In this paper we report an experiment of concentric coherent anti-Stokes Raman scattering (OARS) and coherent Stokes Raman scattering (CSRS) achieved in the dispersive medium calcite crystal under certain properly designed condition.
We theoretically investigate a scheme in which backward coherent anti-Stokes Raman scattering (CARS) is significantly enhanced by using slow light. Specifically, we reduce the group velocity of the Stokes excitation pulse by introducing a coupling laser that causes electromagnetically induced transparency (EIT). When the Stokes pulse has a spatial length shorter than the CARS wavelength, the backward CARS emission is significantly enhanced. We also investigated the possibility of applying this scheme as a CARS lidar with O2 or N2 as the EIT medium. We found that if nanosecond laser with large pulse energy (>1 J) and a telescope with large aperture (~10 m) are equipped in the lidar system, a CARS lidar could become much more sensitive than a spontaneous Raman lidar.