Hyperfine characterisation and enhanced optical to spin storage in rare earth ion doped crystals

Marko Lovrić

Published Feb 9, 2012• 1 citation

Abstract

) 3 , trivalent praseodymium in lanthanum tungstatePrYAP Pr 3+ :YAlO 3 , trivalent praseodymium in yttrium alluminum perovskite

DOI: 10.17877/de290r-3279

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Hyperfine characterisation and enhanced optical to spin storage in rare earth ion doped crystals

Marko Lovrić

Published Feb 9, 2012• 1 citation

Publisher

Abstract

) 3 , trivalent praseodymium in lanthanum tungstatePrYAP Pr 3+ :YAlO 3 , trivalent praseodymium in yttrium alluminum perovskite

DOI: 10.17877/de290r-3279

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Spin Hamiltonian characterization and refinement for Pr 3 + :YAlO 3 and Pr 3 + :Y 2 SiO 5

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Rare-earth ions in dielectric crystals play an important role in high-resolution laser spectroscopy and are interesting candidates for storing quantum states of photons. We characterize the praseodymium hyperfine interaction of the ground-state ( ${}^{3}$ H ${}_{4}$ ) and one excited-state ( ${}^{1}$ D ${}_{2}$ ) for two important compounds: praseodymium doped in yttrium aluminum perovskite and praseodymium doped in yttrium orthosilicate. The spin Hamiltonian parameters are determined by numerical analysis of Raman-heterodyne spectra, which were collected for a range of static external magnetic field strengths and orientations. For Pr ${}^{3+}$ :YAlO ${}_{3}$ , we present a full analysis without restrictions for the Zeeman and quadrupole tensors, and our new characterization for Pr ${}^{3+}$ :Y ${}_{2}$ SiO ${}_{5}$ resolves a controversy in the literature.Rare-earth ions in dielectric crystals play an important role in high-resolution laser spectroscopy and are interesting candidates for storing quantum states of photons. We characterize the praseodymium hyperfine interaction of the ground-state (${}^{3}$H${}_{4}$) and one excited-state (${}^{1}$D${}_{2}$) for two important compounds: praseodymium doped in yttrium aluminum perovskite and praseodymium doped in yttrium orthosilicate. The spin Hamiltonian parameters are determined by numerical analysis of Raman-heterodyne spectra, which were collected for a range of static external magnetic field strengths and orientations. For Pr${}^{3+}$:YAlO${}_{3}$, we present a full analysis without restrictions for the Zeeman and quadrupole tensors, and our new characterization for Pr${}^{3+}$:Y${}_{2}$SiO${}_{5}$ resolves a controversy in the literature.

Physical Review BJan 24, 201224 citations

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Jan 1, 20080 citations

{}^{3}

{}_{4}

) and one excited-state (

{}^{1}

{}_{2}

) for two important compounds: praseodymium doped in yttrium aluminum perovskite and praseodymium doped in yttrium orthosilicate. The spin Hamiltonian parameters are determined by numerical analysis of Raman-heterodyne spectra, which were collected for a range of static external magnetic field strengths and orientations. For Pr

{}^{3+}

:YAlO

{}_{3}

, we present a full analysis without restrictions for the Zeeman and quadrupole tensors, and our new characterization for Pr

{}^{3+}

{}_{2}

SiO

{}_{5}

resolves a controversy in the literature.