The criterion for photon antibunching manifested in the second-order correlation function of a single-mode radiation can be established by the relation1
We consider a way to generate operational inequalities to test nonclassicality (or quantumness) of multimode bosonic fields (or multiparty bosonic systems) that unifies the derivation of many known inequalities and allows to propose new ones. The nonclassicality criteria are based on Vogel's criterion corresponding to analyzing the positivity of multimode P functions or, equivalently, the positivity of matrices of expectation values of, e.g., creation and annihilation operators. We analyze not only monomials but also polynomial functions of such moments, which can sometimes enable simpler derivations of physically relevant inequalities. As an example, we derive various classical inequalities which can be violated only by nonclassical fields. In particular, we show how the criteria introduced here easily reduce to the well-known inequalities describing (a) multimode quadrature squeezing and its generalizations, including sum, difference, and principal squeezing; (b) two-mode one-time photon-number correlations, including sub-Poisson photon-number correlations and effects corresponding to violations of the Cauchy-Schwarz and Muirhead inequalities; (c) two-time single-mode photon-number correlations, including photon antibunching and hyperbunching; and (d) two- and three-mode quantum entanglement. Other simple inequalities for testing nonclassicality are also proposed. We have found some general relations between the nonclassicality and entanglement criteria, in particular those resulting from the Cauchy-Schwarz inequality. It is shown that some known entanglement inequalities can be derived as nonclassicality inequalities within our formalism, while some other known entanglement inequalities can be seen as sums of more than one inequality derived from the nonclassicality criterion. This approach enables a deeper analysis of the entanglement for a given nonclassicality.
The concept of photon antibunching as a manifestation of nonclassical character in single-mode radiation is extended to two-mode radiation. A simple criterion for the existence of nonclassical effects in two-mode radiation is established. It implies that the intermode photon bunching, rather than antibunching, can play a key role in rendering two-mode radiation nonclassical. The two-mode squeezed vacuum states are used as simple examples to illustrate the essential point of the criterion. The criterion is then used to study the nonclassical properties of two types of two-mode squeezed states. A state generated by applying the squeeze operator to the two-mode vacuum first, followed by the displacement operator, is called a two-mode coherent squeezed state. If the order of the two operators is reversed, a two-mode squeezed coherent state is obtained. It is found that the latter has a much stronger tendency to become a nonclassical state than the former, assuming that the parameters involved are all the same. A measure of nonclassical depth of radiation is adopted. It is found that, according to this measure, the effect of squeezing in making two-mode coherent squeezed states nonclassical is not monotonic. Such phenomena do not occur in squeezed coherent states.