Strongly coupled quantum dot-cavity systems provide a non-linear configuration of hybridized light-matter states with promising quantum-optical applications. Here, we investigate the coherent interaction between strong laser pulses and quantum dot-cavity polaritons. Resonant excitation of polaritonic states and their interaction with phonons allow us to observe coherent Rabi oscillations and Ramsey fringes. Furthermore, we demonstrate complete coherent control of a quantum dot-photonic crystal cavity based quantum-bit. By controlling the excitation power and phase in a two-pulse excitation scheme we achieve access to the full Bloch sphere. Quantum-optical simulations are in good agreement with our experiments and provide insight into the decoherence mechanisms.
Strongly coupled quantum dot-cavity systems provide a non-linear configuration of hybridized light-matter states with promising quantum-optical applications. Here, we investigate the coherent interaction between strong laser pulses and quantum dot-cavity polaritons. Resonant excitation of polaritonic states and their interaction with phonons allow us to observe coherent Rabi oscillations and Ramsey fringes. Furthermore, we demonstrate complete coherent control of a quantum dot-photonic crystal cavity based quantum-bit. By controlling the excitation power and phase in a two-pulse excitation scheme we achieve access to the full Bloch sphere. Quantum-optical simulations are in good agreement with our experiments and provide insight into the decoherence mechanisms.
We use the third- and fourth-order autocorrelation functions ${g}^{(3)}({\ensuremath{\tau}}_{1},{\ensuremath{\tau}}_{2})$ and ${g}^{(4)}({\ensuremath{\tau}}_{1},{\ensuremath{\tau}}_{2},{\ensuremath{\tau}}_{3})$ to detect the nonclassical character of the light transmitted through a photonic-crystal nanocavity containing a strongly coupled quantum dot probed with a train of coherent light pulses. We contrast the value of
g(3)(0,0) with the conventionally used
g(2)(0) and demonstrate that, in addition to being necessary for detecting two-photon states emitted by a low-intensity source,
g(3) provides a more clear indication of the nonclassical character of a light source. We also present preliminary data that demonstrates bunching in the fourth-order autocorrelation function ${g}^{(4)}({\ensuremath{\tau}}_{1},{\ensuremath{\tau}}_{2},{\ensuremath{\tau}}_{3})$ as the first step toward detecting three-photon states.