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Physical Review A

Enhanced optical nonlinearity and fiber-optical frequency comb controlled by a single atom in a whispering-gallery-mode microtoroid resonator

Jiahua Li, Suzhen Zhang, Rong Yu, Duo Zhang, Ying Wu

Published Nov 17, 2014• 33 citations
Publisher

Abstract

Based on a single atom coupled to a fiber-coupled, chip-based microresonator [B. Dayan et al., Science 319, 1062 (2008)], we put forward a scheme to generate optical frequency combs at driving laser powers as low as a few nanowatts. Using state-of-the-art experimental parameters, we investigate in detail the influences of different atomic positions and taper-resonator coupling regimes on optical-frequency-comb generation. In addition to numerical simulations demonstrating this effect, a physical explanation of the underlying mechanism is presented. We find that the combination of the atom and the resonator can induce a large third-order nonlinearity which is significantly stronger than Kerr nonlinearity in Kerr frequency combs. Such enhanced nonlinearity can be used to generate optical frequency combs if driven with two continuous-wave control and probe lasers and significantly reduce the threshold of nonlinear optical processes. The comb spacing can be well tuned by changing the frequency beating between the driving control and probe lasers. The proposed method is versatile and can be adopted to different types of resonators, such as microdisks, microspheres, microtoroids or microrings.

DOI
10.1103/physreva.90.053832

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Based on a single atom coupled to a fiber-coupled, chip-based microresonator [B. Dayan et al., Science 319, 1062 (2008)], we put forward a scheme to generate optical frequency combs at driving laser powers as low as a few nanowatts. Using state-of-the-art experimental parameters, we investigate in detail the influences of different atomic positions and taper-resonator coupling regimes on optical-frequency-comb generation. In addition to numerical simulations demonstrating this effect, a physical explanation of the underlying mechanism is presented. We find that the combination of the atom and the resonator can induce a large third-order nonlinearity which is significantly stronger than Kerr nonlinearity in Kerr frequency combs. Such enhanced nonlinearity can be used to generate optical frequency combs if driven with two continuous-wave control and probe lasers and significantly reduce the threshold of nonlinear optical processes. The comb spacing can be well tuned by changing the frequency beating between the driving control and probe lasers. The proposed method is versatile and can be adopted to different types of resonators, such as microdisks, microspheres, microtoroids or microrings.
Optical microresonators can greatly enhance light-matter interactions and reduce the power necessary to observe nonlinear optical effects. Manipulation and application of atom-resonator-coupling-induced strong nonlinearity have received much attention in recent years. Here, we present a scheme to realize quantum-squeezing-engineered third-order Kerr nonlinearity and optical high-order sideband comb in a composite system consisting of a two-level atom and two directly coupled whispering-gallery-mode optical microresonators. By quantum squeezing one of two coupled resonator modes in this system, the effective resonator-resonator and atom-resonator coupling rates as well as the frequency of the squeezed resonator mode can be effectively controlled. Based on this mechanism, we show that the Kerr nonlinearity of the composite system can be effectively engineered by using the resonator-mode squeezing when the system is monochromatically driven beyond the weak-excitation limit. On the other hand, when the composite system is bichromatically driven, the optical high-order sideband combs formed in the transmission spectra of the system can also be effectively engineered by the resonator-mode squeezing. Therefore, our scheme provides a novel mechanism to control the physical properties of composite resonator-atom systems for various applications, and demonstrates that optical nonlinear effects induced by the atom-resonator coupling can be effectively engineered via quantum squeezing.
A dielectric microsphere may be considered as an artificial photonic atom. The electromagnetic modes in the microsphere are completely assigned with indexes similar to those used to characterize simple atomic systems. Microsphere modes, as well as microring or microdisk, trap light in circular orbits near the sphere surface and strongly modify the phase of the interacting light, resulting in very steep dispersions. Pulse propagation experiments were performed in a system consisting of a fiber taper coupled with a silica glass microsphere, and it was shown that the light velocity in the system can be largely changed through the control of the coupling strength. Slow light was also demonstrated in a system in which two ultrahigh-Q silica microspheres of different diameters were coupled in tandem to a fiber taper demonstrating classical analog of electromagnetically induced transparency in atomic system. Here, we employed interferometric techniques based on the Mach-Zehnder interferometer for examining extremely steep dispersions induced by whispering gallery modes with a quality factor on the order of Q 1⁄4 10. Such a narrow resonance in the dielectric microsphere is comparable to that in cooled atomic systems. We successfully observed both normal and anomalous dispersions at the resonant frequency, depending on the coupling strength between the sphere and the fiber. Figure 1 shows our experimental system based on an interferometric setup. We used the second harmonics of a single mode ring cavity Nd3þ yttrium aluminum garnet (Nd3þ:YAG) laser with a line width of 1 kHz at 532 nm. The laser frequency was tuned using thermal control of the ring cavity length, over a mode-hop-free range of greater than 10GHz. The reference arm was empty, while the sample arm contained the microsphere-fiber system. Silica microspheres were fabricated from standard telecommunication optical fiber. The end of the etched fiber was fused using a CO2 laser and the microsphere formed due to the surface tension. The experiments were performed with a microsphere 60 mm in diameter. The fiber taper was also fabricated from the same telecommunication fiber. The typical fiber waist diameter at the coupling region was 0.5 mm. A large number of spectrally overlapping resonance modes exist within a microsphere. The fiber taper method is essential for coupling the incident light to a specific whispering gallery mode selectively and efficiently. The microsphere was attached to a translation stage controlled by a piezo actuator. The relative position between the sphere and the fiber were carefully adjusted so that we could observe spectrally isolated whispering gallery modes with proper coupling strength. The optical path length and dispersion were equalized in each arm as completely as possible. The fringe pattern was captured using a charge-coupled device (CCD) camera for each frequency increment. The observed interference patterns appeared as concentric circles due to the interference between the plain reference wave and the spherical wave from the sample arm. A least square fit for each fringe pattern was performed to extract the phase information in the transmitted light. Figures 2(a) and 2(b) show examples of transmission spectra through the microsphere fiber taper coupled system. These spectra were taken in two different whispering gallery modes at different laser frequencies in the mode-hop-free laser tuning range. The transmission dips appear when the incident laser frequencies are resonant at specific whispering gallery modes in the microsphere. The two whispering gallery modes shown in Figs. 2(a) and 2(b) are denoted as WG1 and WG2, respectively. The transmission minimum was Tmin 1⁄4 0:12, and the resonance width was 1⁄4 BS
We propose a scheme for single-atom, quantum control of the direction of propagation of a coherent field incident, via a tapered fiber, upon a microtoroidal whispering-gallery-mode (WGM) resonator. The scheme involves overcoupling of the fiber taper to the resonator and strong coupling of an atom to the evanescent field of the WGM, i.e., an atom-field coupling that exceeds the total WGM linewidth. In contrast to previous, related schemes that operate in the bad-cavity regime, the proposed scheme can operate effectively with much stronger incident fields, while also preserving their coherent nature. It can also serve to prepare an entangled state of the atom and coherent optical pulses propagating in opposite directions along the fiber. We evaluate the fidelity of preparation of such a state taking into account absorption and atomic spontaneous emission and demonstrate that high fidelities should be possible with realistic parameters.
Optical-frequency combs consisting of equally spaced sharp lines in frequency space have triggered substantial advances in optical-frequency metrology and precision measurements and in applications such as laser-based gas sensing and molecular fingerprinting. Here, we propose a scheme to generate a type of optical-frequency combs and convert them from one cavity to the other in a hybrid optical system composed of a pair of coupled photonic crystal cavities called a photonic molecule (PM) and a single semiconductor quantum dot (QD) embedded in one cavity of the molecule. Optical-frequency combs are formed by the interaction between a cavity mode and a continuous-wave (CW) two-tone driving laser consisting of a pump field and a seed field via QD-induced strong nonlinearity. In this situation, the initial input pump and seed CW lasers can interact among each other and produce optical higher-order sidebands with equal spacing via parametric frequency conversion provided by QD-induced nonlinear optical effects. Using numerical simulations, it is clearly shown that the beat frequency of the two-tone components plays an important role in determining the comb spacing and matched frequency combs can be formed in the PM. We also demonstrate that the present interacting QD-PM system can serve as a platform to generate large-scale quantum entanglement between two comb modes. The results obtained here may be useful for real experiments in a photonic crystal platform.
We report the demonstration of strong coupling between single Cesium atoms and a high-Q chip-based microresonator. Our toroidal microresonators are compact, Si chip-based whispering gallery mode resonators that confine light to small volumes with extremely low losses, and are manufactured in large numbers by standard lithographic techniques. Combined with the capability to couple efficiently light to and from these microresonators by a tapered optical fiber, toroidal microresonators offer a promising avenue towards scalable quantum networks. Experimentally, laser cooled Cs atoms are dropped onto a toroidal microresonator while a probe beam is critically coupled to the cavity mode. When an atom interacts with the cavity, it modifies the resonance spectrum of the cavity, leading to rejection of some of the probe light from the cavity, and thus to an increase in the output power. By observing such transit events while systematically detuning the cavity from the atomic resonance, we determine the maximal accessible single-photon Rabi frequency of Ω0/2π ≈ (100 ± 24) MHz. This value puts our system in the regime of strong coupling, being significantly larger than the dissipation rates in our system.
We manipulated the simulation and apparatus to generate the entangled quantum photons by the enhanced higher quality factor in waveguide of whispering gallery mode resonator in silica microsphere. As the several nonlinear optics effects have been validated in micro-disk (lithium niobate materials based), others micro-cavity (microfiber and micro ring on the chip) and second harmonic generation (SHG) on the surface of silica microsphere because of the characterization of enhanced higher quality factor Q and smaller volume mode in these resonator. However until now for the second third nonlinearity of spontaneous parametric down conversion (SPDC), third order nonlinearity of spontaneous parametric down conversion (TOSPDC) and spontaneous four wave mixing (SFWM) in whispering gallery mode (WGM) resonator of silica microsphere rarely have not been fully investigated and verified to generate the triple and pair entangled photons where are widely applied on the applications of biosensor, quantum communications and spectroscopy, respectively. Specially, the features of silica microsphere have attracted many applications due to the simple fabrication, simplified materials melted by silica fiber. The work we demonstrated in this paper based on the breaking of the dispersion rules to make perfect phase matching in normal dispersion in silica microsphere depending on the blue laser spectrum in visible spectrum, then manipulated the modified size of microsphere to detune the pump laser of free spectral range (FSR) and both shift the geometrical dispersion are characterized in the variation of FSR given by (see PDF for equation), where n is refractive index, R is the microspheres radius and m is mode numbers in resonator, to compensate the materials dispersion given by (see PDF for equation), where c is the speed of light and λ is pump laser wavelength to fulfill the perfect phase matching in parametric down conversion regimes and the modeling fabrication coupling results also will be presented.