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World Scientific series in 20th century physics

Paper 1.3: N. Bloembergen and Y.R. Shen, “Quantum theoretical comparison of nonlinear susceptibilities in parametric media, lasers and raman lasers,” Phys. Rev. 133, A37–A49, 1964.

Published Sep 1, 1996• 5 citations
Publisher
DOI
10.1142/9789812795793_0003

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Cambridge University Press eBooks•Sep 29, 1995•3 citations
A diagrammatic approach to the theory of nonlinear susceptiblities is developed. Including damping, the steady state nonlinear response functions to several simultaneously applied monochromatic electromagnetic fields are obtained in terms of linear response functions in the weak coupling system. Saturation phenomena in microwave resonance and in parametric processes can be understood as lower order responses in the system with higher spin temperature. The condition for the Raman emission is discussed in some details. Results are compared with previous theories, in particular with that of Bloembergen and Shen. The theory is extended to the case where the spacially inhomogeneous perturbation is imposed.
The steady-state response of a nonlinear medium to several simultaneously applied monochromatic electromagnetic fields is described by the density matrix method. A Fourier series expansion in terms of ascending powers of the amplitudes of the applied fields is especially useful to describe the parametric response in spectral regions, where the absorption is small. As the resonances of the material system are approached, the general formalism exhibits the mixture and interference between parametric processes and single- and multiple-photon absorption and emission processes. previously discussed examples of the two-level and three-level system are generalized. The reaction of the general nonlinear medium on the electromagnetic fields is incorporated.
Introduction We have already encountered situations in which light of one frequency falling on an atomic system gives rise to light of different frequencies (cf. Section 15.6). The atom may here be considered to play the role of a (noisy) nonlinear transducer for the incident field. Even stronger nonlinear effects arise when one is dealing with a large number of atoms, or a nonlinear medium . Under these circumstances it is sometimes permissible to ignore the atomic structure and to treat the medium as a continuum, as in Maxwell's electromagnetic theory. The subject of the interaction of the incident field with the nonlinear medium is usually known as nonlinear optics. The subject had its beginnings in an experiment in which a strong beam of red light (wavelength 6943 Å) from a ruby laser was allowed to fall on a quartz crystal, and a faint beam of blue light at a wavelength of 3472 Å, the first harmonic of the red, was produced (Franken, Hill, Peters and Weinreich, 1961). The development of the subject of nonlinear optics into a mature field is due largely to the work of Bloembergen and his collaborators. In the following we shall consider only a few simple illustrative examples of phenomena in nonlinear optics. More topics and more detail can be found in the books by Bloembergen and others (Bloembergen, 1965; Yariv, 1967, Chap. 21; Shen, 1984; Schubert and Wilhelmi, 1986; Butcher and Cotter, 1990; Boyd, 1992).