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Quantum Electronics and Laser Science Conference

New developments in morphological resonances of dielectric spheres (photonic atoms): room-temperature persistent spectral hole-burning

S. R. Arnold

Published May 10, 1992• 0 citations
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Persistent spectral hole burning with multiplicity was realized at room temperature for Nile blue molecules-doped polymeric dielectric spherical microparticles based on morphology-dependent resonances. Hole parameters depending on burning conditions were studied. Dynamical characteristic behavior of hole formation was measured and analyzed with a model based on rate equations. The effective hole formation rate was obtained by simulation. Photophysical and photochemical mechanisms of the room temperature hole burning for this system was discussed.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Sep 3, 1996•0 citations
Recently, photonic atoms (dielectric microspheres) have enjoyed the attention of the optical spectroscopy community. A variety of linear and nonlinear optical processes have been observed in liquid microdroplets. But solid state photonic devices using these properties are scarce. A first of these applications is the room temperature microparticle hole-burning memory. New applications can be envisioned if microparticle resonances can be coupled to traveling waves in optical fibers. In this paper we demonstrate the excitation of narrow morphology dependent resonances of microparticles placed on an optical fiber. Furthermore we reveal a model for this process which describes the coupling efficiency in terms of the geometrical and material properties of the microparticle-fiber system.
Persistent spectral hole burning with multiplicity was realized at room temperature for Nile blue molecules-doped polymeric dielectric spherical microparticles based on morphology-dependent resonances. Hole parameters depending on burning conditions were studied. Dynamical characteristic behavior of hole formation was measured and analyzed with a model based on rate equations. The effective hole formation rate was obtained by simulation. Photophysical and photochemical mechanisms of the room temperature hole burning for this system was discussed.