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Optics Express

Cooperative optical response of 2D dense lattices with strongly correlated dipoles

Sung-Mi Yoo, Sun Mok Paik

Published Jan 27, 2016• 29 citations
Publisher

Abstract

We study light propagation in dense low-temperature atoms on two-dimensional (2D) square and kagome lattices using a basically exact large-scale numerical computations. In the limit of weak laser intensity, shifts of the resonance line are shown in homogeneously broadened stationary samples with high atom densities, whereas the shifts are not shown in the samples with low densities. We obtain the dependence of shifts on interatomic spacing for square lattices with the various numbers of atoms, and our numerical results are in good agreement with shifts derived using a 2D isotropic infinite lattice model and experimental data for nanometric-thickness atomic ensembles in the literature.

DOI
10.1364/oe.24.002156

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We study light propagation in dense low-temperature atoms on two-dimensional (2D) square and kagome lattices using a basically exact large-scale numerical computations. In the limit of weak laser intensity, shifts of the resonance line are shown in homogeneously broadened stationary samples with high atom densities, whereas the shifts are not shown in the samples with low densities. We obtain the dependence of shifts on interatomic spacing for square lattices with the various numbers of atoms, and our numerical results are in good agreement with shifts derived using a 2D isotropic infinite lattice model and experimental data for nanometric-thickness atomic ensembles in the literature.
We study the optical response of a two-dimensional (2D) square lattice of atoms using classical electrodynamics. Because of dipole-dipole interactions, the lattice atoms polarize as if the lattice were an atom with up to three resonance frequencies, with cooperatively shifted resonances and altered transition linewidths. We show that when the distance between two 2D lattices is large enough and Bragg reflections are absent, the lattices interact among themselves as if they radiated a plane wave whose amplitude is in accordance with the radiation from a dipole moment continuously distributed in the lattice plane. We employ these results to study light propagation in stacks of 2D lattices, drawing on simple qualitative pictures of the response of a 2D lattice and light propagation in one-dimensional (1D) waveguides. We show that a stack of 2D lattices may emulate regularly spaced atoms in a lossless 1D waveguide, and argue that in a suitable geometry the resonance shifts characteristic of 1D and 2D lattice structures may completely cancel to eliminate density-dependent resonance shifts of atoms bound to a three-dimensional (3D) lattice. A generalization to the case of anisotropic polarizability, such as in the presence of a magnetic field, reveals light frequencies induced by the magnetic field for which a 2D lattice is either completely transparent or completely opaque.
We theoretically investigate the optical response of many cold atoms within a pair of identical planar lattices mostly in a dense regime using microscopic electrodynamics numerical simulations. We find cooperative optical properties of the double atomic lattices to a normal incidence of low-intensity radiation at particular ranges of sample parameters. The main findings are that resonance shifts, linewidths, and transmittance could be engineered by varying layer-to-layer distance, lattice constant, and parameters for incident light. We also propose a bilayer atomic lattice could be modeled as two effective superatoms. Simulation results qualitatively agree with the ones from an isotropic infinite lattice model in the ranges of external parameters for which a mean-field approximation is not valid. Hopefully, our bilayer lattice samples might be exploited for implementing an optical switch and a photonic device in quantum computing.
Light propagation in disordered media is a fundamental and important problem in optics and photonics. In particular, engineering light-matter interaction in disordered cold atomic ensembles is one of the central topics in modern quantum and atomic optics. The collective response of dense atomic gases under light excitation, which crucially depends on the spatial distribution of atoms and the geometry of the ensemble, has important impacts on quantum technologies like quantum sensors, atomic clocks and quantum information storage. Here we analyze near-resonant light transmission in two-dimensional dense ultracold atomic ensembles with short-range positional correlations. Based on the coupled-dipole simulations under different atom number densities and correlation lengths, we show that the collective effects are strongly influenced by those positional correlations, manifested as significant shifts and broadening or narrowing of transmission resonance lines. We also analyze the eigenstate distribution of different atomic ensembles. This work may provide profound implications on collective and cooperative effects in cold atomic ensembles as well as the study of mesoscopic physics concerning light transport in strongly scattering disorder media.
Manipulation of light using atoms plays a fundamental and important role in emerging technologies such as integrated photonics, information storage, and quantum sensors. Specifically, there have been intense theoretical efforts involving large samples of cold neutral atoms for coherent control of light. Here we present a theoretical scheme that enables efficient computation of collective optical responses of mono- and bi-layer planar square lattices of dense, cold two-level atoms using classical electrodynamics of coupled dipoles in the limit of low laser intensity. The steady-state transmissivity and reflectivity are obtained at a field point far away from the atomic lattices in the regime with no Bragg reflection. While our earlier method was based on exact solution of the electrodynamics for a small-scale lattice, here we calculate the dipole moments assuming that they are the same at all lattice sites, as for an infinite lattice. Atomic lattices with effectively over one hundred times more sites than in our earlier exact computations can then be simulated numerically with fewer computational resources. We have implemented an automatic selection of the number of sites under the given convergence criteria. We compare the numerical results from both computational schemes. We also find similarities and differences of a stack of two atomic lattices from a two-atom sample. Such aspects may be exploited to engineer a stack for potential applications.
We study propagation of low-intensity light in a medium within a one-dimensional (1D) model electrodynamics. It is shown that the coupled theory for light and matter fields may be solved, in principle exactly, by means of stochastic simulations that account for both collective linewidths and line shifts, and for quantum statistical position correlations of the atoms. Such simulations require that one synthesize atomic positions that have correlation functions appropriate for the given type of atomic sample. We demonstrate how one may simulate both a Bose-Einstein condensate (BEC) and a zero-temperature noninteracting Fermi-Dirac gas. Results of simulations of light propagation in such quantum degenerate gases are compared with analytical density expansions obtained by adapting the approach of Morice, Castin, and Dalibard [Phys. Rev. A 51, 3896 (1995)] to the 1D electrodynamics. A BEC exhibits an optical resonance that narrows and stays somewhat below the atomic resonance frequency as collective effects set in with increasing atom density. The first two terms in the analytical density expansion are in excellent agreement with numerical results for a condensate. While fermions display a similar narrowing and shift of the resonance with increasing density, already in the limit of very dilute gas the linewidth is only half of the resonance linewidth of an isolated atom. We attribute this to the regular spacing between the atoms, which is enforced by the Pauli exclusion principle. The analytical density expansion successfully predicts the narrowing, and also gives the next term in the density expansion of the optical response in semiquantitative agreement with numerical simulations.
We derive equations for the strongly coupled system of light and dense atomic ensembles. The formalism includes an arbitrary internal-level structure for the atoms and is not restricted to weak excitation of atoms by light. In the low-light-intensity limit for atoms with a single electronic ground state, the full quantum field-theoretical representation of the model can be solved exactly by means of classical stochastic electrodynamics simulations for stationary atoms that represent cold atomic ensembles. Simulations for the optical response of atoms in a quantum degenerate regime require one to synthesize a stochastic ensemble of atomic positions that generates the corresponding quantum statistical position correlations between the atoms. In the case of multiple ground levels or at light intensities where saturation becomes important, the classical simulations require approximations that neglect quantum fluctuations between the levels. We show how the model is extended to incorporate corrections due to quantum fluctuations that result from virtual scattering processes. In the low-light-intensity limit, we illustrate the simulations in a system of atoms in a Mott-insulator state in a two-dimensional optical lattice, where recurrent scattering of light induces strong interatomic correlations. These correlations result in collective many-atom subradiant and superradiant states and a strong dependence of the response on the spatial confinement within the lattice sites.