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Physical Review A

Exotic fluorescence spectrum of a superconducting qubit driven simultaneously by longitudinal and transversal fields

Yiying Yan, Zhiguo Lü, Hang Zheng, Yang Zhao

Published Mar 7, 2016• 13 citations
Publisher

Abstract

We study the fluorescence spectrum from a two-level system with a controllable energy separation modulated by the longitudinal field and excited by the transversal field. Combining the rotating-wave approximation and the Floquet theory, we derive a formal solution to the Bloch equations in the presence of both longitudinal and transversal driving fields and numerically evaluate the fluorescence spectrum. Exotic spectral features associated with the added longitudinal driving are found to be dramatically different from the standard Mollow triplet with a multipeak structure. The spectrum may be experimentally realized in the context of artificial atoms in a superconducing circuit.

DOI
10.1103/physreva.93.033812

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arXiv:2202.12080•Feb 24, 2022•1 citation
We study the fluorescence spectrum from a two-level system with a controllable energy separation modulated by the longitudinal field and excited by the transversal field. Combining the rotating-wave approximation and the Floquet theory, we derive a formal solution to the Bloch equations in the presence of both longitudinal and transversal driving fields and numerically evaluate the fluorescence spectrum. Exotic spectral features associated with the added longitudinal driving are found to be dramatically different from the standard Mollow triplet with a multipeak structure. The spectrum may be experimentally realized in the context of artificial atoms in a superconducing circuit.
We study the fluorescence spectrum of a strongly driven two-level system (TLS) with modulated transition frequency, which is a bichromatically driven TLS and has multiple resonance frequencies. We are aiming to provide a reliable description of the fluorescence in a regime that is difficult to tackle with perturbation theory and the rotating-wave approximation (RWA), and illustrate the spectral features of the fluorescence under off- and multiphoton-resonance conditions. To go beyond the RWA, we use a semianalytical counter-rotating-hybridized rotating-wave method that combines a unitary transformation and Floquet theory to calculate the two-mode Floquet states and quasienergies for the bichromatically driven TLS. We then solve the master equation accounting for the spontaneous decay in the bases of the two-mode Floquet states, and derive a physically transparent fluorescence spectrum. In comparison with the numerically exact spectrum from the generalized Floquet-Liouville approach, the present spectrum is found to be applicable in a wide range of the parameters where the RWA and the secular approximation may break down. We find that the counter-rotating (CR) terms of the transverse field omitted in the RWA have non-negligible contributions to the spectrum under certain conditions. Particularly, at the multiphoton resonance the width of which is comparable with the Bloch-Siegert shift, the RWA and non-RWA spectra markedly differ from each other because of the CR-induced shift. We also analyze the symmetry of the spectrum in terms of the transition matrix elements between the two-mode Floquet states. We show that the strict symmetry of the spectrum cannot be expected without the RWA but the almost symmetric spectrum can be obtained at the single-photon resonance that takes the Bloch-Siegert shift into account if the driving is moderately strong and at the multiphoton resonance with a sufficiently weak transverse field.
We investigate the fluorescence spectrum of a two-level system driven by a monochromatic classical field by the Born-Markovian master equation based on a unitary transformation. The main purpose is to understand the effects of counter-rotating-wave terms of the driving on spectral features of the fluorescence. We have derived an analytical expression for the fluorescence spectrum, which is different from Mollow's theory, while Mollow's result on resonance is the limiting case of ours in moderately weak driving regimes. Our results demonstrate precisely that the counter-rotating-wave terms of the driving play an important role in the fluorescence spectrum for intense driving: (i) the counter-rotating coupling suppresses the red sideband in the Mollow triplet and it enhances the blue one in explicitly contrast to the well-known equal intensity of the sideband in Mollow's theory, (ii) the higher-order Mollow triplets appear as a characteristic spectral feature arising from counter-rotating-wave terms of the driving, and (iii) a significant frequency shift of the sidebands is observed, which depends on both the detuning and driving strength.
We investigate the fluorescence spectrum of a two-level atom driven by a multiple amplitude-modulated field. The driving field is modeled as a polychromatic field composed of a strong central (resonant) component and a large number of symmetrically detuned sideband fields displaced from the central component by integer multiples of a constant detuning. Spectra obtained here differ qualitatively from those observed for a single pair of modulating fields [B. Blind, P.R. Fontana, and P. Thomann, J. Phys. B 13, 2717 (1980)]. In the case of a small number of the modulating fields, a multipeaked spectrum is obtained with the spectral features located at fixed frequencies that are independent of the number of modulating fields and their Rabi frequencies. As the number of the modulating fields increases, the spectrum ultimately evolves to the well-known Mollow triplet with the sidebands shifted from the central component by an effective Rabi frequency whose magnitude depends on the initial relative phases of the components of the driving field. For equal relative phases, the effective Rabi frequency of the driving field can be reduced to zero resulting in the disappearance of fluorescence spectrum, i.e., the atom can stop interacting with the field. When the central component and the modulating fields are $180\ifmmode^\circ\else\textdegree\fi{}$ out of phase, the spectrum retains its triplet structure with the sidebands located at frequencies equal to the sum of the Rabi frequencies of the component of the driving field. Moreover, we show that the frequency of spontaneous emission can be controlled and switched from one frequency to another when the Rabi frequency or initial phase of the modulating fields are varied.
We present an analytical and numerical Floquet treatment of a driven polar two-level quantum system characterized by both longitudinal and transverse coupling to a periodic field. Analytically, we derive a dressed-frame effective Hamiltonian up to first order in the inverse driving frequency, incorporating the longitudinal coupling nonperturbatively. This yields closed expressions for the effective transverse coupling strength and the effective detuning, both of which are modified by the presence of the longitudinal interaction. In the nonpolar limit, these expressions recover the usual near-resonant Rabi coupling and the Bloch-Siegert shift. As a second main result, we develop a numerical flow-equation framework that yields a time-independent effective Hamiltonian across a broad range of transverse and longitudinal coupling strengths. This dual framework is relevant for a variety of platforms, including driven polar quantum systems, optical lattices, superconducting circuits, and solids subject to surface acoustic waves.
Abstract Strong polychromatic driving reshapes characteristics of the resonance fluorescence spectrum of a two-level system. Employing bichromatic driving feild with a low beat-frequency smaller than the emission rate of the system we demonstrate the exotic features of the fluorescence spectrum calculated by the numerical Floquet-Liouville approach and analytical method. It is found that fluorescence spectrum possesses two broadened sidebands in the place of the Rabi sidebands under certain conditions. Moreover, the heights and widths of the sidebands can be controlled by tuning the driving parameters. The properties of the spectrum is determined by the transitions between the Floquet states in a rotating frame. The broadened sidebands result from the quasi-continuous quasienergy spectrum which happens with steering the beat frequency lower. The present study provides insights into the Floquet engineering of the fluorescence spectral features with polychromatic excitation fields.
We experimentally demonstrate the resonance fluorescence of a two-level artificial atom strongly coupled to a single-mode cavity field. The effect was theoretically predicted thirty years ago by Savage [Phys. Rev. Lett. 63, 1376 (1989)]. The system consists of a superconducting qubit circuit and a one-dimensional transmission line resonator. In addition, a one-dimensional transmission line strongly coupled to the atom serves as an open space. The effect takes place, when a microwave field is applied to the cavity, which in turn is resonantly coupled to the atom. The fluorescence spectrum is measured via the emission into the transmission line. We find that the central peak is determined by the atom spontaneous emission to the open space and the widths of side peaks are largely determined by the coherent interaction between the atom and the cavity, that is, the fluorescence spectrum here is very different from that of the Mollow triplet. We also derive analytical form for the spectrum. Our experimental results agree well with theoretical calculations.