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Springer series in optical sciences/SPringer series in optical sciences

Collisionless Multiquantum Ionization of Atomic Species with 193 nm Radiation

T. S. Luk, Herbert Pummer, Kefneth G. Boyer, Mahnaz Shahidi, H. Egger, C. K. Rhodes

Published Jan 1, 1983• 0 citations
Publisher
DOI
10.1007/978-3-540-38814-2_124

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Radiation-field-driven ionization in laser-assisted slow atomic collisions

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It is generally assumed that for ionization processes, which occur in slow atomic collisions, the coupling of the colliding system to the quantum radiation field is irrelevant. Here we show, however, that -- contrary to expectations -- such a coupling can strongly influence ionization of a beam of atomic species A slowly traversing a gas of atomic species B excited by a weak laser field. Moreover, this coupling becomes even more important when the collision velocity increases, getting comparable or exceeding the typical electron orbiting velocities in A and B. Our results imply furthermore that the Breit interaction can, in fact, dominate over the Coulomb interaction at very low energies.

arXiv:2208.09812•Aug 21, 2022•0 citations
We create a dual-species ultracold neutral plasma (UNP) by photo-ionizing Yb and Ca atoms in a dual-species magneto-optical trap. Unlike single-species UNP expansion, these plasmas are well outside of the collisionless (Vlasov) approximation. We observe the mutual interaction of the Yb and Ca ions by measuring the velocity distribution for each ion species separately. We model the expansion using a fluid code including ion-ion friction and compare with experimental results to obtain a value of the Coulomb logarithm of Λ= 0.04.
The first simultaneous cooling and confinement of two different atomic species from opposite sides of the periodic table in a dual magneto optical trap (DMOT) has been accomplished. The alkali-metal 85Rb and the noble gas 40Ar* have been simultaneously confined, characterized, and interspecies interaction parameters have been measured. The DMOT confined 1.2 × 106 85Rb atoms at a density of 1 × 1010/cm3 and 1.4 × 106 40Ar* atoms with a density of 1.2 × 1010/cm3. A collisional loss rate coefficient for Rb-Ar* has been determined to be γRb-Ar, = (4.8 ± 1.6) × 10−11cm3/s. A typical reduction of 3% of the florescence of the trapped 85Rb was observed when the 40Ar* trap was present. The loss of atoms from the dual trap is presumed to be caused by radiative escape and ionization losses, for an 40Ar* MOT it is due to Penning and associative ionization losses. An Ar* PI/AI ionization ratio of 6.7 ± 3.6 was determined, which makes the Penning ionization rate the dominant loss mechanism. The ionization rate was obtained with a SRS RGA200 mass spectrum analyzer specifically modified to work in conjunction with an ion optical field plate setup to collect the ions expelled from the MOT. The 85Rb was trapped with a 780 nm diode laser while the 40Ar* was slowed and trapped with a 811 nm Ti:sapphire laser, which was specifically modified to be locked to within 1 MHz of the atomic transition with a linewidth of ∼1 MHz. The metastable state 40Ar* was produced with a rf driven resonating cavity discharge which produced an atomic beam with an angular flux density of 4 × 1014 atoms s−1 sr−1.
It is generally assumed that for ionization processes, which occur in slow atomic collisions, the coupling of the colliding system to the quantum radiation field is irrelevant. Here we show, however, that -- contrary to expectations -- such a coupling can strongly influence ionization of a beam of atomic species A slowly traversing a gas of atomic species B excited by a weak laser field. Moreover, this coupling becomes even more important when the collision velocity increases, getting comparable or exceeding the typical electron orbiting velocities in A and B. Our results imply furthermore that the Breit interaction can, in fact, dominate over the Coulomb interaction at very low energies.