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Study on higher-order effect of radiation interacting with medium

Yuexin Liu, Ehv Power

Published Jan 1, 2004• 0 citations
OpenAlex

Abstract

From the theory of quantum mechanics,we studied higher-order effect that radiation field interacts with medium,and got the equation of kinematics of density matrix that medium had excitation in radiation field. From this ,we got the calculating formula when radiation reached saturation.We also got an important conclusion that intensity was in inverse proportion to the square of transition speed and in direct ration to attenuation speed of high and low energy level.

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•Jan 1, 2011•1 citation
From the theory of quantum mechanics,we studied higher-order effect that radiation field interacts with medium,and got the equation of kinematics of density matrix that medium had excitation in radiation field. From this ,we got the calculating formula when radiation reached saturation.We also got an important conclusion that intensity was in inverse proportion to the square of transition speed and in direct ration to attenuation speed of high and low energy level.
Introduction Until now, our discussion of the interaction between radiation and matter has concentrated only on the spectral aspects of radiation. The results could determine the wavelengths for absorption and emission or the selection rules for such transitions, but could not be used to determine the actual extent of emission or absorption. These too are important considerations which are needed to fully quantify radiative energy transfer. Unfortunately, none of the classical theories can predict the extent of emission from an excited medium, or even the extent of absorption. Although the discussion in Section 4.9 (on the propagation of electromagnetic waves through lossy media) touched briefly on the concept of attenuation by absorption, it failed to show the reasons for the spectral properties of the absorption or to accurately predict its extent. We will see later that the classical results are useful only as a benchmark against which the actual absorber is compared. The objective of this chapter is therefore to present an introduction to quantum mechanical processes that control the emission and absorption by microscopic systems consisting of atoms and molecules. The results will then be used to predict the extent of emission by media when excited by an external energy source and to evaluate the absorption of incident radiation. It is now well recognized that all emission or absorption processes are the result of transitions between quantum mechanical energy levels.
Coupled ion pairs in solids have played an important role in the development of new solid-state lasers. The long-range interaction among two or more ions provides a channel for the inversion of population, leading to the discovery of new emission lines. Because of the relatively large optical cross sections, coupled ion pairs may provide new media for the implementation of a solid-state phase conjugate mirror. We present a theory of optical phase conjugation via four-wave mixing in such novel materials. For a model ion-doped solid-state system, the calculations give the following conclusions. First, the spectral linewidth is proportional to the square root of the intensity of the radiation field in an inhomogenously broadened material for fixed ion density. Second, the linewidth decreases with increasing ion density for the fixed intensity level. And last, the saturation intensity also decreases with increasing ion density for the fixed optical intensity. The behavior of the linewidth and the saturation intensity are attributed to the strong interaction among two nearest-neighbor ion pairs, which leads to the generation of additional energy dumping pathways.
In the article, for limited system conditions that form the spatial structure of the field, the attenuation processes of wave packets of finite amplitude are considered. The line width of the wave field may be the result of the dissipative processes (in a quantum system it is inverse of the lifetime of energy levels) or the result of reactive processes (in classical waveguide systems this is the spectral width of the packet). In the case of filling the waveguide with an active two-level medium, a description is possible using a quasiclassical model of the interaction of the field and particles. In this case, the quantum-mechanical description of the medium is combined with the classical representation of the field. Here, the Rabi frequency plays an important role, which determines the probabilities of induced radiation or absorption of field quanta and the oscillatory change in population inversion (nutation). Depending on the relationship between the Rabi frequency and the line width of the wave packet, the process can change the nature of the field behavior. In strong fields or with a significant population inversion, the line width can be neglected, while the field energy density is quite high. In this case, one should expect noticeable nutations of population inversions with different frequencies corresponding to the local Rabi frequency in different regions of the waveguide, the interference of which will determine the oscillatory behavior of the wave field. At a low level of electric field intensity or a slight population inversion, the mode of changing the field amplitude becomes monotonic. Plasma field damping (Landau damping) is considered. The role of population inversion is assumed by a quantity proportional to the derivative with respect to velocity of the electron distribution function. If the spectral width of the packet is small, the process of wave attenuation acquires a characteristic oscillatory form due to the exchange of energy between the wave and the plasma electrons captured by its field. The attenuation of wide packets is almost monotonic with the formation of a characteristic “plateau” in the vicinity of the phase velocity of the wave on the electron velocity distribution function.
This subject introduces the key concepts and formalism of quantum mechanics and their relevance to topics in current research and to practical applications. Starting from the foundation of quantum mechanics and its applications in simple discrete systems, it develops the basic principles of interaction of electromagnetic radiation with matter. Topics covered are composite systems and entanglement, open system dynamics and decoherence, quantum theory of radiation, time-dependent perturbation the...