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Physical Review Letters

Finite-Size Scaling Approach for Critical Wetting: Rationalization in Terms of a Bulk Transition with an Order Parameter Exponent Equal to Zero

Ezequiel Vicente Albano, Kurt Binder

Published Jul 16, 2012• 27 citations
Publisher

Abstract

Clarification of critical wetting with short-range forces by simulations has been hampered by the lack of accurate methods to locate where the transition occurs. We solve this problem by developing an anisotropic finite-size scaling approach and show that then the wetting transition is a "bulk" critical phenomenon with order parameter exponent equal to zero. For the Ising model in two dimensions, known exact results are straightforwardly reproduced. In three dimensions, it is shown that previous estimates for the location of the transition need revision, but the conclusions about a slow crossover away from mean-field behavior remain unaltered.

DOI
10.1103/physrevlett.109.036101

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We performed extensive simulations of the random-bond Ising model confined between walls where competitive surface fields act. By properly taking the thermodynamic limit we unambiguously determined wetting transition points of the system, as extrapolation of localization-delocalization transitions of the interface between domains of different orientation driven by the respective fields. The finite-size scaling theory for wetting with short-range fields [E. V. Albano and K. Binder, Phys. Rev. Lett. 109, 036101 (2012)] establishes that the average magnetization of the sample, with critical exponent $\ensuremath{\beta}$, is the proper order parameter for the study of wetting. While the hyperscaling relationship given by $\ensuremath{\gamma}+2\ensuremath{\beta}={\ensuremath{\nu}}_{\ensuremath{\parallel}}+{\ensuremath{\nu}}_{\ensuremath{\perp}}$ requires $\ensuremath{\beta}=1/2$ ($\ensuremath{\gamma}=4, {\ensuremath{\nu}}_{\ensuremath{\parallel}}=3$, and ${\ensuremath{\nu}}_{\ensuremath{\perp}}=2$), the thermodynamic scaling establishes that ${\mathrm{\ensuremath{\Delta}}}_{s}=\ensuremath{\gamma}+\ensuremath{\beta}$, which in contrast requires $\ensuremath{\beta}=0$ (${\mathrm{\ensuremath{\Delta}}}_{s}=4$), where $\ensuremath{\gamma}, {\ensuremath{\nu}}_{\ensuremath{\parallel}}, {\ensuremath{\nu}}_{\ensuremath{\perp}}$, and ${\mathrm{\ensuremath{\Delta}}}_{s}$ are the critical exponents of the susceptibility, the correlation lengths parallel and perpendicular to the interface, and the gap exponent, respectively. So, we formulate a finite-size scaling theory for wetting without hyperscaling and perform numerical simulations that provide strong evidence of hyperscaling violation (i.e., $\ensuremath{\beta}=0$) and a direct measurement of the susceptibility critical exponent $\ensuremath{\gamma}/{\ensuremath{\nu}}_{\ensuremath{\perp}}=2.0\ifmmode\pm\else\textpm\fi{}0.2$, in agreement with theoretical results for the strong fluctuation regime of wetting transitions with quenched noise.

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Tests of nonuniversality and finite-size scaling for two-dimensional wetting with long-ranged forces

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Effective Hamiltonian models predict nonuniversal critical singularities for two-dimensional wetting transitions with marginal long-ranged forces. We test these predictions by studying interfacial delocalization transitions in an infinitely long Ising strip, of width L (lattice spacings), with external fields that are long ranged and have opposite signs at each surface. Finite-size scaling suggests that the shift of the delocalization temperature T(c)(L) below the (semi-infinite) wetting temperature T(w) scales as L(-1/beta(s)) with beta(s) the adsorption critical exponent. Density-matrix renormalization-group methods allow us to study the behavior of T(c)(L) for L up to several hundred lattice spacings. For short-ranged forces the method recovers the universal value of beta(s)=1 known from the exact solution. While marginal long-ranged forces strongly influence the finite-size scaling of T(c)(L) , the extrapolated asymptotic value for the exponent beta(s) does not appear to confirm the predicted nonuniversality, but instead approaches the same universal value representative of systems with short-ranged forces.

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Clarification of critical wetting with short-range forces by simulations has been hampered by the lack of accurate methods to locate where the transition occurs. We solve this problem by developing an anisotropic finite-size scaling approach and show that then the wetting transition is a "bulk" critical phenomenon with order parameter exponent equal to zero. For the Ising model in two dimensions, known exact results are straightforwardly reproduced. In three dimensions, it is shown that previous estimates for the location of the transition need revision, but the conclusions about a slow crossover away from mean-field behavior remain unaltered.
We performed extensive simulations of the random-bond Ising model confined between walls where competitive surface fields act. By properly taking the thermodynamic limit we unambiguously determined wetting transition points of the system, as extrapolation of localization-delocalization transitions of the interface between domains of different orientation driven by the respective fields. The finite-size scaling theory for wetting with short-range fields [E. V. Albano and K. Binder, Phys. Rev. Lett. 109, 036101 (2012)] establishes that the average magnetization of the sample, with critical exponent $\ensuremath{\beta}$, is the proper order parameter for the study of wetting. While the hyperscaling relationship given by $\ensuremath{\gamma}+2\ensuremath{\beta}={\ensuremath{\nu}}_{\ensuremath{\parallel}}+{\ensuremath{\nu}}_{\ensuremath{\perp}}$ requires $\ensuremath{\beta}=1/2$ ($\ensuremath{\gamma}=4, {\ensuremath{\nu}}_{\ensuremath{\parallel}}=3$, and ${\ensuremath{\nu}}_{\ensuremath{\perp}}=2$), the thermodynamic scaling establishes that ${\mathrm{\ensuremath{\Delta}}}_{s}=\ensuremath{\gamma}+\ensuremath{\beta}$, which in contrast requires $\ensuremath{\beta}=0$ (${\mathrm{\ensuremath{\Delta}}}_{s}=4$), where $\ensuremath{\gamma}, {\ensuremath{\nu}}_{\ensuremath{\parallel}}, {\ensuremath{\nu}}_{\ensuremath{\perp}}$, and ${\mathrm{\ensuremath{\Delta}}}_{s}$ are the critical exponents of the susceptibility, the correlation lengths parallel and perpendicular to the interface, and the gap exponent, respectively. So, we formulate a finite-size scaling theory for wetting without hyperscaling and perform numerical simulations that provide strong evidence of hyperscaling violation (i.e., $\ensuremath{\beta}=0$) and a direct measurement of the susceptibility critical exponent $\ensuremath{\gamma}/{\ensuremath{\nu}}_{\ensuremath{\perp}}=2.0\ifmmode\pm\else\textpm\fi{}0.2$, in agreement with theoretical results for the strong fluctuation regime of wetting transitions with quenched noise.
A long-standing problem in condensed matter physics concerns the nature of the critical wetting phase transition in the Ising model or, more generally, in 3D systems with short-ranged forces.This is of fundamental interest because 3D corresponds to the upper critical dimension of the transition and it is not clear a priori whether the behaviour of the system will be mean-field-like or fluctuation-dominated.Renormalization group studies of the standard coarse-grained effective interfacial Hamiltonian model famously predict strong non-universal critical exponents which depend on the value of the so-called wetting parameter ω.However, these predictions are at odds with extensive Monte Carlo simulations of wetting in the Ising model, due to Binder, Landau and coworkers, which appear to be more mean-field-like.Further amendments to the interfacial Hamiltonian, which included the presence of a position-dependent stiffness, worsened the problem by paradoxically predicting fluctuation-induced first-order wetting behaviour.Here we show from re-analysis of a microscopic Landau-Ginzburg-Wilson model of 3D short-ranged wetting that correlation functions are characterized by two diverging parallel length scales, not one, as previously thought.This has a simple diagrammatic explanation using a non-local interfacial Hamiltonian and yields a thermodynamically consistent theory of wetting in keeping with exact sum rules.The non-local model crucially contains long-ranged two-body interfacial interactions, characterized by the new length scale, which were missing in earlier treatments.For critical wetting the second length cuts off the spectrum of interfacial fluctuations determining the repulsion from the wall.We show how this corrects previous renormalization group predictions for fluctuation effects, based on local interfacial Hamiltonians.In particular, lowering the cut-off leads to a substantial reduction in the effective value of the wetting parameter controlling the non-universality and also prevents the transition being driven first-order.Quantitative comparison with the Ising model simulation studies is also made.
The global phase diagram of wetting in the two-dimensional Ising model is obtained through the exact calculation of the surface excess free energy. In addition to a surface field for inducing wetting, a surface-coupling enhancement is also included. The wetting transition (of second order) is critical for any finite ratio of surface coupling J_{s} to bulk coupling J, and becomes of first order in the limit J_{s}/J→∞. However, for J_{s}/J≫1, the critical region is exponentially small and is practically invisible to numerical studies. A distinct preasymptotic regime exists in which the transition displays first-order character. In this regime, surprisingly, the surface susceptibility and surface specific heat develop a divergence and show anomalous scaling with an exponent equal to 3/2.
Critical and tricritical wetting transitions are studied in a simple-cubic nearest-neighbor Ising model. The magnetization m1{m}_{1}m1​ in the surface layer and the susceptibilities ${\ensuremath{\chi}}_{11}=\frac{\ensuremath{\partial}{m}_{1}}{\ensuremath{\partial}{H}_{1}}$ and ${\ensuremath{\chi}}_{1}=\frac{\ensuremath{\partial}{m}_{1}}{\ensuremath{\partial}H}$, where H1{H}_{1}H1​ is the surface field and HHH the bulk field, are calculated by use of Monte Carlo methods. The critical behavior of these quantities is found to be consistent with simple mean-field behavior; the singularities predicted by various renormalization-group treatments are not observed.
Effective Hamiltonian models predict nonuniversal critical singularities for two-dimensional wetting transitions with marginal long-ranged forces. We test these predictions by studying interfacial delocalization transitions in an infinitely long Ising strip, of width L (lattice spacings), with external fields that are long ranged and have opposite signs at each surface. Finite-size scaling suggests that the shift of the delocalization temperature T(c)(L) below the (semi-infinite) wetting temperature T(w) scales as L(-1/beta(s)) with beta(s) the adsorption critical exponent. Density-matrix renormalization-group methods allow us to study the behavior of T(c)(L) for L up to several hundred lattice spacings. For short-ranged forces the method recovers the universal value of beta(s)=1 known from the exact solution. While marginal long-ranged forces strongly influence the finite-size scaling of T(c)(L) , the extrapolated asymptotic value for the exponent beta(s) does not appear to confirm the predicted nonuniversality, but instead approaches the same universal value representative of systems with short-ranged forces.