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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Higher-order spontaneous parametric down-conversion with back-propagating idler using a submicron poled KTP waveguide

Mark Bashkansky, Marcel W. Pruessner, I. Vurgaftman, Mijin Kim, John F. Reintjes

Published May 19, 2016• 4 citations
Publisher

Abstract

Spontaneous parametric downconversion (SPDC) using periodically poled nonlinear optical crystals under the quasiphase- matching condition has found wide use in quantum optics. High efficiencies and good coupling to single-mode fibers resulted from using channel waveguides in crystals. It is often desirable to have a very narrow bandwidth for the signal and idler photons, but under the typical operating conditions, phase matching dictates the bandwidth of the SPDC to be of the order of <1 nm. This occurs because the co-propagating signal and idler photons are entangled, and an increase of the signal wave-vector is compensated by a decrease of the idler wave-vector. One way to reduce the bandwidth is by forming either external or internal cavities. Additionally, bandwidth reduction is possible without cavities when the signal and idler are counter-propagating, and the changes in the wave-vector with frequency are additive. To accomplish this a domain inversion on the wavelength scale is required. In this work, we experimentally demonstrate SPDC in one-dimensional KTP-based waveguides with sub-micron poling for forward and backward interactions. Some of the spectral features of the generated light are accounted for by mode coupling theory in periodically poled waveguides but other features are as yet not explained.

DOI
10.1117/12.2222303

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Spontaneous parametric downconversion (SPDC) using periodically poled nonlinear optical crystals under the quasiphase- matching condition has found wide use in quantum optics. High efficiencies and good coupling to single-mode fibers resulted from using channel waveguides in crystals. It is often desirable to have a very narrow bandwidth for the signal and idler photons, but under the typical operating conditions, phase matching dictates the bandwidth of the SPDC to be of the order of <1 nm. This occurs because the co-propagating signal and idler photons are entangled, and an increase of the signal wave-vector is compensated by a decrease of the idler wave-vector. One way to reduce the bandwidth is by forming either external or internal cavities. Additionally, bandwidth reduction is possible without cavities when the signal and idler are counter-propagating, and the changes in the wave-vector with frequency are additive. To accomplish this a domain inversion on the wavelength scale is required. In this work, we experimentally demonstrate SPDC in one-dimensional KTP-based waveguides with sub-micron poling for forward and backward interactions. Some of the spectral features of the generated light are accounted for by mode coupling theory in periodically poled waveguides but other features are as yet not explained.
Backward-wave three-wave mixing is a difficult χ (2) interaction to observe, because it requires ultrashort poling periods to achieve phasematching. Having realized sub-micrometer periods in periodically poled KTiOPO 4 (PPKTP), we demonstrate for the first time first-order quasi-phasematched, backward-wave spontaneous parametric downconversion (BW SPDC). We pumped the PPKTP crystal at 800 nm and obtained a forward-wave signal at 1400 nm and a backward-wave idler at 1868 nm. We estimated an internal pair production rate of 4.0 × 10 4 pairs/s/mW. The backward-wave phasematching constraints lead to the unique tuning property that spectral features of the pump are transferred to the forward-wave signal photons, which makes BW SPDC an attractive source of spectrally shaped, heralded single photons. These spectrally shaped photons are useful for quantum computing and quantum interconnects. For the first time, we experimentally show this effect by observing frequency translation between a spectrally shaped pump beam and the BW SPDC signal photons. Due to their unique properties, BW-SPDC-based devices will be important building blocks for quantum information processing.
The properties of the backward-wave spontaneous parametric down-conversion (SPDC) in a periodically poled potassium titanyl phosphate (KTP) waveguide are studied in the context of creating narrowband heralded sources of single-photon states. The effective index of refraction and spatial profile of different waveguide modes, efficiency of different SPDC processes and purity of heralded photons are calculated numerically for a given waveguide. Compared to the usual co-propagating SPDC, spectral narrowing of the backward- wave SPDC was observed as should be expected.
The properties of the backward-wave spontaneous parametric down-conversion (SPDC) in a periodically poled potassium titanyl phosphate (KTP) waveguide are studied in the context of creating narrowband heralded sources of single-photon states. The effective index of refraction and spatial profile of different waveguide modes, efficiency of different SPDC processes and purity of heralded photons are calculated numerically for a given waveguide. Compared to the usual co-propagating SPDC, spectral narrowing of the backward-wave SPDC was observed as should be expected. Generation biphoton states in backward-wave regime is experimentally observed in two-photon detection scheme.
Recently, we verified that spontaneous parametric down conversion (SPDC) is enhanced in a waveguide, in agreement with theory showing an inverse dependence on mode confinement [1]. Here we investigate highly-confined nanophotonic waveguides designed to maximize the SPDC rate. A theory modified to include highly-confined waveguides is used to calculate the spectral width and pair generation rates in a sample system. Pair generation rates exceeding 10(9)/sec/nm/mW are predicted for periodically-poled KTP (PPKTP) nanophotonic waveguides. This results in an enhancement of the downconverted signal power greater than 45x that of low-index-contrast PPKTP waveguides and greater than 6500x that of bulk PPKTP crystals.
We report the generation of frequency-uncorrelated photon pairs from counter-propagating spontaneous parametric down-conversion in a periodically-poled KTP waveguide. The joint spectral intensity of photon pairs is characterized by measuring the corresponding stimulated process, namely, the difference frequency generation process. The experimental result shows a clear uncorrelated joint spectrum, where the backward-propagating photon has a narrow bandwidth of 7.46 GHz and the forward-propagating one has a bandwidth of 0.23 THz like the pump light. The heralded single-photon purity estimated through Schmidt decomposition is as high as 0.996, showing a perspective for ultra-purity and narrow-band single-photon generation. Such unique feature results from the backward-wave quasi-phase-matching condition and does not has a strict limitation on the material and working wavelength, thus fascinating its application in photonic quantum technologies.