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Nature Communications

Laser spectroscopic probing of coexisting superfluid and insulating states of an atomic Bose–Hubbard system

Shinya Kato, Kensuke Inaba, Seiji Sugawa, Kosuke Shibata, Ryuta Yamamoto, Makoto Yamashita, Yoshiro Takahashi

Published Apr 20, 2016• 29 citations
Publisher

Abstract

A system of ultracold atoms in an optical lattice has been regarded as an ideal quantum simulator for a Hubbard model with extremely high controllability of the system parameters. While making use of the controllability, a comprehensive measurement across the weakly to strongly interacting regimes in the Hubbard model to discuss the quantum many-body state is still limited. Here we observe a great change in the excitation energy spectra across the two regimes in an atomic Bose-Hubbard system by using a spectroscopic technique, which can resolve the site occupancy in the lattice. By quantitatively comparing the observed spectra and numerical simulations based on sum rule relations and a binary fluid treatment under a finite temperature Gutzwiller approximation, we show that the spectra reflect the coexistence of a delocalized superfluid state and a localized insulating state across the two regimes.

DOI
10.1038/ncomms11341

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A system of ultracold atoms in an optical lattice has been regarded as an ideal quantum simulator for a Hubbard model with extremely high controllability of the system parameters. While making use of the controllability, a comprehensive measurement across the weakly to strongly interacting regimes in the Hubbard model to discuss the quantum many-body state is still limited. Here we observe a great change in the excitation energy spectra across the two regimes in an atomic Bose-Hubbard system by using a spectroscopic technique, which can resolve the site occupancy in the lattice. By quantitatively comparing the observed spectra and numerical simulations based on sum rule relations and a binary fluid treatment under a finite temperature Gutzwiller approximation, we show that the spectra reflect the coexistence of a delocalized superfluid state and a localized insulating state across the two regimes.
Ultracold atomic gases may be the ultimate quantum simulator.These isolated systems have the lowest temperatures in the observable universe, and their properties and interactions can be precisely and accurately tuned across a full spectrum of behaviors, from few-body physics to highly-correlated many-body effects.The ability to impose potentials on and tune interactions within ultracold gases to mimic complex systems mean they could become a theorist's playground.One of their great strengths, however, is also one of the largest obstacles to this dream: isolation.This thesis touches on both of these themes.First, methods to characterize phases and quantum critical points, and to construct finite temperature phase diagrams using experimentally accessible observables in the Bose Hubbard model are discussed.Then, the transition from a weakly to a strongly interacting Bose-Fermi mixture in the continuum is analyzed using zero temperature numerical techniques.Real materials can be emulated by ultracold atomic gases loaded into optical lattice potentials.We discuss the characteristics of a single boson species trapped in an optical lattice (described by the Bose Hubbard model) and the hallmarks of the quantum critical region that separates the superfluid and the Mott insulator ground states.We propose a method to map the quantum critical region using the single, experimentally accessible, local quantity R, the ratio of compressibility to local number fluctuations.The procedure to map a phase diagram with R is easily generalized to inhomogeneous systems and generic many-body Hamiltonians.We illustrate it here using quantum Monte Carlo simulations of the 2D Bose Hubbard model.Secondly, we investigate the transition from a degenerate Fermi gas weakly coupled List of Tables Table Page 2.1 Techniques to Probe Atoms in Optical Lattices . . . . . .
We study the ground-state properties of ultracold bosons in an optical lattice in the regime of strong interactions. The system is described by a non-standard Bose–Hubbard model with both occupation-dependent tunneling and on-site interaction. We find that for sufficiently strong coupling, the system features a phase transition from a Mott insulator with one particle per site to a superfluid of spatially extended particle pairs living on top of the Mott background—instead of the usual transition to a superfluid of single particles/holes. Increasing the interaction further, a superfluid of particle pairs localized on a single site (rather than being extended) on top of the Mott background appears. This happens at the same interaction strength where the Mott-insulator phase with two particles per site is destroyed completely by particle–hole fluctuations for arbitrarily small tunneling. In another regime, characterized by weak interaction but high occupation numbers, we observe a dynamical instability in the superfluid excitation spectrum. The new ground state is a superfluid, forming a two-dimensional (2D) slab, localized along one spatial direction that is chosen spontaneously.
We provide a numerical method to calculate comprehensively the microwave and the laser spectra of ultracold bosonic atoms in optical lattices at finite temperatures. Our formulation is built up with the sum rules, up to the second order, derived from the general principle of spectroscopy. The sum rule approach allows us to discuss the physical origins of a spectral peak shift and also a peak broadening. We find that a spectral broadening of superfluid atoms can be determined from number fluctuations of atoms, while that of normal-state atoms is mainly attributed to quantum fluctuations resulting from hopping of atoms. To calculate spectra at finite temperatures, based on the sum rule approach, we provide a two-mode approximation assuming that spectra of the superfluid and normal state atoms can be calculated separately. Our method can properly deal with multipeak structures of spectra resulting from thermal fluctuations and also coexisting of the superfluid and the normal states. By combining the two-mode approximation with a finite temperature Gutzwiller approximation, we calculate spectra at finite temperatures by considering realistic systems, and the calculated spectra show nice agreements with those in experiments.
We investigate a strongly correlated Bose gas in an optical lattice. Extending the standard-basis operator method developed by Haley and Erd\"os to a boson Hubbard model, we calculate excitation spectra in the superfluid phase, as well as in the Mott insulating phase, at T=0T=0T=0. In the Mott phase, the excitation spectrum has a finite energy gap, reflecting the localized character of atoms. In the superfluid phase, the excitation spectrum is shown to have an itinerant-localized dual structure, where the gapless Bogoliubov mode (which describes the itinerant character of superfluid atoms) and a band with a finite energy gap coexist. We also show that the rf-tunneling current measurement would give useful information about the duality of a strongly correlated superfluid Bose gas near the superfluid-insulator transition.
Ultracold bosonic gases in optical lattices are strongly correlated quantum systems similar to solids. The strong correlation between the electrons in a solid on the one hand, and the bosonic atoms in optical lattice on the other, exhibit various quantum phenomena like insulation, conductivity, localization of electrons and atoms, respectively. Controlled by the intensity of the lattice laser, the ultracold bosonic gas can be transferred from a regime with superfluid character for shallow lattices into a regime of strong correlations, the Mott insulator. As an additional external parameter besides the lattice depth, one can generate spatial inhomogeneities by superimposing an additional standing wave (so-called two-color superlattices), which gives rise to localization effects or the formation of a Bose-glass phase. In the present work, numerical simulations are employed in order to investigate characteristic signatures of the quantum phases in the low-energy excitation spectrum of one-dimensional systems. We simulate temporal small amplitude modulations of the optical lattice in analogy to experiments, and evaluate the response of the system from the time-evolved initial state. The lattice systems are described in the framework of the Bose-Hubbard model. For the evaluation of the time-evolved state, we employ several numerical methods. We analyze systems of small size (6 particles on 6 sites) using an exact time-evolution by integration of the time-dependent Schrödinger equation. The formulation of an importance truncation scheme enables us to retain only the relevant components of the model space in the strongly correlated regime and, thus, allows for the investigation of systems with 10 particles on 10 sites using exact time-evolution. Based on this method, we present results of the Mott-insulating regime as well as for the Bose-glass phase. Furthermore, we employ particle-hole methods, which allow for the treatment of systems with experimental lattice sizes and particle numbers. Starting from the equation of motion method we adapt the Tamm-Dancoff approximation as well as the random-phase approximation for the occupation number representation of the Bose-Hubbard model. We present results of simulations of up to 50 particles on 50 sites and discuss the impact of the lattice depth on the low-energy excitations (U-resonance). Moreover, the impact of a two-color superlattice and the variation of its amplitude is investigated.
We present an experimental measurement of the ensemble averages of both the kinetic and interaction energies of the three-dimensional Bose-Hubbard model at finite temperature and various optical lattice depths across weakly to strongly interacting regimes, for an almost unit filling factor within single-band tight-binding approximation. The kinetic energy is obtained through Fourier transformation of a time-of-flight signal, and the interaction energy is measured using a newly developed atom-number-projection spectroscopy technique, by exploiting an ultranarrow optical transition of two-electron atoms. The obtained experimental results can be used as benchmarks for state-of-the-art numerical methods of quantum many-body theory. As an illustrative example, we compare the measured energies with numerical calculations involving the Gutzwiller and cluster-Gutzwiller approximations, assuming realistic trap potentials and particle numbers at nonzero entropy (finite temperature); we obtain good agreement without fitting parameters. We also discuss the possible application of this method to temperature estimations for atoms in optical lattices using the thermodynamic relation. This study offers a unique advantage of cold atom system for ``quantum simulators.''