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Springer eBooks

Time Dependence of Harmonic Generation by a Single Atom

Richard Taïeb, A. Maquet, Philippe Antoine, B. Piraux

Published Jan 1, 1996• 0 citations
Publisher
DOI
10.1007/978-94-009-0261-9_42

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We study harmonic generation by a single atom exposed to two short perpendicularly polarized laser pulses. The two perpendicular electric fields oscillate at two different frequencies ${\ensuremath{\omega}}_{1}$ and ${\ensuremath{\omega}}_{2}$. Hence, the resultant field has a polarization which depends on time. Since harmonics are emitted when the resultant oscillating field is linearly polarized, it is expected that a short pulse of harmonics may be emitted if the external field is linearly polarized during a short period of time. We show that, indeed, the atom may emit an ultrashort pulse of a given harmonic. This result has been obtained by time-frequency analyzing the acceleration of the induced dipole moment with a filter whose frequency bandwidth is smaller than twice the frequency of the external field. Our calculation of the dipole acceleration is based on the numerical solution of the time-dependent Schr\"odinger equation. We then address the question of how far it is possible to reduce the duration of the emitted pulse of one given harmonic by adjusting both ${\ensuremath{\omega}}_{1}$ and ${\ensuremath{\omega}}_{2}$ and keeping the amplitude of this pulse significant. In order to answer to this question, we used the quantum version of the two-step model [M. Lewenstein et al., Phys. Rev. A 49, 2117 (1994)].

Physical Review A•Sep 1, 1996•39 citations
We propose a theoretical procedure for calculating harmonics yield from atoms based on the solution of a three-dimensional time-dependent Schr\"odinger equation. The atomic system is described by means of the Hartree-Fock potential, including the exchange interaction. We present results for the harmonics generation in lithium and rubidium in situation when ellipticity of the driving laser changes with time. These results show that harmonics are formed primarily at the intervals of time when the driving laser field has nearly zero ellipticity. This can be used for generation of short (hundreds of attoseconds) bursts of radiation.
We investigate high harmonic generation (HHG) of an atom in the presence of squeezed vacuum of a single harmonic mode. Based on a fully quantum time-dependent Schrödinger equation, we derive an analytical formula for the harmonic amplitude. Our simulations of the HHG spectrum with this formula show that the harmonic amplitude of the corresponding squeezed mode can undergo significant changes with different parameters of the squeezed vacuum. Using the time-frequency analysis method, the physics underlying the effects of the vacuum quantum fluctuation (VQF) on the harmonic generation is revealed, which is found to be consistent with the explanation of Fermi's golden rule. Our work establishes a profound connection between harmonic generation and VQF, and may provide an unconventional approach to manipulating harmonic emission. Published by the American Physical Society 2024
We study harmonic generation by a single atom exposed to two short perpendicularly polarized laser pulses. The two perpendicular electric fields oscillate at two different frequencies ${\ensuremath{\omega}}_{1}$ and ${\ensuremath{\omega}}_{2}$. Hence, the resultant field has a polarization which depends on time. Since harmonics are emitted when the resultant oscillating field is linearly polarized, it is expected that a short pulse of harmonics may be emitted if the external field is linearly polarized during a short period of time. We show that, indeed, the atom may emit an ultrashort pulse of a given harmonic. This result has been obtained by time-frequency analyzing the acceleration of the induced dipole moment with a filter whose frequency bandwidth is smaller than twice the frequency of the external field. Our calculation of the dipole acceleration is based on the numerical solution of the time-dependent Schr\"odinger equation. We then address the question of how far it is possible to reduce the duration of the emitted pulse of one given harmonic by adjusting both ${\ensuremath{\omega}}_{1}$ and ${\ensuremath{\omega}}_{2}$ and keeping the amplitude of this pulse significant. In order to answer to this question, we used the quantum version of the two-step model [M. Lewenstein et al., Phys. Rev. A 49, 2117 (1994)].