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Springer series in chemical physics

Coherent Control in Ultrafast Photon Echo Spectroscopy: Liouville-Space Pathways Interference

Maxim S. Pshenichnikov, Wim P. de Boeij, D. A. Wiersma

Published Jan 1, 1996• 0 citations
Publisher
DOI
10.1007/978-3-642-80314-7_93

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Dephasing-induced resonances, arising from interference between different excitation pathways, are well-known in frequency-domain spectroscopy.[1] It is generally thought that the time-domain analog of this phenomena is difficult to achieve due to the explicit time ordering of the interaction fields.[2,3] In this contribution we report on the observation of time-domain interference in phase-locked stimulated photon echo. We also show how complete control over the interference effect can be exercised.
We demonstrate coherent control over interference between different Liouville-space pathways that describe the generation of the nonlinear optical polarization in a stimulated photon echo. This control was exercised by phase-locking of the excitation pulses and observed in the heterodyne detected echo signal. A theoretical analysis of the effect is presented and found to be in good agreement with the obtained results. The relation between this novel time-domain interference effect and the pressure-induced extra resonance in four-wave mixing spectroscopy is discussed.