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Cambridge University Press eBooks

Complement 8A: Cooling to sub-recoil temperatures by velocity-selective coherent population trapping

G. Grynberg, Alain Aspect, Claude Fabre, Claude N. Cohen-Tannoudji

Published Sep 2, 2010• 0 citations
Publisher

Abstract

In Section 8.3.9, we mentioned that the recoil temperature was not the ultimate barrier to cooling. Several mechanisms have been conceived and implemented to concentrate the atomic velocity distribution in a range of values of width less than V R . In contrast to Doppler or Sisyphus cooling, these mechanisms do not appeal to a friction force, but rather to an optical pumping process (see Complement 2B), able to accumulate the atoms in this narrow range of velocities. We now present one such mechanism called ‘velocity-selective coherent population trapping’, considering only the case where the motion occurs in one space direction (the O z -axis). Note, however, that the method generalizes to two or three dimensions. Coherent population trapping Coherent population trapping is a phenomenon that occurs when an atom has a system of three energy levels in the ∧ configuration shown in Figure 8A.1, where each leg of the ∧ interacts with a laser L − or L + . This was discussed in detail in Section 2D.2 of Complement 2D. Here we consider the case where the two ground states g + and L − , have exactly the same energy, and the two lasers have frequencies ω + and ω − , very close to the resonance frequency ω 0 . In this situation, the selectivity of the interactions is obtained via the polarization selection rules (see Complement 2B): if g − , g + and e have magnetic quantum numbers m = −1, +1 and 0, respectively, the laser wave L − is right-circularly polarized (σ + polarization), while the laser wave L + is left-circularly polarized (σ − polarization).

DOI
10.1017/cbo9780511778261.038

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In Section 8.3.9, we mentioned that the recoil temperature was not the ultimate barrier to cooling. Several mechanisms have been conceived and implemented to concentrate the atomic velocity distribution in a range of values of width less than V R . In contrast to Doppler or Sisyphus cooling, these mechanisms do not appeal to a friction force, but rather to an optical pumping process (see Complement 2B), able to accumulate the atoms in this narrow range of velocities. We now present one such mechanism called ‘velocity-selective coherent population trapping’, considering only the case where the motion occurs in one space direction (the O z -axis). Note, however, that the method generalizes to two or three dimensions. Coherent population trapping Coherent population trapping is a phenomenon that occurs when an atom has a system of three energy levels in the ∧ configuration shown in Figure 8A.1, where each leg of the ∧ interacts with a laser L − or L + . This was discussed in detail in Section 2D.2 of Complement 2D. Here we consider the case where the two ground states g + and L − , have exactly the same energy, and the two lasers have frequencies ω + and ω − , very close to the resonance frequency ω 0 . In this situation, the selectivity of the interactions is obtained via the polarization selection rules (see Complement 2B): if g − , g + and e have magnetic quantum numbers m = −1, +1 and 0, respectively, the laser wave L − is right-circularly polarized (σ + polarization), while the laser wave L + is left-circularly polarized (σ − polarization).
We present a theoretical analysis of a new one-dimensional laser-cooling scheme that was recently demonstrated on a beam of metastable 4He atoms. Both internal and translational degrees of freedom are treated quantum mechanically. Unlike semiclassical approaches, such a treatment can be applied to situations in which the atomic coherence length is of the same order of or larger than the laser wavelength, which is the case for atoms cooled below the one-photon recoil energy. We introduce families of states that are closed with respect to absorption and stimulated emission, and we establish the generalized optical Bloch equations that are satisfied by the corresponding matrix elements. The existence of velocity-selective trapping states that are linear combinations of states with different internal and translational quantum numbers is demonstrated, and the mechanism of accumulation of atoms in these trapping states by fluorescence cycles is analyzed. From a numerical solution of the generalized optical Bloch equations, we study in detail how the final atomic-momentum distribution depends on the various physical parameters: interaction time, width of the initial distribution, laser detuning, laser power, and imbalance between the two counterpropagating waves. We show that the final temperature decreases when the interaction time increases, so that there is no fundamental limit to the lowest temperature that can be achieved by such a method. Finally, possible extensions of this method to two-dimensional cooling are presented.
We have demonstrated velocity-selective coherent population trapping (VSCPT) in a two-level system created by circularly polarized light driving the $2{}^{3}{S}_{1}\ensuremath{\rightarrow}3{}^{3}{P}_{2}$ transition in metastable helium. It is quite different from the usual VSCPT because there need be no consideration of selection rules, polarization, or internal atomic states. This most primitive case elicits the simple nature of VSCPT as a special kind of quantum interference, and demonstrates the presence of VSCPT in a system that has only two internal levels. It is readily observed for this transition because the ratio of the recoil frequency to the natural linewidth is 0.22, two orders of magnitude larger than for most laser cooling experiments. Our trapped state is fed by Doppler cooling, which is unusually effective here because of the large recoil, and is totally absent in previously described VSCPT experiments.
We report the first observation of subrecoil laser cooling in three dimensions, where we use the method of velocity-selective coherent population trapping. We have cooled a cloud of trapped metastable helium atoms to 180 nK, 22 times below the single-photon recoil temperature, with an enhancement in the momentum-space density of 16. We find that the efficiency with which the velocity-selective trap is populated can be augmented by Sisyphus-type frictional forces, while the cooling process is accompanied by the diffusion of atoms to states of very high velocity.
Sub-Doppler laser cooling requires optical pumping among differently light-shifted ground-state sublevels. We describe a study of the simplest possible angular-momentum configuration that permits all sub-Doppler cooling phenomena. The Jg = 1 ⇒ Je = 0 angular-momentum configuration shows recoil-limited cooling in the two most well-known types of polarization gradient, magnetically induced laser cooling, velocity-selective resonances, transient cooling, and velocity-selective population trapping.
We present a fully quantum analysis of velocity selective coherent population trapping (VSCPT) in two schemes for which there is a force which assists in the accumulation of atoms in the trapping state. In the first scheme, the F g =2 to F e =2 transition was studied where the existence of a semiclassical polarization gradient force even for a pure sigma + - sigma - configuration has been demonstrated which gives cooling for blue detuning. We also verify that cooling may be obtained for the F=2 to 1 and F=3 to 2 transitions; our fully quantum mechanical calculations yield a result which is consistent with recent experimental results of Valentin et al. (1992) but differ from previous semiclassical calculations. Secondly, we discuss a scheme of force-assisted VSCPT which combines VSCPT on the F g =1 to F e =1 transition with the coupling to another transition for which a strong sub-Doppler cooling force is present. This scheme allows velocity selective coherent population trapping and the polarization-gradient force to work under optimum conditions simultaneously. We find that both of these two schemes lead to efficient cooling of atoms.
Two-dimensional laser cooling based on velocity-selective coherent population trapping is investigated theoretically for the J = 1 ↔ J = 1 atomic transition. Wave vectors and polarizations of three laser beams are chosen to realize a coherent superposition of three degenerate ground states. For the first time forces related to Doppler and interference effects are combined with coherent population trapping to realize a very efficient cooling. Numerical solutions are presented for laser cooling of helium atoms.