We experimentally demonstrate the importance of two-photon symmetry for the propagation of spatial quantum correlations in a multiple-scattering disordered system. Two distinguishable entangled photons with tunable spatial exchange symmetry are sent through the scattering medium. The two photons are observed to have an ensemble-averaged tendency to cluster together (bosonic symmetry) or to avoid each other (fermionic symmetry). An intermediate degree of clustering is observed for anyonic exchange symmetry.
We experimentally demonstrate the importance of two-photon symmetry for the propagation of spatial quantum correlations in a multiple-scattering disordered system. Two distinguishable entangled photons with tunable spatial exchange symmetry are sent through the scattering medium. The two photons are observed to have an ensemble-averaged tendency to cluster together (bosonic symmetry) or to avoid each other (fermionic symmetry). An intermediate degree of clustering is observed for anyonic exchange symmetry.
This dissertation contains scientific research within the realm of quantum optics, which is a branch of physics. An experimental and theoretical study is made of two-photon interference phenomena in various optical systems. Spatially entangled photon pairs are produced via the nonlinear optical process of spontaneous parametric down-conversion. These entangled photons are then passed through different optical systems to study various aspects of two-photon interference. Firstly, an experimental analysis is made of the high-dimensional entanglement that is present in the orbital angular momentum of the photons. Secondly, we present a comprehensive description of two-photon quantum interference behind a double slit. We demonstrate how to control the quantum correlations and present the first observations of complete two-photon diffraction patterns behind a double slit. Finally, we present pioneering experiments on spatially entangled two-photon states that are scattered of random media. We have observed and theoretically analyzed the structure in the random two-photon interference patterns called two-photon speckle patterns. Spatial entanglement gives two-photon speckle a much richer structure than ordinary one-photon speckle. Our experiments also demonstrate a two-photon interference phenomenon that survives averaging over different realizations of disorder. The latter results are closely related to bosonic, fermionic, and anyonic particle exchange symmetries.
Photons are bosons, and yet, when prepared in specific entangled states, they can exhibit non-bosonic behaviour. While this phenomenon has so far been studied in two-photon systems, exchange symmetries and interference effects in multi-photon scenarios remain largely unexplored. In this work, we show that multi-photon states uncover a rich landscape of exchange symmetries. With three photons already, multiple pairwise combinations are possible, where each pair of photons can exhibit either bosonic, fermionic, or anyonic exchange symmetry. This gives rise to mixed symmetry systems that are not possible to achieve with two photon alone. We experimentally investigate how these symmetry configurations manifest themselves in the observed interference of three photons. We show that multi-photon interference can be effectively turned on and off by tuning the symmetry of the constituent pairs. The possibility of accessing and tuning new quantum statistics in a scalable photonic platform not only deepens our understanding of quantum systems, but is also highly relevant for quantum technologies that rely on quantum interference.
We present the experimental realization of spatial quantum correlations of photons that are induced by multiple scattering of squeezed light. The quantum correlation relates photons propagating along two different light paths through the random medium and is infinite in range. Both positive and negative spatial quantum correlations are observed when varying the quantum state incident to the multiple scattering medium, and the strength of the correlations is controlled by the number of photons. The experimental results are in excellent agreement with recent theoretical proposals by implementing the full quantum model of multiple scattering.
We report the observation of speckle patterns in quantum correlations within light that is scattered by a disordered medium. The random medium is illuminated with spatially entangled photon pairs, and fourth-order speckle patterns are spatially resolved by two independently scanning detectors. Spatial entanglement gives two-photon speckle a much richer structure than ordinary one-photon speckle. Our experiments demonstrate that two-photon speckle from a surface scatterer and a volume scatterer look entirely different.
Understanding the complex interactions of the quantum light with different media provides valuable insights into potential applications in quantum tomography, microscopy, circuit and network design, and imaging. This thesis investigates quantum light interaction with two types of media: I. Random media entailing multiple scattering (Chapters 2-5), and II. Structured media, specifically designed to control quantum interferences (Chapters 6 and 7). In the first part of the thesis, and through solving the Lippmann-Schwinger equation for collections of small scatterers, a first principle scalar model for multiple scattering in finite-sized random media is developed. This efficient numerical model serves as the basis for investigating the coherent backscattering, a manifestation of weak localization in random media, for several bounded random media and various illuminations. Through employing mode expansion, next, the developed model is adapted to a general class of quantum-optical studies and quantum correlations are successfully derived and analyzed in scattering from finite disordered structures as well as systems of few scatterers. In multiple scattering of two-photon states in weak localization regime, the emergence of coherent two-photon backscattering is presented for the first time in coincidence detection, and it is demonstrated that quantum correlations can be used as a probe of entanglement dimensionality. Multiple scattering of two-photon states results in granular patterns known as speckle patterns. The statistical properties of single- and two-photon speckle patterns in scattering of different states are numerically calculated and the speckle visibilities and relevant parameters are derived. Specifically, the deviation of the probability density functions from negative exponential distributions, traditionally recognized as Rayleigh statistics in classical scattering, is identified, and shown to significantly depend on the presence of entanglement. Lastly, a different numerical implementation (based on COMSOL Multiphysics package) is used to consolidate our findings by incorporating the polarization effects. Coherent backscattering and coherent two-photon backscattering are observed for co-polarized fields in scattering from synthesized disordered media. It is demonstrated that depending on the particle exchange symmetry in polarization entangled excitation, the photons can exhibit statistical tendency to bunch together in the same mode, appear in separate modes (antibunching), or show a mixed response after multiple scattering. These bosonic-, fermionic-, and anyonic-like behaviors are studied in connection with coherent backscattering phenomenon, and it is demonstrated that the degree of enhancement in backscattering depends on the exchange symmetries. The simplicity and effectiveness of the implemented scattering analysis and the significance of the consequent conclusions suggest our approach as a promising platform for ‘numerical experiments’ without the limitations of analytical or semi-analytical models, and a practical tool prior to experiments. In the second part of the thesis, the random media operating as multimode platforms are replaced with engineered surfaces, i.e., metasurfaces, to realize targeted quantum interferences. First, a design roadmap for general lossy, asymmetric, and unbalanced coupling networks is presented, allowing to achieve maximum programmability in two-photon interferences. Next, two switchable metasurface-based coupling networks are designed to control nonclassical two-photon interferences via thermally driven crystallographic phase transitions. Numerical simulations confirm smooth transition between coalescence and anti-coalescence, aiming to address the current need in quantum optics for free-space compact devices creating tunable quantum interferences and acting as fast modulators for the second order quantum correlations. Our proposed compact and rapidly controllable devices pave the way towards new quantum applications as well as improving the current free-space quantum systems.
Quantum mechanics defines two classes of particles-bosons and fermions-whose exchange statistics fundamentally dictate quantum dynamics. Here we develop a scheme that uses entanglement to directly observe the correlated detection statistics of any number of fermions in any physical process. This approach relies on sending each of the entangled particles through identical copies of the process and by controlling a single phase parameter in the entangled state, the correlated detection statistics can be continuously tuned between bosonic and fermionic statistics. We implement this scheme via two entangled photons shared across the polarisation modes of a single photonic chip to directly mimic the fermion, boson and intermediate behaviour of two-particles undergoing a continuous time quantum walk. The ability to simulate fermions with photons is likely to have applications for verifying boson scattering and for observing particle correlations in analogue simulation using any physical platform that can prepare the entangled state prescribed here.