We discuss the use of asymptotic-in and -out fields in a Hamiltonian treatment of nonlinear electromagnetic problems. Our approach allows a description of nonlinear phenomena in a number of geometries and is suitable to treat integrated photonic structures, particularly cavities. We present examples in which the nonlinear phenomena are weak enough for pump depletion to be neglected, and we report some results related to the description of second-order nonlinear processes in ring resonators and layered structures.
We discuss the use of asymptotic-in and -out fields in a Hamiltonian treatment of nonlinear electromagnetic problems. Our approach allows a description of nonlinear phenomena in a number of geometries and is suitable to treat integrated photonic structures, particularly cavities. We present examples in which the nonlinear phenomena are weak enough for pump depletion to be neglected, and we report some results related to the description of second-order nonlinear processes in ring resonators and layered structures.
We present two complementary strategies for modeling nonlinear quantum optics in realistic integrated optical devices, where scattering loss is present. In the first strategy, we model scattering loss as an attenuation; in the second, we employ a Hamiltonian treatment that includes a mechanism for scattering loss, such as a phantom waveguide. These strategies can be applied to a broad range of structures and processes. As an example, we use these two approaches to model spontaneous four-wave mixing in (i) a ring-channel system and (ii) an add-drop system. Even for these well-understood systems, our strategies yield some additional results. We show the rates of photon pairs, broken pairs, and lost pairs and their dependence on system parameters. We show that the properties of lost and broken photon pairs in such structures can be related to those of the unscattered photon pairs, which are relatively simple to measure.
The generation of engineered quantum states of light via nonlinear processes is fundamental for quantum technologies based on photons. Although embedding nonlinear materials within resonant structures allows for the enhancement and tailoring of photon properties, accurately modeling these quantum interactions remains a challenge. In this work, we apply the asymptotic-fields formalism, an approach based on scattering theory, to describe nonlinear optical processes within a Fabry-Pérot cavity. Unlike previous applications of this formalism, we explicitly account for reflections in the system. We derive the interaction Hamiltonian and calculate photon-pair generation rates using perturbation theory. The versatility of this model is illustrated through three examples: (i) spontaneous parametric down-conversion in an idealized cavity with flat-response mirrors; (ii) the generation of counter-propagating photon pairs in a periodically-poled material; and (iii) spontaneous four-wave mixing in a cavity built with Bragg reflectors.
In earlier chapters we have considered in detail the susceptibility formalism of nonlinear optics, which is perhaps the most familiar approach and has a wide range of application. Starting from the constitutive relations of Chapter 2, the susceptibility formalism is quite general. In many practical applications, a particular phenomenon can be described accurately by a single order of nonlinearity, and the susceptibility then provides a useful and convenient description. However, this is not always the case. Some of the most interesting phenomena in nonlinear optics involve close resonance with the transition frequencies of the medium, and perhaps also the use of very intense optical fields. As remarked in §4.5, in these circumstances the resonant susceptibilities display mathematical divergences which are clearly unphysical. Strictly, these divergences occur only because higher-order nonlinearities have been neglected. Successive orders of nonlinearity take into account such effects as saturation, power broadening and level shifts (optical Stark effect). For intense fields or very close resonance, the contributions from several orders of nonlinearity may be comparable in magnitude. Therefore, despite its generality, the susceptibility formalism does not necessarily provide the most practical approach for the description of resonant processes. This chapter is concerned with the problem of deriving alternative and more manageable descriptions of resonant nonlinear processes, illustrated by examples. For much of the chapter, the nonlinear medium is treated as a two-level system (described in §6.2).
Photonic integrated circuits with second-order (χ(2)) nonlinearities are rapidly scaling to remarkably low powers. At this time, state-of-the-art devices achieve saturated nonlinear interactions with thousands of photons when driven by continuous-wave lasers, and further reductions in these energy requirements enabled by the use of ultrafast pulses may soon push nonlinear optics into the realm of single-photon nonlinearities. This tutorial reviews these recent developments in ultrafast nonlinear photonics, discusses design strategies for realizing few-photon nonlinear interactions, and presents a unified treatment of ultrafast quantum nonlinear optics using a framework that smoothly interpolates from classical behaviors to the few-photon scale. These emerging platforms for quantum optics fundamentally differ from typical realizations in cavity quantum electrodynamics due to the large number of coupled optical modes. Classically, multimode behaviors have been well studied in nonlinear optics, with famous examples including soliton formation and supercontinuum generation. In contrast, multimode quantum systems exhibit a far greater variety of behaviors, and yet closed-form solutions are even sparser than their classical counterparts. In developing a framework for ultrafast quantum optics, we will identify what behaviors carry over from classical to quantum devices, what intuition must be abandoned, and what new opportunities exist at the intersection of ultrafast and quantum nonlinear optics. While this article focuses on establishing connections between the classical and quantum behaviors of devices with χ(2) nonlinearities, the frameworks developed here are general and are readily extended to the description of dynamical processes based on third-order (χ(3)) nonlinearities.
Photonic integrated circuits with second-order ( χ (2) ) nonlinearities are rapidly scaling to remarkably low powers. At this time, state-of-the-art devices achieve saturated nonlinear interactions with thousands of photons when driven by continuous-wave lasers, and further reductions in these energy requirements enabled by the use of ultrafast pulses may soon push nonlinear optics into the realm of single-photon nonlinearities. This tutorial reviews these recent developments in ultrafast nonlinear photonics, discusses design strategies for realizing few-photon nonlinear interactions, and presents a unified treatment of ultrafast quantum nonlinear optics using a framework that smoothly interpolates from classical behaviors to the few-photon scale. These emerging platforms for quantum optics fundamentally differ from typical realizations in cavity quantum electrodynamics due to the large number of coupled optical modes. Classically, multimode behaviors have been well studied in nonlinear optics, with famous examples including soliton formation and supercontinuum generation. In contrast, multimode quantum systems exhibit a far greater variety of behaviors, and yet closed-form solutions are even sparser than their classical counterparts. In developing a framework for ultrafast quantum optics, we identify what behaviors carry over from classical to quantum devices, what intuition must be abandoned, and what new opportunities exist at the intersection of ultrafast and quantum nonlinear optics. Although this article focuses on establishing connections between the classical and quantum behaviors of devices with χ (2) nonlinearities, the frameworks developed here are general and are readily extended to the description of dynamical processes based on third-order χ (3) nonlinearities.
In Chapter 1, we treated the electromagnetic field as classical. Henceforth, we will want to treat it as a quantum field. In order to do so, we will first present some of the formalism of quantum field theory. This formalism is very useful in describing many-particle systems and processes in which the number of particles changes. Why this is important to a quantum description of nonlinear optics can be seen by considering a parametric amplifier of the type discussed in the last chapter. A pump field, consisting of many photons, amplifies idler and signal fields by means of a process in which a pump photon splits into two lower-energy photons, one at the idler frequency and one at the signal frequency. Therefore, what we would like to do in this chapter is to provide a discussion of some of the basics of quantum field theory that will be useful in the treatment of the quantization of the electromagnetic field. In particular, we will begin with a summary of quantum theory notation, and a discussion of many-particle Hilbert spaces. These provide the arena in which all of the action takes place. We will then move on to a treatment of the canonical quantization procedure for fields. This will allow us to develop a scattering theory for fields, which is ideally what we need. This relates the properties of a field entering a medium to those of the field leaving it, and this corresponds to what is done in an experiment.