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IMPERIAL COLLEGE PRESS eBooks

Correlated Quantum Chains with a Finite Concentration of Impurities

Published May 1, 2005• 0 citations
Publisher
DOI
10.1142/9781860946868_0008

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Effects of nonmagnetic impurity doping on an AF spin-1/2 Heisenberg ladder system are studied by the QMC method. A single nonmagnetic impurity induces a localized spin-1/2 moment accompanied by "static" and enhanced AF correlations around it. Small and finite concentration of impurities induces a remarkable change of magnetic and thermodynamic properties with gapless excitations. It also shows rather sharp but continuous crossover around the concentration of about 4%. Above the crossover concentration, all the spins are strongly coupled participating in the enhanced and rather uniform power-law decay of the antiferromagnetic correlation. Below the crossover, each impurity forms an antiferromagnetic cluster only weakly coupled each other. For random distribution of impurities, large Curie-like susceptibility accompanied with small residual entropy is obtained at low temperatures in agreement with recent experimental observation in Zn-doped SrCu2O3SrCu_{2}O_{3}SrCu2​O3​. Temperature dependence of AF susceptibility shows power-law-like but weaker divergence than the single chain AFH in the temperature range studied.