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Springer series in optical sciences/SPringer series in optical sciences

High Precision Measurements of Atomic Level Splittings by Means of Periodic Pumping with Picosecond Light Pulses

H. Harde, H. Burggraf

Published Jan 1, 1983• 1 citation
Publisher
DOI
10.1007/978-3-540-38814-2_34

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quant-pharXiv:2601.15565•Jan 23, 2026•0 citations
We have demonstrated the feasibility of Doppler-free two-photon spectroscopy with a train of picosecond standing-wave light pulses from a synchronously pumped mode-locked cw dye laser. The actively controlled mode spectrum provides a means for accurate measurements of large frequency intervals. From a multipulse spectrum of the sodium $3s\ensuremath{-}4d$ transition we have determined a new value of the 4d4d4d fine-structure splitting, 1028\ifmmode\pm\else\textpm\fi{}0.4 MHz.
Squeezed states of light enable enhanced measurement precision by reducing noise below the standard quantum limit. A key application of squeezed light is nonlinear microscopy, where state-of-the-art performance is limited by photodamage and quantum-limited noise. Such microscopes require bright, pulsed light for optimal operation, yet generating and detecting bright pulsed squeezing at high levels remains challenging. In this work, we present an efficient technique to generate high levels of bright picosecond pulsed squeezed light using a χ2χ^2χ2 optical parametric amplification process in a waveguide. We measure −3.2 dB-3.2~\mathrm{dB}−3.2 dB of bright squeezing with optical power compatible with nonlinear microscopy, as well as −3.6 dB-3.6~\mathrm{dB}−3.6 dB of vacuum squeezing. Corrected for losses, these squeezing levels correspond to −15.4−8.7+2.7 dB-15.4^{+2.7}_{-8.7}~\mathrm{dB}−15.4−8.7+2.7​ dB of squeezing generated in the waveguide. The measured level of bright amplitude pulsed squeezing is to our knowledge the highest reported to date, and will contribute to the broader adoption of quantum-enhanced nonlinear microscopy in biological studies.