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Transport theory of nuclear collective motion

Helmut Hofmann

Published Apr 17, 2008• 0 citations
Publisher

Abstract

Abstract This chapter develops a quantal transport theory for non-linear nuclear collective motion, the coordinates of which are functionals of the nucleonic degrees of freedom, the latter being interpreted as ‘heat bath’. Introduced on the mean field level the collective variables must be quantized. This is accomplished through the Bohm-Pines method, which leads to an extended Hamiltonian for the entire system. On this basis, transport equations are deduced through a non-perturbative Nakajima-Zwanzig procedure. This scheme is carried out within a locally harmonic approximation, in which all collective forces are linearized locally and in which Gaussian forms are used for propagators of Wigner functions. The diffusion coefficients are determined by the quantal fluctuation dissipation theorem, which for unstable modes requires appropriate analytic continuations. This scheme breaks down below a critical value of temperature identical to that found in the Caldeira-Leggett model for real time propagation. Fundamental properties of these propagators are studied.

DOI
10.1093/acprof:oso/9780198504016.003.0007

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Abstract This chapter develops a quantal transport theory for non-linear nuclear collective motion, the coordinates of which are functionals of the nucleonic degrees of freedom, the latter being interpreted as ‘heat bath’. Introduced on the mean field level the collective variables must be quantized. This is accomplished through the Bohm-Pines method, which leads to an extended Hamiltonian for the entire system. On this basis, transport equations are deduced through a non-perturbative Nakajima-Zwanzig procedure. This scheme is carried out within a locally harmonic approximation, in which all collective forces are linearized locally and in which Gaussian forms are used for propagators of Wigner functions. The diffusion coefficients are determined by the quantal fluctuation dissipation theorem, which for unstable modes requires appropriate analytic continuations. This scheme breaks down below a critical value of temperature identical to that found in the Caldeira-Leggett model for real time propagation. Fundamental properties of these propagators are studied.
We study the emergence of collective dynamics in the integrable Hamiltonian system of two finite ensembles of coupled harmonic oscillators. After identification of a collective degree of freedom, the Hamiltonian is mapped onto a model of Caldeira-Leggett type, where the collective coordinate is coupled to an internal bath of phonons. In contrast to the usual Caldeira-Leggett model, the bath in the present case is part of the system. We derive an equation of motion for the collective coordinate which takes the form of a damped harmonic oscillator. We show that the distribution of quantum transition strengths induced by the collective mode is determined by its classical dynamics. This allows us to derive the spreading for the collective coordinate from first principles. After that we study the interplay between collective and incoherent single--particle motion in a model of two chains of particles whose interaction comprises a non--integrable part. In the perturbative regime, but for a general form of the interaction, we calculate the Fourier transform of the time correlation for the collective coordinate. We obtain the remarkable result that it always has a unique semi-classical interpretation. We show this by a proper renormalization procedure which also allows us to map the non-integrable system to the integrable model of Caldeira--Leggett--type considered previously in which the bath is part of the system.
Quantum diffusion equations featuring explicitly time-dependent transport coefficients are derived from generalized non-Markovian Langevin equations. Generalized fluctuation-dissipation relations and analytic expressions for calculating the friction and diffusion coefficients in nuclear processes are obtained. The asymptotic behavior of the transport coefficients and correlation functions for a damped harmonic oscillator that is linearly coupled in momentum to a heat bath is studied. The coupling to a heat bath in momentum is responsible for the appearance of the diffusion coefficient in coordinate. The problem of regression of correlations in quantum dissipative systems is analyzed.
We address the dynamics of damped collective modes in terms of first and second moments. The modes are introduced in a self-consistent fashion with the help of a suitable application of linear response theory. Quantum effects in the fluctuations are governed by diffusion coefficients D μν . The latter are obtained through a fluctuation dissipation theorem generalized to allow for a treatment of unstable modes. Numerical evaluations of the D μν are presented. We discuss briefly how this picture may be used to describe global motion within a locally harmonic approximation. Relations to other methods are discussed, like "dissipative tunneling", RPA at finite temperature and generalizations of the "Static Path Approximation".
Quantum diffusion equations with transport coefficients explicitly depending on time are derived from the generalized non-Markovian Langevin equations. The asymptotic behavior of the friction and diffusion coefficients is investigated in the case of the FC and RWA couplings between the collective and internal subsystems. An asymptotic expression is obtained for the propagator of the density matrix of the open quantum system with the general quadratic Hamiltonian, linearly coupled (in coordinate and momentum) to internal degrees of freedom. The effect of different sets of transport coefficients on the decoherence and decay rate of the metastable state is investigated using the master equation for the reduced density matrix of open quantum systems. The developed approach is used to study the capture of the projectile nucleus by the target nucleus at energies near the Coulomb barrier. Capture cross sections in asymmetric reactions are well described with allowance for the calculated capture probabilities. Particular cases where dissipation favors penetration through the potential barrier are found. The generalized Kramers formula for the quasi-stationary decay rate of the quantum metastable systems is analytically derived.
We formulate a theory for the transfer of energy from collective degrees of freedom to internal degrees of freedom when the former belong to the adiabatic large-amplitude regime. The framework is that of an extended mean-field theory including dissipation, with the following salient features: (i) The Born-Oppenheimer approximation is extended to finite excitation energy by the introduction of the concept of thermal state, that is pure with respect to collective coordinates and a (square root of a)a)a) density matrix with respect to internal coordinates. (ii) By assuming that these states form an approximate complete set for application of the Kerman-Klein method, the self-consistent theory of large amplitude collective motion is extended to finite excitation energy. (iii) The mean-field limit is taken, and further study is carried out in the basis of natural orbitals that diagonalizes the one-particle density matrix. In the approximation maintained uniformly in this work, the equations of motion for the orbitals are shown to be of Hamiltonian form; to these are conjoined the master equations for the time rate of change of the occupation numbers. The latter are studied in two extreme limits. In the collisionless limit, dissipation still arises from the response of the mean field to the collective motion (one-body friction). At the opposite extreme, collisions are assumed to be so effective as to force the system always to be in a state of local (constrained) equilibrium. (iv) We review a procedure by which the noncollective variables in the Hamiltonian may be eliminated, leading to equations of motion for the collective variables with dissipative terms that in general depend on the history of the system. The limit of instantaneous friction can be justified in an adiabatic approximation. (v) A decoupling procedure is developed for deriving the form of these equations of motion from the mean-field theory, with the ultimate aim of obtaining the macroscopic parameters that appear in the classical equations of motion for the collective variables. This procedure generalizes that developed in extensive previous work on large amplitude collective motion at zero temperature. (vi) Associating the dissipative equations of motion for the collective variables with one of the assumptions concerning the rates of change of the occupation numbers provides a description of the relaxation of a system initially perturbed from a state of dynamic equilibrium.
A classical microscopic theory of mixed states has recently been formulated in order to deal with the theoretical description of nuclear phenomena observed in highly excited states. In this theory, which is here briefly reviewed, the degrees of freedom of real fermions are doubled by fictitious fermions, in the context of the formalism of thermofield dynamics. The requirement of static stability of the thermal state of equilibrium plays, in the theory, a relevant role. The possibility of constraining the dynamics of the fictitious degrees of freedom, in such a way as to eliminate spurious thermal excitations, is discussed. The concept of canonical collective variables for mixed states is analyzed. Boson expansions appropriate to describe collective excitations of hot quantal systems are introduced and their properties investigated. It is shown that thermal boson expansions based on the formalism of thermofield dynamics are free from formal inconsistencies which may be present in boson expansions derived by an ad hoc quantization of conventional thermal mean field theories. The formalism is applied to the Lipkin model, and the correlation energy of a hot system is discussed.