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Physical Review B

Two-photon interference from remote quantum dots with inhomogeneously broadened linewidths

P. Gold, A. Thoma, Stefan Alexander Maier, Stephan Reitzenstein, Christian Schneider, Sven Höfling, Martin Kamp

Published Jan 27, 2014• 70 citations
Publisher

Abstract

In this paper, we study the influence of quasiresonant and nonresonant excitation on the interference properties of single photons emitted from quantum dots (QDs). The quasiresonant excitation scheme leads to an increase of interference visibility of photons emitted from the same QD to 69% compared to 12% for nonresonant excitation. Furthermore, we demonstrate quantum interference of photons emitted from separate QDs which are simultaneously excited into their $p$ shell. We can readily extract a two-photon interference visibility as high as (39 \ifmmode\pm\else\textpm\fi{} 2)% for nonpostselected coincidences exceeding the predicted value based on coherence and radiative decay times of the quantum dot emission ($\ensuremath{\sim}$25%). We account for this observation by treating the emission of both quantum dots as inhomogeneously broadened ensembles of Fourier-limited photons and observe good congruence between experiment and model.

DOI
10.1103/physrevb.89.035313

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•May 13, 2012•0 citations
In this paper, we study the influence of quasiresonant and nonresonant excitation on the interference properties of single photons emitted from quantum dots (QDs). The quasiresonant excitation scheme leads to an increase of interference visibility of photons emitted from the same QD to 69% compared to 12% for nonresonant excitation. Furthermore, we demonstrate quantum interference of photons emitted from separate QDs which are simultaneously excited into their ppp shell. We can readily extract a two-photon interference visibility as high as (39 \ifmmode\pm\else\textpm\fi{} 2)% for nonpostselected coincidences exceeding the predicted value based on coherence and radiative decay times of the quantum dot emission (\ensuremath∼\ensuremath{\sim}\ensuremath∼25%). We account for this observation by treating the emission of both quantum dots as inhomogeneously broadened ensembles of Fourier-limited photons and observe good congruence between experiment and model.
We report on two-photon interference of highly indistinguishable single photons emitted by a quantum dot. Strictly resonant excitation with picosecond laser pulses has been used to prepare coherent states with a significantly increased coherence time $({T}_{2}\ensuremath{\sim}1\text{ns})$ and reduced lifetime $({T}_{1}\ensuremath{\sim}650\text{ps})$, as compared to a nonresonant excitation scheme. Indistinguishable photons, with visibilities greater than 70%, have been observed by measuring the Hong-Ou-Mandel dip without postselection of the interfering photons. Near-unity indistinguishable photons should be achievable by preventing fluctuations in the electrostatic environment in the vicinity of the dots, considered as an important source of decoherence.
The visibility of two-photon interference is limited by the indistinguishability of the photons. In the cascaded emission of a three-level system, such as a single quantum dot, the indistinguishability of each photon in the pair is primarily affected by two main factors: the temporal correlation between paired photons and dephasing. Investigating the individual effects of these factors on photon indistinguishability is challenging, as both factors affect it simultaneously. In this study, we investigate the temperature-dependent two-photon interference visibility of the biexciton and exciton photons emitted from a single quantum dot under two-photon resonant excitation, while keeping the temporal correlation between the paired photons intact. Finally, we simultaneously extract the coherence times of the biexciton and exciton photons as a function of temperature.
Abstract In the quest to realize a scalable quantum network, semiconductor quantum dots (QDs) offer distinct advantages including high single-photon efficiency and indistinguishability, high repetition rate (tens of GHz with Purcell enhancement), interconnectivity with spin qubits, and a scalable on-chip platform. However, in the past two decades, the visibility of quantum interference between independent QDs rarely went beyond the classical limit of 50% and the distances were limited from a few meters to kilometers. Here, we report quantum interference between two single photons from independent QDs separated by 302 km optical fiber. The single photons are generated from resonantly driven single QDs deterministically coupled to microcavities. Quantum frequency conversions are used to eliminate the QD inhomogeneity and shift the emission wavelength to the telecommunication band. The observed interference visibility is 0.67\pm0.02 (0.93\pm0.04) without (with) temporal filtering. Feasible improvements can further extend the distance to ~600 km. Our work represents a key step to long-distance solid-state quantum networks.
In the quest to realize a scalable quantum network, semiconductor quantum dots (QDs) offer distinct advantages, including high single-photon efficiency and indistinguishability, high repetition rate (tens of gigahertz with Purcell enhancement), interconnectivity with spin qubits, and a scalable on-chip platform. However, in the past two decades, the visibility of quantum interference between independent QDs rarely went beyond the classical limit of 50%, and the distances were limited from a few meters to kilometers. Here, we report quantum interference between two single photons from independent QDs separated by a 302 km optical fiber. The single photons are generated from resonantly driven single QDs deterministically coupled to microcavities. Quantum frequency conversions are used to eliminate the QD inhomogeneity and shift the emission wavelength to the telecommunication band. The observed interference visibility is 0.67 ± 0.02 (0.93 ± 0.04) without (with) temporal filtering. Feasible improvements can further extend the distance to ∼600 km. Our work represents a key step to long-distance solid-state quantum networks.
Single photon emission is one of the most striking optical properties of semiconductor quantum dots (QDs), and the corresponding photon anti-bunching effect was observed by non-resonant and resonant photoluminescence experiments in single QDs [1,2]. Up to now, all the measurements reported in the literature focus on the incoherent photoluminescence signal for achieving single photon emission. In this regime, the linewidth of the photoluminescence spectrum is limited to the so-called radiative limit. In this paper, we report on the resonant emission (RE) of the exciton in single InAs/GaAs QDs embedded in a planar microcavity [2]. We present an original type of single photon source based on the coherent laser light scattering by a single QD [3]. Besides the antibunching effect showing the nonclassical nature of the emitted light, we observe that the QD emission spectrum is determined by the spectrum of the resonant excitation laser. Figure (a,b,c) shows high-resolution measurements by Fourier transform spectroscopy of the RE where the data are fitted to the first-order correlation function g(1)(τ) of the RE of a two-level system. The inverse Fourier transform of the g(1)(τ) function allows a direct comparison of the different RE emission profiles in figure (d,e,f). By reducing the resonant excitation power, the Mollow triplet shrinks to a single narrow Lorentzian line, while the relative intensity of this narrow peak increases and tends to overwhelm the RE spectrum. This implies that single QDs can produce single photons with a coherence time that is not limited anymore by the QD electronic properties, resulting in an ultra-coherent character [3]. References [1] P. Michler et al, Science 290, 2282 (2000). [2] H. S. Nguyen et al, Phys. Rev. Lett. (accepted, in press). See arXiv 1109.4304. [3] H. S. Nguyen et al, Appl. Phys. Lett. 99, 261904 (2011).