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Frontiers in Optics

Strong coupling of propagating laser light to single emitters: from absorption to stimulated emission

Vahid Sandoghdar

Published Jan 1, 2009• 0 citations
Publisher

Abstract

The quest for further miniaturization of computers and the prospects of quantum information processing have motivated scientists to seek nonlinear and transistor functionalities in quantum mechanical building blocks such as atoms. However, all-optical nonlinear operation at the single emitter level has been deemed exceptionally challenging and only been considered in high-finesse microcavities or waveguides. In our laboratories, we have performed a number of experiments that investigate the very fundamental scenario where a single emitter interacts coherently with a freely propagating incident laser beam.

DOI
10.1364/ls.2009.lstud1

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The quest for further miniaturization of computers and the prospects of quantum information processing have motivated scientists to seek nonlinear and transistor functionalities in quantum mechanical building blocks such as atoms. However, all-optical nonlinear operation at the single emitter level has been deemed exceptionally challenging and only been considered in high-finesse microcavities or waveguides. In our laboratories, we have performed a number of experiments that investigate the very fundamental scenario where a single emitter interacts coherently with a freely propagating incident laser beam.
Quantum information processing systems and related technologies are likely to involve switching and amplification functions in ultrasmall objects such as nanotubes. In today's electronic devices the transistor performs these functions. A 'quantum age' equivalent of the conventional transistor would, ideally, use photons rather than electrons as information carriers because of their speed and robustness against decoherence. But robustness also stops them being easily controlled. Now a team from optETH and ETH in Zurich demonstrates the realization of a single-molecule optical transistor. In it, a single dye molecule coherently attenuates or amplifies a tightly focused laser beam, depending on the power of a second 'gating' beam. The transistor is the most fundamental building block in present-day technologies. For the purpose of quantum information processing schemes and for the development of a 'quantum computer', photons are attractive information carriers because of their speed and robustness against decoherence. However, their robustness also prevents them from being easily controlled; despite this, experiments now show the realization of a quantum optical transistor. The transistor is one of the most influential inventions of modern times and is ubiquitous in present-day technologies. In the continuing development of increasingly powerful computers as well as alternative technologies based on the prospects of quantum information processing, switching and amplification functionalities are being sought in ultrasmall objects, such as nanotubes, molecules or atoms1,2,3,4,5,6,7,8,9. Among the possible choices of signal carriers, photons are particularly attractive because of their robustness against decoherence, but their control at the nanometre scale poses a significant challenge as conventional nonlinear materials become ineffective. To remedy this shortcoming, resonances in optical emitters can be exploited, and atomic ensembles have been successfully used to mediate weak light beams7. However, single-emitter manipulation of photonic signals has remained elusive and has only been studied in high-finesse microcavities10,11,12,13 or waveguides8,14. Here we demonstrate that a single dye molecule can operate as an optical transistor and coherently attenuate or amplify a tightly focused laser beam, depending on the power of a second ‘gating’ beam that controls the degree of population inversion. Such a quantum optical transistor has also the potential for manipulating non-classical light fields down to the single-photon level. We discuss some of the hurdles along the road towards practical implementations, and their possible solutions.
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