Computing Correlated Electrons: Roadmap and Roadblocks

David Sénéchal, A.–M. S. Tremblay, C. Bourbonnais

D. Scott Holmes, Erik P. DeBenedictis

The International Roadmap for Devices and Systems (IRDS) recently succeeded the International Technology Roadmap for Semiconductors (ITRS). The roadmap driver changed from scaling physical dimensions to application requirements and now includes a broader range of non-semiconductor technologies, such as superconductor electronics (SCE). We review current applications for SCE, ranging from development activities to small- scale commercial products. Computational accelerators within data centers and other future applications will require significant improvements in circuit density, complexity, functional capability, memory capacity, and data rates in and out of the cryogenic environment. As a first step, we propose to develop an application-driven roadmap for superconducting digital computing that will include key decisions to be made by the superconductor electronics community.

Pinaki Sengupta

Fabio Caruso, Michael A. Sentef, Claudio Attaccalite +7 more

The exploration of ultrafast phenomena is a frontier of condensed matter research, where the interplay of theory, computation, and experiment is unveiling new opportunities for understanding and engineering quantum materials. With the advent of advanced experimental techniques and computational tools, it has become possible to probe and manipulate nonequilibrium processes at unprecedented temporal and spatial resolutions, providing insights into the dynamical behavior of matter under extreme conditions. These capabilities have the potential to revolutionize fields ranging from optoelectronics and quantum information to catalysis and energy storage. This roadmap captures the collective progress and vision of leading researchers, addressing challenges and opportunities across key areas of ultrafast science and condensed matter. Contributions in this roadmap span the development of ab initio methods for time-resolved spectroscopy, the dynamics of driven correlated systems, the engineering of materials in optical cavities, and the adoption of FAIR principles for data sharing and analysis. Together, these efforts highlight the interdisciplinary nature of ultrafast research and its reliance on cutting-edge methodologies, including quantum electrodynamical density-functional theory, correlated electronic structure methods, nonequilibrium Green’s function approaches, quantum and ab initio simulations.

Steven Allan Kivelson

Fabio Caruso, Michael A. Sentef, Claudio Attaccalite +27 more

Abstract The exploration of ultrafast phenomena is a frontier of condensed matter research, where the interplay of theory, computation, and experiment is unveiling new opportunities for understanding and engineering quantum materials. With the advent of advanced experimental techniques and computational tools, it has become possible to probe and manipulate nonequilibrium processes at unprecedented temporal and spatial resolutions, providing insights into the dynamical behavior of matter under extreme conditions. These capabilities have the potential to revolutionize fields ranging from optoelectronics and quantum information to catalysis and energy storage. This roadmap captures the collective progress and vision of leading researchers, addressing challenges and opportunities across key areas of ultrafast science and condensed matter. Contributions in this roadmap span the development of ab initio methods for time-resolved spectroscopy, the dynamics of driven correlated systems, the engineering of materials in optical cavities, and the adoption of FAIR principles for data sharing and analysis. Together, these efforts highlight the interdisciplinary nature of ultrafast research and its reliance on cutting-edge methodologies, including quantum electrodynamical density-functional theory, correlated electronic structure methods, nonequilibrium Green’s function approaches, quantum and ab initio simulations.