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Quantum Electronics and Laser Science Conference

Polarization-ellipse rotation by induced gyrotropy in sodium vapor

William V. Davis, Alexander L. Gaeta, Robert W. Boyd

Published May 12, 1991• 0 citations
OpenAlex

Abstract

We show that for a broad range of intensities the polarization ellipse of a laser beam can undergo rotation while propagating through an atomic vapor. The ellipse rotation is predicted to occur for the case in which the field is tuned near a J = 1/2 to J-1/2 transition of the atomic vapor and the input intensity is sufficiently strong to saturate the ground-state optical pumping but not the transition itself. Under these conditions, the ellipse rotation is independent of the laser intensity and, hence, is unlike the ellipse rotation predicted and observed by Maker and Terhune1 for a tensor nonlinear susceptibility.

Related papers

Polarization-ellipse rotation by induced gyrotropy in atomic vapors

William V. Davis, Alexander L. Gaeta, Robert W. Boyd

We study theoretically and experimentally a new mechanism for the rotation of the polarization ellipse of a single laser beam propagating through an atomic vapor with a frequency tuned near an atomic resonance. The results of a theoretical treatment for the case of a J = (1/2) to J = (1/2) atomic transition show that a rotation of the polarization ellipse of the laser beam will occur as a result of ground-state optical pumping and that the angle of rotation is independent of the laser intensity over a broad range of laser intensities. The predictions of this theoretical model are tested experimentally through the use of potassium vapor and are found to agree with the experimental data.

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Polarization rotation effects in atomic sodium vapor

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Polarization rotation effects in atomic sodium vapor are studied both experimentally and theoretically. Two pulsed dye laser beams propagate collinearly through a cell containing sodium vapor. The direction of polarization of a linearly polarized dye laser beam of frequency ${\ensuremath{\omega}}_{1}$ is found to be rotated by a circularly polarized beam of frequency ${\ensuremath{\omega}}_{2}$. This rotation is due to the difference in refractive index at ${\ensuremath{\omega}}_{1}$ for right and left circularly polarized light which is produced by the circularly polarized beam. When ${\ensuremath{\omega}}_{1}+{\ensuremath{\omega}}_{2}$ is tuned near the $3S\ensuremath{-}5S$ two-photon transition of atomic sodium, this difference is primarily due to the dispersion associated with the two-photon transition. Other sources of polarization rotation which were identified include (i) real transfers of population to excited atomic levels due to collisionally induced transitions and (ii) optically induced atomic energy-level shifts. The theory includes both the effects of two-photon dispersion and optically induced energy shifts. The application of the two-photon polarization rotation effect as a fast, optically controlled shutter or modulator and as a sensitive detection technique for two-photon spectroscopy are briefly discussed.

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Transverse ‘‘bouncing’’ of polarized laser beams in sodium vapor

R. Holzner, Patrik Eschle, A. W. McCord +1 more

Two intersecting laser beams of orthogonal circular polarization near resonant to the homogeneously broadened D1 transition of Na vapor were observed to deflect each other upon contact. The experimental results are in good agreement with calculations based on a model which includes diffraction and a local nonlinear atomic susceptibility wihch fully takes into account saturation and optical pumping effects. The contact deflection (or ``bouncing'') was also observed when both beams were tuned to the atomic resonance frequency.

Physical Review Letters•Oct 12, 1992•21 citations

Optical pumping-induced spatio-temporal modifications to propagation, polarization and intensity of laser beams in sodium vapour

R. Holzner, S. Dangel

Circularly polarized laser beams propagating through sodium vapour and tuned to the buffer-gas-broadened atomic transition can optically pump sodium atoms into a non-absorbing ground state. This causes an intensity-dependent refractive index gradient along as well as transverse to the laser beam propagation direction, giving rise to a number of nonlinear spatio-temporal intensity and polarization pattern creating processes. In the case of a single circularly polarized laser beam we have observed self-focusing and defocusing, the transformation of the incident Gaussian beam intensity profiles into ring profiles, a large shift of about 5 GHz of the maximum of the absorption profile when suitable magnetic fields are applied and the deflection of a beam by the inhomogeneous transverse magnetic field of a current-carrying wire. When two beams of opposite circular polarization are superimposed, astonishing effects such as the mutual deflection of both beams (beam bouncing), the mutual extinction of both beams (beam switching), the separation of initially overlapping beams (beam splitting) and the mutual attraction of both beams (beam attraction) can be observed. While most of the effects can be well described for the stationary state by a to atomic transition model, the correct description of the dynamics requires the consideration of all hyperfine states.

Quantum and Semiclassical Optics Journal of the European Optical Society Part B•Feb 1, 1998•5 citations

Collision-aided Faraday effect in sodium vapor

M. Pinard, Philippe Verkerk, E. Giacobino +1 more

We have observed a collisionally induced rotation of the polarization of a linearly polarized probe beam interacting with a nonresonant circularly polarized pump beam in sodium vapor. We interpret this Faraday effect of a new kind both by a nonlinear-susceptibility calculation and by an optical-pumping calculation, and we show the close connection between the two approaches.

Physical Review A•Apr 1, 1987•6 citations
We show that for a broad range of intensities the polarization ellipse of a laser beam can undergo rotation while propagating through an atomic vapor. The ellipse rotation is predicted to occur for the case in which the field is tuned near a J = 1/2 to J-1/2 transition of the atomic vapor and the input intensity is sufficiently strong to saturate the ground-state optical pumping but not the transition itself. Under these conditions, the ellipse rotation is independent of the laser intensity and, hence, is unlike the ellipse rotation predicted and observed by Maker and Terhune1 for a tensor nonlinear susceptibility.
We study theoretically and experimentally a new mechanism for the rotation of the polarization ellipse of a single laser beam propagating through an atomic vapor with a frequency tuned near an atomic resonance. The results of a theoretical treatment for the case of a J = (1/2) to J = (1/2) atomic transition show that a rotation of the polarization ellipse of the laser beam will occur as a result of ground-state optical pumping and that the angle of rotation is independent of the laser intensity over a broad range of laser intensities. The predictions of this theoretical model are tested experimentally through the use of potassium vapor and are found to agree with the experimental data.
Polarization rotation effects in atomic sodium vapor are studied both experimentally and theoretically. Two pulsed dye laser beams propagate collinearly through a cell containing sodium vapor. The direction of polarization of a linearly polarized dye laser beam of frequency ${\ensuremath{\omega}}_{1}$ is found to be rotated by a circularly polarized beam of frequency ${\ensuremath{\omega}}_{2}$. This rotation is due to the difference in refractive index at ${\ensuremath{\omega}}_{1}$ for right and left circularly polarized light which is produced by the circularly polarized beam. When ${\ensuremath{\omega}}_{1}+{\ensuremath{\omega}}_{2}$ is tuned near the $3S\ensuremath{-}5S$ two-photon transition of atomic sodium, this difference is primarily due to the dispersion associated with the two-photon transition. Other sources of polarization rotation which were identified include (i) real transfers of population to excited atomic levels due to collisionally induced transitions and (ii) optically induced atomic energy-level shifts. The theory includes both the effects of two-photon dispersion and optically induced energy shifts. The application of the two-photon polarization rotation effect as a fast, optically controlled shutter or modulator and as a sensitive detection technique for two-photon spectroscopy are briefly discussed.
Circularly polarized laser beams propagating through sodium vapor and tuned to the buffer gas broadened atomic D1 transition can optically pump sodium atoms into a nonabsorbing groundstate. The corresponding groundstate populations depend on the intensity distribution, the polarization and the magnetic fields. They lead to refractive index gradients along as well as transverse to the laser beam propagation direction and therefore modify the light path giving rise to a number of nonlinear spatiotemporal intensity and polarization pattern creating processes.
Two intersecting laser beams of orthogonal circular polarization near resonant to the homogeneously broadened D1 transition of Na vapor were observed to deflect each other upon contact. The experimental results are in good agreement with calculations based on a model which includes diffraction and a local nonlinear atomic susceptibility wihch fully takes into account saturation and optical pumping effects. The contact deflection (or ``bouncing'') was also observed when both beams were tuned to the atomic resonance frequency.
Circularly polarized laser beams propagating through sodium vapour and tuned to the buffer-gas-broadened atomic transition can optically pump sodium atoms into a non-absorbing ground state. This causes an intensity-dependent refractive index gradient along as well as transverse to the laser beam propagation direction, giving rise to a number of nonlinear spatio-temporal intensity and polarization pattern creating processes. In the case of a single circularly polarized laser beam we have observed self-focusing and defocusing, the transformation of the incident Gaussian beam intensity profiles into ring profiles, a large shift of about 5 GHz of the maximum of the absorption profile when suitable magnetic fields are applied and the deflection of a beam by the inhomogeneous transverse magnetic field of a current-carrying wire. When two beams of opposite circular polarization are superimposed, astonishing effects such as the mutual deflection of both beams (beam bouncing), the mutual extinction of both beams (beam switching), the separation of initially overlapping beams (beam splitting) and the mutual attraction of both beams (beam attraction) can be observed. While most of the effects can be well described for the stationary state by a to atomic transition model, the correct description of the dynamics requires the consideration of all hyperfine states.