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Journal of Physics Conference Series

Entanglement with negative Wigner function of three thousand atoms heralded by one photon

Robert McConnell, Hao Zhang, Jiazhong Hu, Senka Ćuk, Vladan Vuletić

Published Jun 1, 2016• 3 citations
Publisher

Abstract

Quantum-mechanically correlated (entangled) states of many particles are of interest in quantum information, quantum computing and quantum metrology. Metrologically useful entangled states of large atomic ensembles have been experimentally realized [1, 2, 3, 4, 5, 6, 7, 8, 9, 10], but these states display Gaussian spin distribution functions with a non-negative Wigner function. Non-Gaussian entangled states have been produced in small ensembles of ions [11, 12], and very recently in large atomic ensembles [13, 14, 15]. Here, we generate entanglement in a large atomic ensemble via the interaction with a very weak laser pulse; remarkably, the detection of a single photon prepares several thousand atoms in an entangled state. We reconstruct a negative-valued Wigner function, an important hallmark of nonclassicality, and verify an entanglement depth (minimum number of mutually entangled atoms) of 2910 ± 190 out of 3100 atoms. Attaining such a negative Wigner function and the mutual entanglement of virtually all atoms is unprecedented for an ensemble containing more than a few particles. While the achieved purity of the state is slightly below the threshold for entanglement-induced metrological gain, further technical improvement should allow the generation of states that surpass this threshold, and of more complex Schrödinger cat states for quantum metrology and information processing.

DOI
10.1088/1742-6596/723/1/012054

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Quantum-mechanically correlated (entangled) states of many particles are of interest in quantum information, quantum computing and quantum metrology. Metrologically useful entangled states of large atomic ensembles have been experimentally realized [1, 2, 3, 4, 5, 6, 7, 8, 9, 10], but these states display Gaussian spin distribution functions with a non-negative Wigner function. Non-Gaussian entangled states have been produced in small ensembles of ions [11, 12], and very recently in large atomic ensembles [13, 14, 15]. Here, we generate entanglement in a large atomic ensemble via the interaction with a very weak laser pulse; remarkably, the detection of a single photon prepares several thousand atoms in an entangled state. We reconstruct a negative-valued Wigner function, an important hallmark of nonclassicality, and verify an entanglement depth (minimum number of mutually entangled atoms) of 2910 ± 190 out of 3100 atoms. Attaining such a negative Wigner function and the mutual entanglement of virtually all atoms is unprecedented for an ensemble containing more than a few particles. While the achieved purity of the state is slightly below the threshold for entanglement-induced metrological gain, further technical improvement should allow the generation of states that surpass this threshold, and of more complex Schrödinger cat states for quantum metrology and information processing.
The generation of entanglement in atomic systems plays a central topic in the fields of quantum information storage and processing. Moreover, a special category of entangled states of multi-atom ensembles, spin squeezed states, have been proven to lead to considerable improvement in the sensitivity of precision measurements compared to systems involving uncorrelated atoms. A treatment of entanglement in open systems is, however, incomplete without a precise description of the process of decoherence which necessarily accompanies it. The theory of entanglement and decoherence are the two main topics of this thesis. Methods are described for the generation of strong correlations in large atomic ensembles using either cavity quantum electrodynamics or measurement outcome conditioned quantum dynamics. Moreover, the description of loss of entanglement resulting from the coupling to a noise reservoir (electromagnetic vacuum) is explored. A spin squeezing parameter is used throughout this thesis as both a measure of entanglement strength and as an indication of the sensitivity improvement above the so-called standard quantum limit (sensitivity obtained with uncorrelated particles) in metrology. The first scheme considered consists of a single mode cavity field interacting with a collection of atoms for which spin squeezing is produced in both resonant and off-resonant regimes. In the resonant case, transfer of squeezing from a field state to the atoms is analyzed, while in the off-resonant regime squeezing is produced via an effective nonlinear interaction (one-axis twisting Hamiltonian). A second, more experimentally realistic case, is one involving the interaction of free space atoms with laser pulses; a projective measurement of a source field originating from atomic fluctuations provides a means of preparing atomic collective states such as spin squeezed and Schrodinger cat states. A new unravelling is proposed, that employs the detection of photon number in a single output channel and is capable of producing mesoscopic Schrodinger cat states in a single step. As a first step to understanding the role of cooperative decoherence, of importance in the case of dense pencil-shaped atomic ensembles, the collective spin decoherence of a two multilevel atom system is derived. This calculation is also relevant to entanglement loss for two qubits manipulated using with reading/writing pulses. Finally, a scheme is proposed in which arbitrarily strong entanglement can be produced in a four-wave mixing setup, where the preparation of the atoms in a dark state limits the decoherence to negligible values.
We propose and analyze a probabilistic but heralded scheme to generate pure, entangled, non-Gaussian states of collective spin in large atomic ensembles by means of single-photon detection. One photon announces the preparation of a Dicke state, while two or more photons announce Schr\"odinger cat states. The method produces pure states even for finite photon detection efficiency and weak atom-photon coupling. The entanglement generation can be made quasideterministic by means of repeated trial and feedback, enabling metrology beyond the standard quantum limit.
Quantum physics allows for entanglement between microscopic and macroscopic objects, described by discrete and continuous variables, respectively. As in Schrödinger's famous cat gedanken experiment, a box enclosing the objects can keep the entanglement alive. For applications in quantum information processing, however, it is essential to access the objects and manipulate them with suitable quantum tools. Here we reach this goal and deterministically generate entangled light-matter states by reflecting a coherent light pulse with up to four photons on average from an optical cavity containing one atom. The quantum light propagates freely and reaches a remote receiver for quantum state tomography. We produce a plethora of quantum states and observe negative-valued Wigner functions, a characteristic sign of non-classicality. As a first application, we demonstrate a quantum-logic gate between an atom and a light pulse, with the photonic qubit encoded in the phase of the light field.
In Chapter 7 we discussed the interaction between atoms and photons. We found that the coupling between a single atom and a single photon is rather weak, unless the atom and the photon are contained within a small cavity. The only way to significantly affect a free atom with light is to use a state of light with many photons, and in particular we showed how to use classical laser fields to prepare particular atomic states. However, there is another way of enhancing the interaction in a useful way. We can use many atoms rather than a single one. In this chapter, we will show that the interaction between a single photon and an ensemble of atoms can be greatly increased through the phenomenon of collective enhancement. We will show that this gives an atomic ensemble a relatively large susceptibility, and that multilevel atoms can be used to generate large optical nonlinearities. These offer the possibility of slowing, and even stopping, a beam of light; a phenomenon that goes hand in hand with electromagnetically induced transparency. We will discuss how a quantum state of light can be stored in and retrieved from an ensemble of atoms, and how the states of different atomic ensembles can be entangled with one another. We will show that collective states of atoms can even be used as a single qubit or several qubits, and finally, we will show that atomic ensembles can be use to mediate a photon–photon interaction.
In the present PhD work, we focus on a specific class of quantum states of light: the non-Gaussian states. These states have the particularity of exhibiting Wigner functions with some negative values. This quantum feature is a necessary condition to perform some quantum computation task; furthermore it is also useful for various other applications, including quantum communication and metrology. Different strategies can be used to generate these states. Here, we start from Gaussian states produced by optical parametric oscillators in the continuous wave regime, (i.e. single-mode and two-mode squeezed vacuum states). The non-Gaussian feature can only be obtained by non-linear phenomena (over-quadratic Hamiltonian). In our case, the non-linearity is induced by photon-counting-based measurements (also called non-Gaussian measurements). This study is mainly divided into two parts. First, the generation of non-classical states associated with two types of qubit encoding: the single-photon state, used for quantum information with discrete variables, and the coherent state superposition (the so-called optical Schrodinger cat state), used for quantum information with continuous variables. These two states have then been used to perform some quantum information protocols. The first one addresses the problem of single-photon entanglement witness, and the other the generation of entanglement between the two encodings (also called hybrid entanglement).
All Together Now In quantum entanglement, correlations between particles mean that the measurement of one determines the outcome of the other(s). Generally, when trying to exploit quantum entanglement, the larger the number of entangled particles, the better. However, the size of entangled systems has been limited. Haas et al. (p. 180 , published online 27 March; see the Perspective by Widera ) prepared a small ensemble of ultracold atoms into a collective entangled state. Starting from one internal quantum state, the system of cold atoms was excited with a weak microwave pulse leading to a small excitation probability. Because it is not known which atom is promoted into the excited state, the detection of one quantum of excitation projects the system into an entangled quantum state, called a W-state. A fast repeat-until-success scheme produced such W-states quasi-deterministically. Using such a technique was able to yield entangled states of more than 40 particles. The relatively large ensemble-entangled states could potentially in the future find use in quantum sensing or enhanced quantum metrology applications.