Critical velocity and dissipation mechanism in finite superfluid $^4$ He nanodropletsCritical velocity and dissipation mechanism in finite superfluid $^4$He nanodroplets

Keshav Sishodia, Ernesto García‐Alfonso, Nadine Halberstadt +2 more

A hallmark of superfluidity is the frictionless motion of an object below the Landau critical velocity; Whether this concept applies to nanoscale droplets remains unclear. Using time-dependent density functional theory, we investigate the motion of a sodium atom on the surface and inside a superfluid helium nanodroplet. For surface motion, we identify a critical velocity above which energy dissipation through ripplon excitation and the formation of surface-bound quantized vortices leads to rapid deceleration. Inside the droplet, the atom is slowed down to a steady-state velocity that depends on the initial speed, contrasting experiments reporting a critical velocity for dopants ejected from droplets [Phys. Rev. Lett. 111, 153002 (2013)]. Remarkably, the velocity of the ejected atom is nearly independent of its initial velocity. We demonstrate that this behavior results from the bursting of the bubble surrounding the atom at the droplet surface, challenging the previous experimental interpretation.A hallmark of superfluidity is the frictionless motion of an object below the Landau critical velocity; Whether this concept applies to nanoscale droplets remains unclear. Using time-dependent density functional theory, we investigate the motion of a sodium atom on the surface and inside a superfluid helium nanodroplet. For surface motion, we identify a critical velocity above which energy dissipation through ripplon excitation and the formation of surface-bound quantized vortices leads to rapid deceleration. Inside the droplet, the atom is slowed down to a steady-state velocity that depends on the initial speed, contrasting experiments reporting a critical velocity for dopants ejected from droplets [Phys. Rev. Lett. 111, 153002 (2013)]. Remarkably, the velocity of the ejected atom is nearly independent of its initial velocity. We demonstrate that this behavior results from the bursting of the bubble surrounding the atom at the droplet surface, challenging the previous experimental interpretation.

arXiv:2610.35728Oct 26, 20260 citations

Dynamics of Superfluids

WORLD SCIENTIFIC eBooksFeb 1, 20080 citations

Optical centrifuge as a probe of strong dissipative coupling between a molecular rotor and superfluid helium

Ian MacPhail-Bartley, Sören E. Mahr, Cameron E. Peters +7 more

A macroscopic manifestation of superfluidity is that objects moving through liquid helium experience negligible friction below the Landau critical velocity. How this frictionless motion breaks down at the nanoscale remains an open question. Molecules embedded in helium nanodroplets represent a well-controlled system for studying this breakdown, yet none has reached the regime of strong dissipative coupling, when energy transfer from the molecule to the superfluid dominates the observed dynamics. Molecular rotation, induced by short laser pulses, offer a suitable probe to reach rotational energies in the range of the roton gap, where superfluid helium supports a large number of elementary excitations. However, the solvation shell around a rotating molecule caps the energy reachable by a free rotor after impulsive excitation well below the roton excitation energy. Here we show that continuous driving with an ultraslow optical centrifuge overcomes this limitation: the strong field dresses the molecule into pendular states whose energies fall within the spectrum of the collective excitations of the superfluid, placing the system in the strong-dissipation regime. The resulting rapid thermalization locks the molecule to the rotating field until the rotation-induced level splittings overtake the thermalization rate, beyond which the molecular alignment is progressively lost. Our approach offers a direct measurement of the molecule-bath coupling in a quantum fluid.A macroscopic manifestation of superfluidity is that objects moving through liquid helium experience negligible friction below the Landau critical velocity. How this frictionless motion breaks down at the nanoscale remains an open question. Molecules embedded in helium nanodroplets represent a well-controlled system for studying this breakdown, yet none has reached the regime of strong dissipative coupling, when energy transfer from the molecule to the superfluid dominates the observed dynamics. Molecular rotation, induced by short laser pulses, offer a suitable probe to reach rotational energies in the range of the roton gap, where superfluid helium supports a large number of elementary excitations. However, the solvation shell around a rotating molecule caps the energy reachable by a free rotor after impulsive excitation well below the roton excitation energy. Here we show that continuous driving with an ultraslow optical centrifuge overcomes this limitation: the strong field dresses the molecule into pendular states whose energies fall within the spectrum of the collective excitations of the superfluid, placing the system in the strong-dissipation regime. The resulting rapid thermalization locks the molecule to the rotating field until the rotation-induced level splittings overtake the thermalization rate, beyond which the molecular alignment is progressively lost. Our approach offers a direct measurement of the molecule-bath coupling in a quantum fluid.

quant-pharXiv:2608.25161Aug 27, 20260 citations

Onset of nanoscale dissipation in superfluid He4 at zero temperature: Role of vortex shedding and cavitation

Francesco Ancilotto, M. Barranco, Jussi Eloranta +1 more

Two-dimensional flow past an infinitely long cylinder of nanoscopic radius in superfluid $^{4}\mathrm{He}$ at zero temperature is studied using time-dependent density-functional theory. The calculations reveal two distinct critical phenomena for the onset of dissipation: (i) vortex-antivortex pair shedding from the periphery of the moving cylinder, and (ii) the appearance of cavitation in the wake, which possesses similar geometry to that observed experimentally for fast-moving micrometer-scale particles in superfluid $^{4}\mathrm{He}$ . The formation of cavitation bubbles behind the cylinder is accompanied by a sudden jump in the drag exerted on the moving cylinder by the fluid. Vortex pairs with the same circulation are occasionally emitted in the form of dimers, which constitute the building blocks for the Benard--von Karman vortex street structure observed in classical turbulent fluids and Bose-Einstein condensates. The cavitation-induced dissipation mechanism should be common to all superfluids that are self-bound and have a finite surface tension, which include the recently discovered self-bound droplets in ultracold Bose gases. These systems would provide an ideal testing ground for further exploration of this mechanism experimentally.Two-dimensional flow past an infinitely long cylinder of nanoscopic radius in superfluid $^{4}\mathrm{He}$ at zero temperature is studied using time-dependent density-functional theory. The calculations reveal two distinct critical phenomena for the onset of dissipation: (i) vortex-antivortex pair shedding from the periphery of the moving cylinder, and (ii) the appearance of cavitation in the wake, which possesses similar geometry to that observed experimentally for fast-moving micrometer-scale particles in superfluid $^{4}\mathrm{He}$. The formation of cavitation bubbles behind the cylinder is accompanied by a sudden jump in the drag exerted on the moving cylinder by the fluid. Vortex pairs with the same circulation are occasionally emitted in the form of dimers, which constitute the building blocks for the Benard--von Karman vortex street structure observed in classical turbulent fluids and Bose-Einstein condensates. The cavitation-induced dissipation mechanism should be common to all superfluids that are self-bound and have a finite surface tension, which include the recently discovered self-bound droplets in ultracold Bose gases. These systems would provide an ideal testing ground for further exploration of this mechanism experimentally.

arXiv:1705.03236Physical review. B./Physical review. BAug 2, 20179 citations

Critical velocity and dissipation mechanism in finite superfluid

^4

He nanodroplets

Two-dimensional flow past an infinitely long cylinder of nanoscopic radius in superfluid

^{4}\mathrm{He}

at zero temperature is studied using time-dependent density-functional theory. The calculations reveal two distinct critical phenomena for the onset of dissipation: (i) vortex-antivortex pair shedding from the periphery of the moving cylinder, and (ii) the appearance of cavitation in the wake, which possesses similar geometry to that observed experimentally for fast-moving micrometer-scale particles in superfluid

^{4}\mathrm{He}

. The formation of cavitation bubbles behind the cylinder is accompanied by a sudden jump in the drag exerted on the moving cylinder by the fluid. Vortex pairs with the same circulation are occasionally emitted in the form of dimers, which constitute the building blocks for the Benard--von Karman vortex street structure observed in classical turbulent fluids and Bose-Einstein condensates. The cavitation-induced dissipation mechanism should be common to all superfluids that are self-bound and have a finite surface tension, which include the recently discovered self-bound droplets in ultracold Bose gases. These systems would provide an ideal testing ground for further exploration of this mechanism experimentally.