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Physical review. B./Physical review. B

Laser-induced polarization of a quantum spin system in the steady-state regime

Andrei A. Zvyagin

Published May 9, 2016• 1 citation
Publisher

Abstract

The effect of the circularly polarized laser field on quantum spin systems in the steady-state regime, in which relaxation plays the central role, has been studied. The dynamical mean-field-like theory predicts several general results for the behavior of the time-average magnetization caused by the laser field. The induced magnetization oscillates with the frequency of the laser field (while Rabi-like oscillations, which modulate the latter in the dynamical regime, are damped by the relaxation in the steady-state regime). At high frequencies, that magnetization is determined by the value to which the relaxation process is directed. At low frequencies the slope of that magnetization as a function of the frequency is determined by the strength of the laser field. The anisotropy determines the resonance behavior of the time-averaged magnetization in both the ferromagnetic and antiferromagnetic cases with nonzero magnetic anisotropy. Nonlinear effects (in the magnitude of the laser field) have been considered. The effect of the laser field on quantum spin systems is maximal in resonance, where the time-averaged magnetization, caused by the laser field, is changed essentially. Out of resonance the changes in the magnetization are relatively small. The resonance effect is caused by the nonzero magnetic anisotropy. The resonance frequency is small (proportional to the anisotropy value) for spin systems with ferromagnetic interactions and enhanced by exchange interactions in the spin systems with antiferromagnetic couplings. We show that it is worthwhile to study the laser-field-induced magnetization of quantum spin systems caused by the high-frequency laser field in the steady-state regime in ``easy-axis'' antiferromagnetic spin systems (e.g., in Ising-like antiferromagnetic spin-chain materials). The effects of the Dzyaloshinskii-Moriya interaction and the spin-frustration couplings (in the case of the zigzag spin chain) have been analyzed.

DOI
10.1103/physrevb.93.184407

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The effect of the circularly polarized laser field on quantum spin systems in the steady-state regime, in which relaxation plays the central role, has been studied. The dynamical mean-field-like theory predicts several general results for the behavior of the time-average magnetization caused by the laser field. The induced magnetization oscillates with the frequency of the laser field (while Rabi-like oscillations, which modulate the latter in the dynamical regime, are damped by the relaxation in the steady-state regime). At high frequencies, that magnetization is determined by the value to which the relaxation process is directed. At low frequencies the slope of that magnetization as a function of the frequency is determined by the strength of the laser field. The anisotropy determines the resonance behavior of the time-averaged magnetization in both the ferromagnetic and antiferromagnetic cases with nonzero magnetic anisotropy. Nonlinear effects (in the magnitude of the laser field) have been considered. The effect of the laser field on quantum spin systems is maximal in resonance, where the time-averaged magnetization, caused by the laser field, is changed essentially. Out of resonance the changes in the magnetization are relatively small. The resonance effect is caused by the nonzero magnetic anisotropy. The resonance frequency is small (proportional to the anisotropy value) for spin systems with ferromagnetic interactions and enhanced by exchange interactions in the spin systems with antiferromagnetic couplings. We show that it is worthwhile to study the laser-field-induced magnetization of quantum spin systems caused by the high-frequency laser field in the steady-state regime in ``easy-axis'' antiferromagnetic spin systems (e.g., in Ising-like antiferromagnetic spin-chain materials). The effects of the Dzyaloshinskii-Moriya interaction and the spin-frustration couplings (in the case of the zigzag spin chain) have been analyzed.
It is shown that a linear polarized laser can cause magnetization of a spin system with magnetic anisotropy, the distinguished axis of which is perpendicular to the polarization of the laser field. In the dynamical regime the magnetization oscillates around the nonzero value determined by the parameters of the system. Oscillations have the frequency of the laser field, modulated by the lower Rabi-like frequencies. In the steady-state regime, for a large time scale greater than the characteristic relaxation time, the Rabi-like oscillations are damped, and the magnetization oscillates with the frequency of the laser field around the value which is determined by the relaxation rate also. Analytic results are presented for the spin-1/2 chain. The most direct manifestation of such a behavior can be observed in spin-1/2 Ising chain materials if the linear polarization of the laser field is chosen to be perpendicular to the Ising axis.
We theoretically predict a nonequilibrium phase transition in quantum spin systems induced by a laser, which provides a purely quantum-mechanical way of coherently controlling magnetization. Namely, when a circularly polarized laser is applied to a spin system, the magnetic component of a laser is shown to induce a magnetization normal to the plane of polarization, leading to an ultrafast phase transition. We first demonstrate this phenomenon numerically for an S=1S=1S=1 antiferromagnetic Heisenberg spin chain, where a new state emerges with magnetization perpendicular to the polarization plane of the laser in place of the topologically ordered Haldane state. We then elucidate its physical mechanism by mapping the system to an effective static model. The theory also indicates that the phenomenon should occur in general quantum spin systems with a magnetic anisotropy. The required laser frequency is in the terahertz range, with the required intensity being within a prospective experimental feasibility.
Dynamical non-equilibrium effects after a quantum quench in a quantum spin system, which permits exact analytical solution in both closed and open cases, are studied. The exact analytic results are obtained for the bi-axial paramagnet, both for the “easy axis”- and the “easy-plane”-like situations, and for the field directed along both principal axes of the system. Quantum quench of the external magnetic field produces a nonlinear response. For the closed system the average magnetic moment oscillates with time and with the final value of the external field. Such oscillations exist also for the open system, connected to the bath, in the dynamical regime. For the steady-state regime in the open case the oscillations are damped. Non-equilibrium effects yield specific hysteresis phenomena in the considered single spin system.
The dynamical mean-field-like theory of the electron spin resonance (ESR) in spin-1/2 chains with nearest and next-nearest neighbor interactions (or zigzag spin ladders) and alternation is developed. It is explained that either the magnetic anisotropy of spin-spin couplings or the Dzyaloshinskii-Moriya interaction causes shifts of the resonance position in spin chains, comparing to only magnetically isotropic interactions. The power of the ac ESR field, absorbed by the spin chain, is calculated. It is shown that the temperature dependence of the shift of the resonance position is related to the temperature dependence of the ESR absorption. Depending on the strength of next-nearest neighbor interactions, the shift of the ESR position can become either exponentially small or can be increased near quantum critical points. The absorbed by the alternating spin chain power of the ac magnetic field is calculated, manifesting two resonances. The influence of mentioned spin-spin interactions on the linewidth of the ESR is analyzed.
The time evolution of magnetization induced by circularly polarized light in an S=1S=1S=1 Heisenberg chain with large easy-plane anisotropy is studied numerically and analytically. Results at constant light frequency $\mathrm{\ensuremath{\Omega}}={\mathrm{\ensuremath{\Omega}}}_{0}$ are interpreted in terms of absorption lines of the electronic spin resonance spectrum. The application of time-dependent frequency $\mathrm{\ensuremath{\Omega}}=\mathrm{\ensuremath{\Omega}}(t)$ light, so called chirping, is shown to be an efficient procedure in order to obtain within a short time a large, controlled value of the magnetization Mz{M}^{z}Mz. Furthermore, comparison with a two-level model provides a qualitative understanding of the induced magnetization process.
Exact results for time evolution of a many-body quantum system (a transverse field Ising spin chain) under the action of several pulses of an external field are obtained. Unlike the situation with a single pulse, the magnetization depends on time for the sequence of two pulses. For the two-pulse case the magnetization does not depend on the value of the time spacing between pulses, in sharp contrast with the standard spin echo cases. Modulated oscillations of magnetization with time do not decay if the energy of eigenstates of the system before pulses is kkk independent (k(k(k is the quasimomentum), while for kkk-dependent initial eigenstates the modulated oscillations of magnetization decay (without inclusion of the ``external'' relaxation) to the steady-state value, depending on the parameters of pulses; i.e., the oscillations reveal time irreversibility.