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IEEE Transactions on Applied Superconductivity

Superconducting NbN Nanowires and Coherent Quantum Phase-Slips in DC Transport

J. C. Fenton, Jonathan Burnett

Published Feb 19, 2016• 5 citations
Publisher

Abstract

A quantum current standard dual to the Josephson voltage standard has been trumpeted as a primary application for the phenomenon of coherent quantum phase-slips (CQPS) in superconducting nanowires, but it requires a dc transport geometry, distinct from the ring geometry in which CQPS have been probed by microwave spectroscopy measurements. We present measurements on NbN nanowires with a width of 15 nm and including integrated thin-film resistors to provide a high-impedance environment. Analysis shows that the nanowire behavior is in line with expectations. The results demonstrate that the process is promising both for future dc transport CQPS measurements and for the fabrication of other circuits in which low-width superconducting nanowires are required.

DOI
10.1109/tasc.2016.2531005

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A quantum current standard dual to the Josephson voltage standard has been trumpeted as a primary application for the phenomenon of coherent quantum phase-slips (CQPS) in superconducting nanowires, but it requires a dc transport geometry, distinct from the ring geometry in which CQPS have been probed by microwave spectroscopy measurements. We present measurements on NbN nanowires with a width of 15 nm and including integrated thin-film resistors to provide a high-impedance environment. Analysis shows that the nanowire behavior is in line with expectations. The results demonstrate that the process is promising both for future dc transport CQPS measurements and for the fabrication of other circuits in which low-width superconducting nanowires are required.
The phenomenon of coherent quantum phase-slips (CQPS) in superconducting nanowires was some time ago proposed to be the exact dual of the Josephson effect, a proposal accompanied by predictions of a new quantum current standard dual to the Josephson voltage standard. Unambiguous experimental observation of CQPS in nanowire structures has only recently been achieved through microwave spectroscopy which showed an avoided crossing between flux states for a superconducting ring interrupted by a superconducting nanowire. This observation raises expectations that the CQPS quantum current standard and a slew of CQPS devices dual to devices containing Josephson junction might be realised, including a tunable capacitance, a sensitive charge detector and small-signal detector. To date, experimental evidence for CQPS in a dc transport geometry has not been considered conclusive, and the impact of decoherence in CQPS devices still remains to be evaluated. We present experimental work which has enabled us to crystallise pertinent issues which have prevented the realisation of CQPS in dc transport experiments to date.
Abstract Quantum phase slip (QPS) is an important effect that occurs in one-dimensional (1D) or quasi-1D superconducting (SC) materials. Due to the extremely high requirements on the uniformity and quality of SC nanowires, it is currently very challenging to obtain repeatable and controllable QPS devices. Here, we report a systematic study of the QPS effect in NbN SC nanowires. High-quality NbN nanowires with different widths are fabricated by combining the processes of photo-lithography, electron beam lithography, and inductively coupled plasma etching. It is found that the electrical transport of the nanowires showed a systematic variation with the wire width, and a clear evolution from single to multiple QPS events with the decrease in wire width is uncovered at low temperatures. Based on these experimental results, the phase diagram reflecting the evolution of the physical states of the nanowires with wire width and temperature is obtained. In addition, we observed the features of the critical voltage, which is a characteristic of the occurrence of coherent QPS (cQPS), in samples with a width of 36 nm in the multiple QPS region. It is worth noting that this cQPS behavior was detected in a non-high-impedance environment.
We present a detailed report of microwave irradiation of ultranarrow superconducting nanowires. In our nanofabricated circuits containing a superconducting NbSi nanowire, a dc blockade of current flow was observed at low temperatures below a critical voltage Vc{V}_{\mathrm{c}}Vc​, a strong indicator of the existence of quantum phase-slip (QPS) in the nanowire. We describe the results of applying microwaves to these samples, using a range of frequencies and both continuous-wave and pulsed drive, in order to search for dual Shapiro steps which would constitute an unambiguous demonstration of quantum phase-slip. We observed no steps, and our subsequent thermal analysis suggests that the electron temperature in the series CrO resistors was significantly elevated above the substrate temperature, resulting in sufficient Johnson noise to wash out the steps. To understand the system and inform future work, we have constructed a numerical model of the dynamics of the circuit for dc and ac bias (both continuous-wave and pulsed drive signals) in the presence of Johnson noise. Using this model, we outline important design considerations for device and measurement parameters which should be used in any future experiment to enable the observation of dual Shapiro steps at experimentally accessible temperatures and, thus, lead to the development of a QPS-based quantum current standard.
Quantum phase slips (QPS) or the macroscopic quantum tunneling (MQT) of a nanowire’s order parameter through an activation energy barrier have remained the subject of intense debate for many years. They are expected to occur at low enough temperature where thermally activated phase slips (TAPS) have been frozen out in analogy with Josephson junctions where the macroscopic tunneling of phase at low temperatures has been conclusively experimentally demonstrated. We address this question by following a similar experimental strategy to that employed for establishing MQT in JJs. By measuring switching current distributions, we can probe the phase slip rate and determine if it corresponds to thermal activation or quantum tunneling. Having established that the behavior we see is consistent with being in the quantum regime, we can alter properties of the nanowires and see if the response is consistent with the expectations of the quantum model. To do this we employ an in-situ modification technique using high bias voltage pulses. Using these pulses, we can change resistance, critical temperature, critical current and morphology of the nanowire. We can also change the shunting capacitance of the nanowire by altering the photolithography step used to create the nanowires electrodes. The resulting response of the nanowires agrees well with being in the quantum tunneling dominated regime. An interesting side benefit of the pulsing technique is that we can exactly set the nanowires switching current to a desired value. This may be instrumental in the development of superconducting nanowire qubits.
An accurate standard of electric current is a long-standing challenge of modern metrology. It has been predicted that a superconducting nanowire in the regime of quantum fluctuations can be considered as the dynamic equivalent of a chain of conventional Josephson junctions. In full analogy with the quantum standard of electric voltage based on the Josephson effect, the quantum phase slip phenomenon in ultrathin superconducting nanowires could be used for building the quantum standard of electric current. This work presents advances toward this ultimate goal.
At low temperatures non-equilibrium voltage fluctuations can be generated in current-biased superconducting nanowires due to proliferation of quantum phase slips (QPS) or, equivalently, due to quantum tunneling of magnetic flux quanta across the wire. In this paper we review and further extend recent theoretical results related to this phenomenon. Employing the phase-charge duality arguments combined with Keldysh path integral technique we analyze such fluctuations within the two-point and four-point measurement schemes demonstrating that voltage noise detected in such nanowires in general depends on the particular measurement setup. In the low frequency limit we evaluate all cumulants of the voltage operator which turn out to obey Poisson statistics and exhibit a power law dependence on the external bias. We also specifically address a non-trivial frequency dependence of quantum shot noise power spectrum SΩ for both longer and shorter superconducting nanowires. In particular, we demonstrate that SΩ decreases with increasing frequency Ω and vanishes beyond a threshold value of Ω at T → 0. Furthermore, we predict that SΩ may depend non-monotonously on temperature due to quantum coherent nature of QPS noise. The results of our theoretical analysis can be directly tested in future experiments with superconducting nanowires.