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Cambridge University Press eBooks

Optical forces and laser cooling

P. van der Straten, Harold J. Metcalf

Published Dec 31, 2015• 0 citations
Publisher

Abstract

The usual form of electromagnetic forces is given by but for neutral atoms q = 0. The next order of force is the dipole term, but this also vanishes because neutral atoms have no inherent dipole moment. However, a dipole moment can be induced by a field, and this is most efficient if the field is alternating near the atomic resonance frequency. Since these frequencies are typically in the optical range, dipole moments are efficiently induced by shining nearly resonant light on the atoms. Laser cooling and trapping rely on the interaction between laser light and atoms to exert a controllable force on the atoms, and many sophisticated schemes have been developed using the special properties of the interaction. This chapter begins with the simplest schemes for exerting optical forces on atoms, namely a single-frequency light field interacting with a two-level atom. Although this is the simplest possible scheme, it is pedagogically valuable because it shows many of the features that will be encountered further on. The ultimate temperature using such a scheme is limited, but lower temperatures can be achieved with multilevel atoms. This topic is addressed later in the chapter. Two kinds of optical forces When an atom absorbs nearly resonant light, it makes a transition to the excited state, and its subsequent return to the ground state can be either by spontaneous or by stimulated emission. The nature of the optical force that arises from these two different processes is quite different, and will be described separately [1]. The spontaneous emission case is different from the familiar quantum mechanical calculations using state vectors to describe the state of the system, because spontaneous emission causes the state of the system to evolve from a pure state into a mixed state (see Exercise 6.9). Spontaneous emission is an essential ingredient for the dissipative nature of the optical forces in monochromatic light, and the density matrix is needed to describe it (see Chap. 6). When an atom absorbs light, its energy excites the atom and its angular momentum changes the electron's orbit. Both of these are internal atomic properties. However, the linear momentum of the light, can change only the external, translational motion of the atom.

DOI
10.1017/cbo9781316106242.020

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The usual form of electromagnetic forces is given by but for neutral atoms q = 0. The next order of force is the dipole term, but this also vanishes because neutral atoms have no inherent dipole moment. However, a dipole moment can be induced by a field, and this is most efficient if the field is alternating near the atomic resonance frequency. Since these frequencies are typically in the optical range, dipole moments are efficiently induced by shining nearly resonant light on the atoms. Laser cooling and trapping rely on the interaction between laser light and atoms to exert a controllable force on the atoms, and many sophisticated schemes have been developed using the special properties of the interaction. This chapter begins with the simplest schemes for exerting optical forces on atoms, namely a single-frequency light field interacting with a two-level atom. Although this is the simplest possible scheme, it is pedagogically valuable because it shows many of the features that will be encountered further on. The ultimate temperature using such a scheme is limited, but lower temperatures can be achieved with multilevel atoms. This topic is addressed later in the chapter. Two kinds of optical forces When an atom absorbs nearly resonant light, it makes a transition to the excited state, and its subsequent return to the ground state can be either by spontaneous or by stimulated emission. The nature of the optical force that arises from these two different processes is quite different, and will be described separately [1]. The spontaneous emission case is different from the familiar quantum mechanical calculations using state vectors to describe the state of the system, because spontaneous emission causes the state of the system to evolve from a pure state into a mixed state (see Exercise 6.9). Spontaneous emission is an essential ingredient for the dissipative nature of the optical forces in monochromatic light, and the density matrix is needed to describe it (see Chap. 6). When an atom absorbs light, its energy excites the atom and its angular momentum changes the electron's orbit. Both of these are internal atomic properties. However, the linear momentum of the light, can change only the external, translational motion of the atom.
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Chapter 11 presents the simplest and most intuitive approach to atom-optical interactions: the atom is modelled as a damped harmonic oscillator with spontaneous emission as the damping agent. The semiclassical viewpoint, in which the atom is treated as a quantum object but the fields are classical, is adopted throughout the chapter. Next, the two-level atom is introduced, which sets the stage for establishing light forces at the atomic level: the dipole-gradient force and the radiation pressure force. The Einstein B coefficient is revisited as stimulated dipole emission. Finally, the optical Bloch equations are used to reformulate more generally the appearance of optical forces and to describe the existence of atom Doppler cooling.
The dipole force, which avoids the closed cycle of pumping and spontaneous emission that renders laser cooling unsuitable for molecules, is conservative: without dissipation, particles entering a trap retain the energy to escape. Fortunately, dissipation need not involve spontaneous emission if it instead results from the decoherence or decay of the optical trapping field that is coupled to the particle. To enhance the weak attraction of an atom to its reflection, cavity-mediated cooling recycles light through multiple reflections, amplifying the force and the retardation - a process related to the mechanical amplification in a near confocal cavity [5]. Resonant cavities and structures can increase the retardation, but not the intensity, even when the atoms or particles lie outside them - e.g. when the cavity is the narrow-band coating of a single mirror. Plasmon resonances of a structured metal can enhance both the delay and the optical intensity. Such processes, possible with arrays of micromirrors, resemble speckle field cooling [6], except that spontaneous emission is again replaced by decay of the optical field, and offer a new class of cooling mechanisms in which weak cooling is extended over a broad array, rather than concentrated at the centre of a single external cavity.
Over the past 30 years, optical manipulation of neutral atoms has been primarily performed with a monochromatic laser beam. The simplest tool for the control of atomic motion is the radiative force exerted by a monochromatic laser on a twolevel atom. The radiative force arises from absorption followed by spontaneous emission, and its magnitude is limited by the atom's excited state lifetime. The coherent momentum exchanges between light elds and atoms can be exploited to produce long-range optical forces much greater than the radiative force through the use of absorption-stimulated emission processes. Adiabatic Rapid Passage (ARP) is a long-existing method to invert the population of a two-level nuclear spin system. Its extension to the optical domain necessitates a frequency chirped light pulse to interact with a two-level atom via the dipole interaction. I will first present a numerical study of the properties of optical forces on moving atoms derived from purely stimulated processes produced by multiple ARP sequences. This will be followed by experimental observations of long-range ARP forces much larger than the radiative force in metastable helium. Sequences of properly timed laser pulses may be used for rapid deceleration of neutral atomic (or molecular) beams. | 171 pages
Light emission occurs as a result of interaction between light and matter. Let us assume a two-level atom with levels 1 (ground state) and 2 (excited state). The energies of the ground and excited states are E 1 and E 2 , respectively, and the energy difference is therefore given by the difference ΔE 12 =E 2 −E 1 . When light with photons of energy equal to this difference is absorbed by the atomic or molecular system, an electron will be excited from level 1 to level 2. The energy of the photons is given by ΔE 12 =E 12 =hν 12 (h is Planck's constant and 1→2 is the frequency of light resulting from the level 1→2 transition). This energy is absorbed by an atom or a molecule that has energy levels, separated by ΔE, where these energy levels are the ground and the excited states. This kind of “quantum jump” of an electron between two states occurs in atomic systems between electronic levels; it can be extended to molecular systems, where vibrational and translational energy levels participate in the quantum jump. The interaction between light and matter involves the transition of electrons between different states. This interaction results in the absorption of photons (stimulated absorption) as well as spontaneous and stimulated emission. These processes can be described using Einstein's A and B coefficients, as will be described in the next paragraphs.
It has been known for some time that the interaction of laser light with a free atom can give rise to electromagnetic pressure forces that act on its centre of mass. These forces have been extensively examined both theoretically and experimentally: see, for example Metcalf and van der Straten (5.1) or Adams and Riis (5.2). A simple model of a two-level atom subject to a plane electromagnetic wave may be shown to give rise to two kinds of force acting on the atom centre of mass. These are, a dissipative force arising from the absorption of the light by the atom and its subsequent spontaneous emission in a random direction and a dipole force arising from the non-uniformity of the field distribution which can attract the atom to the regions of intense field. These forces underpin the manipulation of atoms by lasers in a variety of beam configurations. The dissipative force has been exploited in the Doppler cooling of the atomic motion (5.3, 5.4) and the dipole force used for trapping (5.5), while a combination of these effects has led to the realisation of Bose-Einstein condensation (5.6). These forces are, of course, closely related to the ones discussed in Section 4.