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Physics World

Laser cooling the atom of atoms

Dieter Meschede

Published Jun 1, 1993• 0 citations
Publisher

Abstract

Experiments with atomic hydrogen are widespread because hydrogen is the simplest and theoretically most accessible atom. This is not only true for isolated atoms, but also for spin-polarised gases of cold hydrogen. In this unique system, in which the total spins of all the hydrogens are parallel, the atoms only interact in one of the large number of possible molecular potentials. This potential (Known as 3 Σ) does not allow bound states, leading to the expectation that spin-polarised hydrogen remains gaseous down to zero kelvin. But the lack of a suitable laser source for cooling hydrogen has prevented experimenters investigating the wealth of new physics expected at these temperatures.

DOI
10.1088/2058-7058/6/6/19

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Experiments with atomic hydrogen are widespread because hydrogen is the simplest and theoretically most accessible atom. This is not only true for isolated atoms, but also for spin-polarised gases of cold hydrogen. In this unique system, in which the total spins of all the hydrogens are parallel, the atoms only interact in one of the large number of possible molecular potentials. This potential (Known as 3 Σ) does not allow bound states, leading to the expectation that spin-polarised hydrogen remains gaseous down to zero kelvin. But the lack of a suitable laser source for cooling hydrogen has prevented experimenters investigating the wealth of new physics expected at these temperatures.
Introduction This chapter describes remarkable new experiments that have been made possible through recent advances in laser cooling of atoms. Cooling of atoms in a gas by laser light is in itself surprising and this technique is important in a range of applications. In particular the experiments described here take atoms that have been laser cooled and then use other methods to reach even lower temperatures, at which wonderful and fascinating quantum effects occur. As well as revealing new phenomena, these experiments explore the deep analogies between the roles played by light waves in lasers and matter waves. These techniques are widely accessible and enable skilled researchers in laboratories all over the world to explore exciting new physics. The key physics and techniques of laser cooling are described in depth in Chapter 6. What is “temperature”? We use the words “cold” and “hot” every day; for example to refer to the temperature of the air outside. But what do “cold” and “hot” mean for the air’s molecules? Broadly speaking, we can say that atoms in a hot gas move faster than those in a cold gas and that cooling, by taking energy out of the gas, slows the atoms down. In this description of the gas as a collection of atoms behaving like billiard balls, or little hard spheres, the lowest possible temperature occurs when the atoms stop moving but, as we shall see, this picture does not give an accurate description at very low energies, for which quantum effects become important. In this chapter we will look at the fascinating properties of atomic gases cooled to temperatures within one millionth of a degree Kelvin from absolute zero. We shall use the term “ultra-cold” to refer to such extremely low temperatures that have only recently been achieved in experiments on atomic gases. The techniques used to cool liquids and solids have a longer history and have made available a different set of possibilities (see Chapter 8). Note that most of this chapter refers to gases in which the individual particles are atoms, but the general statements about temperature scales apply equally well to gases of molecules, e.g. air, whose major constituents, oxygen and nitrogen, exist as diatomic molecules.
Despite the prominent role of laser cooling in modern atomic physics, with applications ranging from quantum sensors to high-precision spectroscopy and ultracold chemistry, laser cooling techniques are still limited to atoms with simple energy level structure and closed transitions that are accessible by currently available continuous wave (cw) laser sources. Two main obstacles prevent the extension of laser cooling techniques to a variety of atomic species and molecules. The first is associated with technical difficulties in creating cw laser light in the vacuum ultraviolet (VUV) spectral range - the absence of those laser sources prevents laser cooling of simple atoms such as hydrogen, deuterium, and antihydrogen. The second obstacle is associated with complex energy level structure of many atoms and almost all molecules - it permits decay of an excited state into a number of lower-lying states that can be widely separated in energy, which makes laser cooling of such species inefficient and experimentally very challenging.
INTRODUCTION A variety of techniques have been developed over the past two decades for influencing the motion of atomic gases using laser light. These techniques, termed collectively 'laser cooling,' produce samples of atoms with temperatures one millionth of a degree above absolute zero, ushering in a new era of atomic physics. The exquisite control offered by these techniques has made possible measurements of fundamental constants, atomic clocks used in the realization of the SI unit of time, new atom-wave interferometers, and the realization of Bose-Einstein condensation. To understand the impact of gravity on such cold atoms, consider that if the atmosphere were an ideal gas cooled to one micro-Kelvin, it would only extend just 5 microns above the Earth's surface.
Of the many applications of lasers, the one with possibly the most dramatic impact on fundamental physics is laser cooling and trapping: the Nobel Prize for physics was awarded for laser cooling in 1997. Laser cooling allows one to obtain samples of atoms essentially at rest, with temperatures in the micro-Kelvin region being routine. At such low temperatures, it becomes easy to trap or move atoms with modest electromagnetic forces and a whole new class of experiments previously confined to the realm of fantasy becomes possible. The high brightness of masers and lasers makes it possible to access a regime of atomic excitation for which Einstein’s rate equations are inadequate. Three-dimensional optical molasses using counter-propagating laser beams along three mutually orthogonal directions was first observed in 1985 by Chu et al. The Sisyphus mechanism works well for atoms that are already cold and has a smaller capture velocity than conventional Doppler cooling.
Abstract The methods of laser cooling of atoms have long been applied to obtain cold and ultracold atomic gases, including degenerate states and the atomic Bose–Einstein condensate in particular. Until recently the application of laser cooling methods to molecules was assumed to be impossible because of the complex structure of molecular levels and the absence of closed cooling cycles for transitions between the electron levels of molecules in the general case. However, it has recently become clear that laser cooling can be performed for a large class of molecules, including not only the simplest diatomic molecules but also polyatomic molecules. We here present the general principles for identifying suitable molecules and discuss current studies on and further developments in the laser cooling of molecules.