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Theory of spin-polarized solutions

E. Roland Dobbs

Published May 10, 2001• 0 citations
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Abstract

Abstract Very dilute solutions of 3He in superfluid 4He behave as an almost ideal Fermi gas at millikelvin temperatures, which can be strongly polarized in high magnetic fields. This has enabled studies of their equilibrium, transport, and dynamical spin properties to be made over a wide range of temperatures, concentrations, and polarizations covering systems that are highly degenerate to those that are non-degenerate. This chapter discusses polarized Fermi gas, model theories, equilibrium theories, transport properties, and spin dynamics.

DOI
10.1093/acprof:oso/9780198506409.003.0014

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•Jan 1, 1983•0 citations
Abstract Very dilute solutions of 3He in superfluid 4He behave as an almost ideal Fermi gas at millikelvin temperatures, which can be strongly polarized in high magnetic fields. This has enabled studies of their equilibrium, transport, and dynamical spin properties to be made over a wide range of temperatures, concentrations, and polarizations covering systems that are highly degenerate to those that are non-degenerate. This chapter discusses polarized Fermi gas, model theories, equilibrium theories, transport properties, and spin dynamics.
We carried out experiments on a spin polarized 3He- 4He mixture with 3He concentration x 3 = 6.26 × 10−4, and on pure 3He liquid. Spin polarization affects the transport properties of these Fermi systems. The effect on momentum transport was studied by using a vibrating-wire viscometer to measure viscosity of the 3He-4He mixture over the temperature range 6.09 mK–100 mK in 7.96 T and 1.00 T magnetic fields. A large viscosity increase was observed upon application of the 7.96 T magnetic field for temperature T < TF(TF = 19.5 mK is the Fermi temperature). The observed viscosity is in very good agreement with theoretical calculations for a dilute Fermi gas by Jeon and Mullin [1988, 1989] and Mullin and Jeon [1992]. The polarization effect on spin transport was investigated by measuring the transverse diffusion coefficient D ⊥ in pure 3He liquid at saturated vapor pressure and at 15.85 bar over the temperature range 4.5 mK–159 mK in a 7.96 T magnetic field. We used a pulsed NMR spin echo technique in a field gradient of 16.0 G/cm to do the measurements and fits to the Leggett equations [1970] to obtain D⊥. For T < 20 mK, we found D⊥ is less than measured in earlier experiments at lower magnetic fields. D⊥ does not increase with decreasing temperature as 1/T2, but appears to approach a constant as T → 0 while it is expected that the longitudinal spin diffusion coefficient D∥ ∝ 1/ T2. This is called spin diffusion anisotropy and it was observed for the first time in our 3He liquid experiments. The anisotropy temperature we determined for 3He liquid was Ta = 16.4 ± 2.2 mK at saturated vapor pressure and in a 7.96 T magnetic field. The transverse spin diffusion in 3 He results agree qualitatively with theories proposed by Meyerovich and Musaeflan [1992, 1994]. They also agree qualitatively with theories proposed by Golosov and Ruckenstein [1995, 1998] by extrapolation of the dilute theory to a strongly interacting system.
A complete quantum phase shift calculation of several transport coefficients in spin polarized quantum gases (3He, H↑ and D↑) has been carried out for temperatures ranging from 0.04 K to 10 K and nuclear polarizations M varying from 0 to 1. After a detailed analysis of the dynamical features of the collision, the various direct and exchange « cross sections » necessary to describe the collision between two spin-polarized atoms are studied Emphasis is then placed on some particle-indistinguishability consequences that could be seen in 3He or H↑ systems, such as the strong M dependence of the heat capacity, a mode coupling between heat capacity and longitudinal spin diffusion and the oscillatory character of the evolution of the transverse components of M.
The last five years have seen a burst of activity leading to the current view that 3He atoms dissolved in superfluid liquid 4He show remarkable resemblance to a weakly-interacting Fermi gas. This is because the solvent 4He, having vanishingly small entropy, specific heat, viscosity and magnetic susceptibility, behaves almost as if it were a massive vacuum, in which 3He atoms float. So at last a real Fermi ‘gas’ is available and can readily be cooled to temperatures well below its Fermi degeneracy temperature. This model of solute 3He, with its weaknesses and strengths, is the basis of this article.
Experiments have been performed at high B/T to try to establish the existence and value of an anisotropy temperature (Ta) for pure 3He, and for 6.2% and 0.7% 3He-4He mixtures. The anisotropy of diffusion in dilute Fermi gases as the temperature T goes to zero has been predicted, though experimental evidence for such anisotropy has not been universally accepted.\n\nFinite size effects have required careful analysis of the theory of the cell for the 6.2% mixture. This alters the result as determined by the usual Leggett-Rice formula. Further investigation, beyond the scope of this thesis, is currently underway for the case of pure 3He.\n\nThe possibility of using a quartz tuning fork as a viscometer has also been investigated. It is shown that tuning forks can be used field-inpendently above 3 mK in saturated 3He-4He mixtures, and to detect the superfluid A and B-phase transitions in pure 3He. It is strongly suggested from the data that the tuning fork has great potential as a high-field viscometer; however further experiments are required to fully appreciate its useful range, in both normal and superfluids.
Spin polarized hydrogen and helium are being studied extensively because they are expected to exhibit quantum effects on a macroscopic scale. Here, low density properties of spin polarized hydrogen gas in two and three dimensions are studied using a quantum virial expansion. These properties include heat capacities, chemical potentials, and estimates of critical temperatures and densities for Bose-Einstein condensation in three dimensions and for a possible superfluid transition in two dimensions. The classical virial expansion and the validity of effective-range theory is also discussed. The heat capacity of adsorbed helium films of 3He, 4He and spin polarized 3He is also studied. Virial calculations with a structureless substrate approximation but with substrate mediated corrections to the Lennard-Jones potential are performed as a function of applied magnetic field and magnetization. Effects of substrate potential and geometry on the thermodynamics, low density submonolayer helium films physisorbed on rare gas plated graphite substrates are investigated using a tight-binding formalism and a lattice version of potential scattering theory. A generalization of the formalism to lattices with a basis is made and applied to the honeycomb lattice. The calculations with this theory exhibit systematic trends in the specific heat that are in qualitative agreement with presentlymore » available experimental data.« less