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Elsevier eBooks

Spontaneous Emission and Its Effects

L. F. Mollenauer, J. P. Gordon

Published Jan 1, 2006• 0 citations
Publisher
DOI
10.1016/b978-012504190-4/50004-9

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We present results of experiments on the spontaneous emission rate of a europium complex in dense supercritical CO2{\mathrm{CO}}_{2}CO2​. The refractive index of the supercritical gas is varied from 1.00 to 1.27 by increasing the pressure up to a 1000 bars. Accordingly, the spontaneous emission rate changes. Local-field effects on spontaneous emission are clearly observed in these experiments. The empty-cavity model for the spontaneous emission rate inside dielectrics is confirmed.
The authors achieved their initial goal in the study of basic radioactive processes using Rydberg atoms - the observation of inhibited spontaneous emission. An experiment was carried out demonstrating that spontaneous emission can be effectively turned off. The underlying principle is that spontaneous emission results from the radioactive coupling between matter and a continuum of vacuum states. However, the assumptions underlying the conventional calculation of the density of modes in free space are not always valid. In particular, cavities can dramatically effect spontaneous emission. Such effects are difficult to observe in the optical regime because of the problem of making good fundamental mode cavities at short wavelengths. Excellent cavities can be made at microwave wavelengths, but spontaneous emission is enhanced by a factor of n4 where n is the principal quantum number, allowing such effects to be studied.
We numerically solve an effective single-atom Hartree-Fock master equation in order to investigate the effects of spontaneous emission on atomic Thirring solitons and atomic gap solitons. We show that spontaneous emission detrimentally effects the existence of Thirring solitons, as expected from the fact that they only occur on resonance. In contrast, gap solitons, which can also exist off resonance, survive in the presence of spontaneous emission in weakly allowed transitions, albeit at high atomic densities. This result is illustrated in the case of the [2 1^{1}1S0{\mathit{S}}_{0}S0​\ensuremath{\leftrightarrows}2 3^{3}3P1{\mathit{P}}_{1}P1​]- intercombination line of magnesium.