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Springer series in solid-state sciences

Charge-Spin Separation and Pairing by Chiral Spin Fluctuations

C. Kübert, A. Muramatsu

Published Jan 1, 1994• 0 citations
Publisher
DOI
10.1007/978-3-642-85129-2_21

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We have studied here the topological aspects of monopole superconductivity in 3+1 dimensions. It is pointed out that Heisenberg spin system may be associated with non-Abelian gauge fields. When the spin and charge become separated, spinons and holons emerge and holons interacting with such a gauge field associate a magnetic flux giving rise to nonzero Berry phase and causes the existence of chiral spin liquid. This also suggests that these holons are much heavier than their free counterpart and the pair of such holons forms a bosonic state respecting rotational invariance. Superconductivity arises out of this pair condensation.
Triplet formation and its regulation have always been of central interest in understanding the photophysical behavior of living systems. In organic systems, excessive triplet formation poses significant challenges, as it can promote photochemical damage and reduce the efficiency of charge separation processes, making its regulation critically important.Here, we present a theoretical investigation of the intrinsic quantum spin dynamics governing triplet formation in the heliobacterial reaction center, a system that operates without any internal magnetic field. Using an open quantum systems approach based on the Lindblad formalism, we simulate the spin-correlated radical pair dynamics occurring during charge separation in the heliobacterial reaction center. The study systematically examines how triplet formation is regulated by variations in two key parameters, hyperfine coupling strengths and recombination rates, and how this regulation is further influenced by the inclusion of chirality-induced spin selectivity (CISS) in conjunction with the radical pair mechanism (RPM). Our results demonstrate that the CISS effect significantly suppresses triplet formation across the parameter space relevant to the heliobacterial molecular environment, revealing an intrinsic quantum protective mechanism operating through spin control in heliobacterial photosynthesis.
We study the two-dimensional spin-charge separated Ginzburg-Landau theory containing U(1) gauge interactions as a semi-phenomenological model describing fluctuating condensates in high temperature superconductivity. Transforming the original GL action, we abstract the effective action of Cooper pair. Especially, we clarify how Cooper pair correlation evolves in the normal state from the point of view of spin-charge separation. Furthermore, we point out how Cooper pair couples to gauge field in a gauge-invariant way, stressing the insensitivity of Cooper pair to infrared gauge field fluctuation.