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Physical Review A

Two-photon interferences with degenerate and nondegenerate paired photons

Chang Liu, J. F. Chen, Shanchao Zhang, Shuyu Zhou, Yoon-Ho Kim, M. M. T. Loy, George K. Wong, Shengwang Du

Published Feb 13, 2012• 36 citations
Publisher

Abstract

We generate narrow-band frequency-tunable entangled photon pairs from spontaneous four-wave mixing in three-level cold atoms and study their two-photon quantum interference after a beam splitter. We find that the path-exchange symmetry plays a more important role in the Hong-Ou-Mandel interference than the temporal or frequency indistinguishability, and observe coalescence interference for both degenerate and nondegenerate photons. We also observe a quantum beat in the same experimental setup using either slow or fast detectors.

DOI
10.1103/physreva.85.021803

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We generate narrow-band frequency-tunable entangled photon pairs from spontaneous four-wave mixing in three-level cold atoms and study their two-photon quantum interference after a beam splitter. We find that the path-exchange symmetry plays a more important role in the Hong-Ou-Mandel interference than the temporal or frequency indistinguishability, and observe coalescence interference for both degenerate and nondegenerate photons. We also observe a quantum beat in the same experimental setup using either slow or fast detectors.
The temporal purity of single photons is crucial to the indistinguishability of independent photon sources for the fundamental study of the quantum nature of light and the development of photonic technologies. Currently, the technique for single photons heralded from time-frequency entangled biphotons created in nonlinear crystals does not guarantee the temporal-quantum purity, except using spectral filtering. Nevertheless, an entirely different situation is anticipated for narrow-band biphotons with a coherence time far longer than the time resolution of a single-photon detector. Here we demonstrate temporally pure single photons with a coherence time of 100 ns, directly heralded from the time-frequency entangled biphotons generated by spontaneous four-wave mixing in cold atomic ensembles, without any supplemented filters or cavities. A near-perfect purity and indistinguishability are both verified through Hong-Ou-Mandel quantum interference using single photons from two independent cold atomic ensembles. The time-frequency entanglement provides a route to manipulate the pure temporal state of the single-photon source.
Hong-Ou-Mandel interference between independent sources is a fundamental primitive of many quantum communication and computation protocols. We present a study of the Hong-Ou-Mandel interference of single photons generated via two different physical processes by two independent atomic systems: scattering by a single atom, and parametric generation via four-wave mixing in a cloud of cold atoms. By controlling the coherence time and central frequency of the heralded single photons generated by four-wave mixing we observe quantum beat and a varying degree of interference.
We report on the study of two-photon interference in the frequency domain. Bell and Hong-Ou-Mandel experiments are investigated. These experiments involve the manipulation of photons in the frequency domain, using off-the-shelf telecommunication components such as electro-optic phase modulators and narrow-band frequency filters. In the first experiment, photon pairs entangled in frequency are created and separated. Each photon is then directed through an independent electro-optic phase modulator. Variation of the radio-frequency parameters of the modulation gives rise to a well-controlled Bessel-shape two-photon interference pattern in the frequency domain. This is efficiently measured with narrow-band frequency filters and superconducting single photon detectors. Experimental measurements exhibit high visibilities (over 99 percent both for net and raw visibilities) and allow the (theoretically proven) optimal violation of a Bell inequality for our setup (by more than 18 standard deviations). The second experiment is a Hong-Ou-Mandel experiment in the frequency domain. We show that a grating (spatial domain) or a phase modulator (temporal domain) can be seen as a frequency beam splitter. A broadband spectrum of photon pairs is divided into two interleaved frequency combs, each one used as an independent input to this acting beam splitter. A theoretical calculation shows clear photon anti-bunching behavior.
The interference of single photons from independent sources is an essential tool in quantum information processing. However, the interfering of photons with long temporal states in a time-resolved manner has rarely been studied. This is because without transmitting spectral filters or coupling to a cavity mode single photons generated in traditional nonlinear crystals suffer from a short temporal profile below 1 ns. With spectral correlation maintained in the biphotons generated from spontaneous four-wave mixing process in cold atom clouds, here we demonstrate the temporal interference of two frequency-tunable long photons from two independent cold atomic sources. We observe and analyze the interference of frequency-mismatched photons, where the phenomenon of the quantum beat at megahertz separation is displayed. Our paper provides more details for the quantum beat of two independent narrow-band single photons, which may find potential application in frequency-encoded photonic qubits in quantum information processing.
Two-photon interference effects arise because photons are indistinguishable particles. In the wellknown Hong-Ou-Mandel (HOM) effect, the transmission of two photons at a beam splitter interferes destructively with the reflection of both photons, requiring both photons to "bunch up" by leaving the beam splitter on the same side. Here, we show that the interference between locally propagating photons and photons exchanged by a mode swap can be implemented by post-selecting spatially separated photon outputs of a four-path interferometer. Even though the photons detected at spatially separated locations must have travelled along paths that never met up at the same beam splitter, the Hong-Ou-Mandel effect can be observed in correlations between the output ports that originate from the association of detection events with non-local output modes defined by the two single photon inputs. Local phase shifts can be used to map out non-classical correlations between the photons detected at different output locations, clarifying the role of linear optics in generating entanglement between spatially separated photons. Our work thus establishes a fundamental relation between multiphoton interference and entanglement, opening the door to new possibilities in optical quantum technologies.
We present experimental observations of a nonclassic and nonlocal interference effect with frequency-entangled photon pairs. We observed two-photon interference in a Hong–Ou–Mandel interferometer by monitoring the coincidence-counting rate as we varied the path-length difference or the relative time delay between two photons. The quantum-mechanical probabilities of joint detection by two detectors that respond to different frequency components exhibit differences that depend not only on the arrangement of the detector pairs but on the spectral filtering. The experimental results provide more understanding of two-photon entanglement and of the interference effects that arise from superposition of indistinguishable probability amplitudes.