. Lawrie, Raphael C. Pooser, Alberto M. Marino

Published Aug 26, 2016• 56 citations
Publisher

Abstract

Here, we demonstrate the transduction of macroscopic quantum entanglement by independent, distant plasmonic structures embedded in separate thin silver films. In particular, we show that the plasmon-mediated transmission through each film conserves spatially dependent, entangled quantum images, opening the door for the implementation of parallel quantum protocols, super-resolution imaging, and quantum plasmonic sensing geometries at the nanoscale level. The conservation of quantum information by the transduction process shows that continuous variable multi-mode entanglement is momentarily transferred from entangled beams of light to the space-like separated, completely independent plasmonic structures, thus providing a first important step toward establishing a multichannel quantum network across separate solid-state substrates.

DOI
10.1364/optica.3.000985

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We demonstrate the transduction of macroscopic quantum correlations by Ag localized surface plasmons (LSPs). Quantum noise reduction, or squeezed light, generated through four-wave mixing in Rb vapor, is coupled to a Ag nanohole array designed to exhibit LSP-mediated extraordinary-optical transmission spectrally coincident with the squeezed light source at 795 nm. This first demonstration of the coupling of quantum light into LSPs conserves spatially dependent quantum information, allowing for parallel quantum protocols in on-chip subwavelength quantum information processing.
The control of quantum states of light at the nanoscale has become possible in recent years with the use of plasmonics. Here, many types of nanophotonic devices and applications have been suggested that take advantage of quantum optical effects, despite the inherent presence of loss. A key example is quantum plasmonic sensing, which provides sensitivity beyond the classical limit using entangled N00N states and their generalizations in a compact system operating below the diffraction limit. In this work, we experimentally demonstrate the excitation and propagation of a two-plasmon entangled N00N state (N=2) in a silver nanowire, and assess the performance of our system for carrying out quantum sensing. Polarization entangled photon pairs are converted into plasmons in the silver nanowire, which propagate over a distance of 5 um and re-convert back into photons. A full analysis of the plasmonic system finds that the high-quality entanglement is preserved throughout. We measure the characteristic super-resolution phase oscillations of the entangled state via coincidence measurements. We also identify various sources of loss in our setup and show how they can be mitigated, in principle, in order to reach super-sensitivity that goes beyond the classical sensing limit. Our results show that polarization entanglement can be preserved in a plasmonic nanowire and that sensing with a quantum advantage is possible with moderate loss present.
Photonic quantum technologies have been extensively studied in quantum information science, owing to the high-speed transmission and outstanding low-noise properties of photons. However, applications based on photonic entanglement are restricted due to the diffraction limit. In this work, we demonstrate for the first time the maintaining of quantum polarization entanglement in a nanoscale hybrid plasmonic waveguide composed of a fiber taper and a silver nanowire. The transmitted state throughout the waveguide has a fidelity of 0.932 with the maximally polarization entangled state Φ(+). Furthermore, the Clauser, Horne, Shimony, and Holt (CHSH) inequality test performed, resulting in value of 2.495 ± 0.147 > 2, demonstrates the violation of the hidden variable model. Because the plasmonic waveguide confines the effective mode area to subwavelength scale, it can bridge nanophotonics and quantum optics and may be used as near-field quantum probe in a quantum near-field micro/nanoscope, which can realize high spatial resolution, ultrasensitive, fiber-integrated, and plasmon-enhanced detection.
The resonance energy transfer and entanglement between two-level quantum emitters are typically limited to sub-wavelength distances due to the inherently short-range nature of the dipole-dipole interactions. Moreover, the entanglement of quantum systems is hard to preserve for a long time period due to decoherence and dephasing mainly caused by radiative and nonradiative losses. In this work, we outperform the aforementioned limitations by presenting efficient long-range inter-emitter entanglement and large enhancement of resonance energy transfer between two optical qubits mediated by epsilon-near-zero (ENZ) and other plasmonic waveguide types, such as V-shaped grooves and cylindrical nanorods. More importantly, we explicitly demonstrate that the ENZ waveguide resonant energy transfer and entanglement performance drastically outperforms the other waveguide systems. Only the excited ENZ mode has an infinite phase velocity combined with a strong and homogeneous electric field distribution, which leads to a giant energy transfer and efficient entanglement independent of the emitters' separation distances and nanoscale positions in the ENZ nanowaveguide, an advantageous feature that can potentially accommodate multi-qubit entanglement. Moreover, the transient entanglement can be further improved and become almost independent of the detrimental decoherence effect when an optically active (gain) medium is embedded inside the ENZ waveguide. We also present that efficient steady-state entanglement can be achieved by using a coherent external pumping scheme. Finally, we report a practical way to detect the steady-state entanglement by computing the second-order correlation function. The presented findings stress the importance of plasmonic ENZ waveguides in the design of the envisioned on-chip quantum communication and information processing plasmonic nanodevices.