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Physical review. B./Physical review. B

Publisher's Note: Umbrella-coplanar transition in the triangular XXZ model with arbitrary spin [Phys. Rev. B93, 224402 (2016)]

Giacomo Marmorini, Daisuke Yamamoto, Ippei Danshita

Published Jun 29, 2016• 1 citation
Publisher
DOI
10.1103/physrevb.93.219905

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Quantum magnetic phases near the magnetic saturation of triangular-lattice antiferromagnets with XXZ anisotropy have been attracting renewed interest since it has been suggested that a nontrivial coplanar phase, called the $\ensuremath{\pi}$-coplanar or $\mathrm{\ensuremath{\Psi}}$ phase, could be stabilized by quantum effects in a certain range of anisotropy parameter $J/{J}_{z}$ besides the well-known 0-coplanar (known also as $V)$ and umbrella phases. Recently, Sellmann et al. [Phys. Rev. B 91, 081104(R) (2015)] claimed that the $\ensuremath{\pi}$-coplanar phase is absent for $S=1/2$ from an exact-diagonalization analysis in the sector of the Hilbert space with only three down-spins (three magnons). We first reconsider and improve this analysis by taking into account several low-lying eigenvalues and the associated eigenstates as a function of $J/{J}_{z}$ and by sensibly increasing the system sizes (up to 1296 spins). A careful identification analysis shows that the lowest eigenstate is a chirally antisymmetric combination of finite-size umbrella states for $J/{J}_{z}\ensuremath{\gtrsim}2.218$ while it corresponds to a coplanar phase for $J/{J}_{z}\ensuremath{\lesssim}2.218$. However, we demonstrate that the distinction between 0-coplanar and $\ensuremath{\pi}$-coplanar phases in the latter region is fundamentally impossible from the symmetry-preserving finite-size calculations with fixed magnon number. Therefore, we also perform a cluster mean-field plus scaling analysis for small spins $S\ensuremath{\le}3/2$. The obtained results, together with the previous large-$S$ analysis, indicate that the $\ensuremath{\pi}$-coplanar phase exists for any $S$ except for the classical limit $(S\ensuremath{\rightarrow}\ensuremath{\infty})$ and the existence range in $J/{J}_{z}$ is largest in the most quantum case of $S=1/2$.

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The quantum triangular XXZ model has recently enjoyed a wealth of new theoretical results, especially in relation to the modeling of the Ba3CoSb2O9{\mathrm{Ba}}_{3}{\mathrm{CoSb}}_{2}{\mathrm{O}}_{9}Ba3​CoSb2​O9​ compound. In particular, it has been understood that in a longitudinal magnetic field the umbrella (cone) phase, classically stable in all the easy-plane region of the ground-state phase diagram, is considerably reduced by the effect of quantum fluctuations. We provide more quantitative information for this phenomenon at arbitrary value of the site spin SSS, by employing the dilute Bose gas expansion, valid in the high-field regime; our results improve the available estimates of the 1/S1/S1/S expansion. We quantify the extent to which a higher spin suppresses the effect of quantum fluctuations. Besides, we show how in three-dimensional layered systems a relatively small antiferromagnetic interlayer coupling has a similar consequence of bringing back the umbrella phase in some part of the phase diagram.
Quantum magnetic phases near the magnetic saturation of triangular-lattice antiferromagnets with XXZ anisotropy have been attracting renewed interest since it has been suggested that a nontrivial coplanar phase, called the $\ensuremath{\pi}$-coplanar or $\mathrm{\ensuremath{\Psi}}$ phase, could be stabilized by quantum effects in a certain range of anisotropy parameter J/JzJ/{J}_{z}J/Jz​ besides the well-known 0-coplanar (known also as V)V)V) and umbrella phases. Recently, Sellmann et al. [Phys. Rev. B 91, 081104(R) (2015)] claimed that the $\ensuremath{\pi}$-coplanar phase is absent for S=1/2S=1/2S=1/2 from an exact-diagonalization analysis in the sector of the Hilbert space with only three down-spins (three magnons). We first reconsider and improve this analysis by taking into account several low-lying eigenvalues and the associated eigenstates as a function of J/JzJ/{J}_{z}J/Jz​ and by sensibly increasing the system sizes (up to 1296 spins). A careful identification analysis shows that the lowest eigenstate is a chirally antisymmetric combination of finite-size umbrella states for $J/{J}_{z}\ensuremath{\gtrsim}2.218$ while it corresponds to a coplanar phase for $J/{J}_{z}\ensuremath{\lesssim}2.218$. However, we demonstrate that the distinction between 0-coplanar and $\ensuremath{\pi}$-coplanar phases in the latter region is fundamentally impossible from the symmetry-preserving finite-size calculations with fixed magnon number. Therefore, we also perform a cluster mean-field plus scaling analysis for small spins $S\ensuremath{\le}3/2$. The obtained results, together with the previous large-SSS analysis, indicate that the $\ensuremath{\pi}$-coplanar phase exists for any SSS except for the classical limit $(S\ensuremath{\rightarrow}\ensuremath{\infty})$ and the existence range in J/JzJ/{J}_{z}J/Jz​ is largest in the most quantum case of S=1/2S=1/2S=1/2.