A cold atomic cloud is a versatile object, because it offers many handles to control and tune its properties. This facilitates studies of its behavior in various circumstances, such as sample temperature, size and density, composition, dimensionality and coherence time. The range of possible experiments is constrained by the specifications of the atomic species used. In this thesis presents the work done in the experiment for laser cooling of strontium atoms, focusing on its stability, which should provide cold and ultracold samples for the study of collective effects in light scattering. From the initial apparatus, innumerous changes were performed. The vacuum system got improved and now reached lower ultra high vacuum due to the pre-baking done to its parts and adding a titanium-sublimation stage. The quadrupole trap were improved by the design and construction of a new pair of coils. The stability of the blue, green and red laser systems and the loss prevention of laser light were improved, giving rise to a robust apparatus. Another important point is the development of homemade devices to reduce the costs and to be used as a monitor of different parts of an cold atoms experiment. From this homemade devices, we could demonstrate a dramatic linewidth narrowing by injection lock of an low cost 461 nm diode laser and its application to our strontium experiment. In the end, this improved experimental apparatus made possible the study of a new scattering effect, the mirror assisted coherent back-scattering (mCBS).
A cold atomic cloud is a versatile object, because it offers many handles to control and tune its properties. This facilitates studies of its behavior in various circumstances, such as sample temperature, size and density, composition, dimensionality and coherence time. The range of possible experiments is constrained by the specifications of the atomic species used. In this thesis presents the work done in the experiment for laser cooling of strontium atoms, focusing on its stability, which should provide cold and ultracold samples for the study of collective effects in light scattering. From the initial apparatus, innumerous changes were performed. The vacuum system got improved and now reached lower ultra high vacuum due to the pre-baking done to its parts and adding a titanium-sublimation stage. The quadrupole trap were improved by the design and construction of a new pair of coils. The stability of the blue, green and red laser systems and the loss prevention of laser light were improved, giving rise to a robust apparatus. Another important point is the development of homemade devices to reduce the costs and to be used as a monitor of different parts of an cold atoms experiment. From this homemade devices, we could demonstrate a dramatic linewidth narrowing by injection lock of an low cost 461 nm diode laser and its application to our strontium experiment. In the end, this improved experimental apparatus made possible the study of a new scattering effect, the mirror assisted coherent back-scattering (mCBS).
A cold atomic cloud is a versatile object, because it offers many handles to control and tune its properties. This facilitates studies of its behavior in various circumstances, such as sample temperature, size and density, composition, dimensionality and coherence time. The range of possible experiments is constrained by the specifications of the atomic species used. In this thesis presents the work done in the experiment for laser cooling of strontium atoms, focusing on its stability, which should provide cold and ultracold samples for the study of collective effects in light scattering. From the initial apparatus, innumerous changes were performed. The vacuum system got improved and now reached lower ultra high vacuum due to the pre-baking done to its parts and adding a titanium-sublimation stage. The quadrupole trap were improved by the design and construction of a new pair of coils. The stability of the blue, green and red laser systems and the loss prevention of laser light were improved, giving rise to a robust apparatus. Another important point is the development of homemade devices to reduce the costs and to be used as a monitor of different parts of an cold atoms experiment. From this homemade devices, we could demonstrate a dramatic linewidth narrowing by injection lock of an low cost 461 nm diode laser and its application to our strontium experiment. In the end, this improved experimental apparatus made possible the study of a new scattering effect, the mirror assisted coherent back-scattering (mCBS).
The diode laser system for laser cooling on the 1S 0 → 3P1 intercombination line of strontium discussed in this thesis allows us to cool and trap an atomic strontium sample to 15 muK. Samples in this temperature range are useful for the development of the next generation of atomic frequency standards, cold collision studies, and as a step towards quantum degeneracy. This laser system consists of a Littrow configuration external-cavity diode laser, which is frequency locked to a high finesse cavity. The cavity is subsequently locked to an absorption feature to produce a few mW of tunable, stabilized, single mode power at the target wavelength. We present the design and characterization of this system, including a linewidth measurement of 70 kHz, as well as preliminary results from cooling and trapping.
Atomic Caesium clocks have made an astonishing development in the past few decades, with them gaining an order of magnitude in precision every decade. A new generation of atomic optical clocks is now emerging, which is moving to the forefront of timekeeping. By going from microwave to optical frequencies these clocks are now reaching fractional uncertainty levels in the 10\\(^-\\)\\(^1\\)\\(^8\\), opening a whole new range of exciting applications. This thesis presents the design and implementation of an experiment for laser cooling of strontium atoms, focusing on the mobility of the setup, opening a range of new applications as a mobile clock. The experimental apparatus applies a range of new techniques for strontium, such as the use of a two dimensional magneto-optical trap for pre cooling atoms, allowing for a compact and transportable system. A mobile laser system for laser cooling strontium atoms was realized. This includes a frequency doubling system for the main cooling transition. The constructed monolithic frequency doubling cavity has generated 300 mW of blue light and proven to be a stable setup suitable for a mobile system. The 3D-MOT was able to capture 4 * 10\\(^5\\) atoms with a long lifetime of 5.5 s, with further improvements for a significant increase in atom number currently being implemented.
This thesis describes the first steps to fulfill the main objective of our project: the development of a gravimetry system based on the continuous monitoring of Bloch oscillations performed by ultra-cold strontium atoms.The realization of this project comprises three main stages: the first stage consists in obtaining a magneto-optical trap in the broad transition of 461 nm of strontium, the second stage is the transfer to a magneto-optical trap in the narrow intercombination line of 689 nm, and finally the third stage is the monitoring of Bloch oscillations of the cloud of atoms in a ring cavity.This work details the first stage of the project, the creation of an experimental apparatus which produces ultra-cold strontium atoms in the transition of 461 nm, as well as the characterization of the cloud of atoms, temperature, size, number of atoms, etc.For this project, a new experimental apparatus has been designed and realized.It involves an ultra-high vacuum system, magnetic field sources, laser systems and optical instruments which are required for cooling, trapping and repumping strontium atoms.A novel feature is the implementation of a transversely loaded two-dimensional magneto-optical trap, which serves as a source of a cold strontium atomic beam.A loading rate of the atomic beam into a nearby three-dimensional magneto-optical trap exceeding 10 5 s -1 for the 88 Sr isotope at a moderate dispenser temperature of 600 • C are reported.The temperature of the cloud is about 4 mK and its size 0.3 mm, these characteristics suggest that the state of the atomic trap is in optimal conditions to make the transfer to the optical magneto trap in the intercombination line and thus continue with the second stage of the project.
Ultracold polar molecules have emerged as promising platforms for quantum simulation, quantum information science, precision measurements of fundamental symmetry violations, and quantum chemistry. Over the past decade, rapid progress in direct laser cooling of molecules has enabled new capabilities such as magneto-optical traps (MOTs), sub-Doppler cooling, and optical dipole traps (ODTs), expanding the quantum toolbox with ultracold molecules of complex internal structures and strong dipolar interactions. This thesis presents the design, construction, and operation of an experiment on ultracold strontium monofluoride (88Sr19F) molecules, demonstrating state-of-the-art techniques for molecular laser cooling and trapping. The apparatus integrates a broad range of technical sub-systems, including cryogenics, ultra-high vacuum, optics, electronics, and automated laboratory control software. SrF molecules produced in a slowed cryogenic buffer gas beam are captured into a dual-frequency MOT. Subsequent Λ-enhanced gray molasses cooling reduces the molecule temperature to as low as 5 μK. A novel blue-detuned MOT is also implemented to further compress the molecular cloud, increasing the density by a factor of ∼ 400. At this high density, SrF molecules are efficiently loaded into an ODT, a tight, conservative trap with long lifetimes. Population transfer between different rotational levels is achieved via optical pumping and coherent microwave control, yielding ∼ 0.8 ms coherence time in Rabi oscillation and ∼ 90 % transfer efficiency. This thesis also describes the development of an ultracold rubidium (87Rb) atom experiment, in which a loading rate of ∼ 10^10 atoms/s into a radio-frequency (RF) MOT is demonstrated. A modular two-dimensional MOT serves as the Rb source and can be seamlessly integrated into the SrF apparatus, opening the possibility for future studies of co-trapping and sympathetic cooling of SrF molecules with atoms. The results presented in this thesis establish an experimental foundation for exploring new frontiers in ultracold molecular physics.
We study the coherent transmission of light through cold strontium atomic clouds, using the narrow intercombination line. In the first part of the thesis, the cooperative emission in the coherent transmission is studied experimentally. By applying fast changes to the incident probe field, flashes of light are observed in the forward direction. The peak intensity of the flashes can be much larger than the incident intensity. These flashes are called superflashes. Due to cooperative effect, the time scale of the flashes are shortened with respect to the single scatterer lifetime. By packing these flashes, we generate a pulse train with short repetition time, where the dynamics can almost be fully governed by cooperative effect. The effect of atomic density on the coherent transmission of light is also studied theoretically and numerically. The effective refractive index of the cloud is calculated up to the second order in atomic density. It is eventually validated with a numerical simulation of the coherent light transmission. The second part of the thesis focuses on the effect of magnetic field on the coherent transmission of light. The strontium intercombination line has a sensitivity in the milligauss regime, which is the typical value of stray magnetic field in the lab. An active magnetic field control system is implemented to cancel the low frequency and AC 50~Hz stray magnetic field. Using this control system, we study the nonlinear magneto-optical rotation (NMOR) effect due to a high intensity light field transmitting through a dilute and thin cloud of strontium atom. Interestingly, at sufficiently high cloud temperature, the NMOR effect can have a higher sensitivity to the magnetic field, compared to its linear counterpart at the same cloud temperature.