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Acta Optica Sinica

Full quantum theory of optically pumped two-photon laser

Shuhui Sun

Published Jan 1, 1987• 0 citations
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Abstract

In this paper, the model which consists of homogeneous broadened three atomic level is proposed, when both the pump classical field and laser field exist we discuss the gain, frequency pulling and threshold condition of the weak pumping. We also discuss the effect of the coherent pumping on the laser line width. The results are compared with what derived for non-coherent pumping and no-pumping.

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Physical Review A•Nov 1, 1987•31 citations
In this paper, the model which consists of homogeneous broadened three atomic level is proposed, when both the pump classical field and laser field exist we discuss the gain, frequency pulling and threshold condition of the weak pumping. We also discuss the effect of the coherent pumping on the laser line width. The results are compared with what derived for non-coherent pumping and no-pumping.
The Langevin quantum theory has been used to treat the optically pumped three-level laser system. We derive an equation of motion for laser field in the type of Van der Pol equation when the photon number of the laser field is not too high. It includes not only both incoherent and coherent pumping, but also both strong and weak optical pumping. If an average over reservoir is taken, the equation will give all the semi-classical results. Our results show that the laser gain comes from two basic processes, i.e., a two-photon process and a two-step process. When the pumping strength is larger than some value, the dynamic Stark effect will appear. The laser linewidth is mainly contributed by the thermal noise, the vaecum fluctuation, the spontaneous emissions between the laser levels and the spontaneous Raman scattering.
The Langevin quantum theory has been used to treat the optically pumped three-level laser system. We derive an equation of motion for laser field in a type of Van der Pol equation when the photon number of the laser field is not too high. It includes not only both incoherent and coherent pumping, but also both strong and weak optical pumping. If an average over the reservoir is taken, the equation will give all the semi-classical results. Our results show that the laser gain comes from two basic processes, i.e., a two-photon process and a two-step process. When the pumping strength is larger than a certain value, the dynamic Stark effect will appear. The laser linewidth is mainly contributed by the thermal noise, the vacuum fluctuation, the spontaneous emissions between the laser levels and the spontaneous Raman scattering.
A quantum theory of a two-photon laser is developed by making use of the antinormal-ordering Q function. Starting from the microscopic atom-field interaction Hamiltonian for cascade three-level atoms and including saturable absorbers, we first present a master equation for the field-density operator, and then transform the master equation into a Fokker-Planck equation for the Q function. The Q-function approach enables us to study the two-photon laser analytically, obtaining simple expressions for nonlinear gain, mean photon number, frequency pulling, natural linewidth, and photon-number variance in a unified method. We find that the field in a two-photon laser will build up from a vacuum without triggering if its linear gain is larger than the cavity loss. Also hysteresis can occur in the two-photon laser even without triggering. With an overall two-photon resonance, the normalized photon-number variance approaches a common value 11/8 well above ``threshold,'' independent of the one-photon detuning. We compare these results with previous results obtained from an effective interaction Hamiltonian. We find that the domain of validity of the effective Hamiltonian for the photon-number variance is much smaller than that for the mean photon number. Well above ``threshold'' the effective Hamiltonian overestimates both the natural linewidth and the photon-number variance.
Interaction of two coherent fields of arbitrary intensity with a general homogeneously broadened three-level molecular system for both an amplifier as well as a laser oscillator under general conditions of pumping is discussed. The amplifier solution is obtained through the time-averaged density-matrix formalism with two coherent fields treated classically. A detailed consideration of both real and imaginary parts of the electric susceptibility at pump and emission frequencies, corresponding to gain and dispersion in the active medium has been taken into account. The results obtained are used to study a number of situations for weak and strong pumping in the laser amplifier. Subsequently these are applied to a mode analysis of a unidirectional single-mode laser oscillator to determine the output characteristics of the laser and to establish conditions under which emission becomes dynamically unstable resulting in sustained oscillatory emission. The results obtained are found to be in good agreement with those of a full numerical analysis of the atomic and field coupled equations describing the system.