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ACTA PHOTONICA SINICA

Investigation on Stimulated Photon Echo Induced by Optical Transition of 1se1sh Excitons in Core-shell CdSe/ZnS Quantum Dot-quantum Well

龚少华 GONG Shao-hua, 傅军 FU Jun, 符运良 FU Yun-liang, 沈振江 SHEN Zhen-jiang

Published Jan 1, 2012• 0 citations
Publisher

Abstract

在建模和理论分析的基础上, 对三脉冲飞秒激光作用下核壳结构CdSe/ZnS量子点量子阱中1s e 1s h 激子光跃迁引起的受激光子回波效应进行了深入研究.运用有效质量近似方法求解了载流子的静态薛定谔方程,得到能量本征值和对应波函数.基于光学Bloch方程,分析了受激光子回波的参量相关性.结果显示受激光子回波信号可以通过量子点量子阱结构和尺寸的改变进行有效调节.同时,在量子尺寸限制理论的基础上讨论了结构和尺寸的变化对受激光子回波信号的具体影响.

DOI
10.3788/gzxb20124101.0054

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在建模和理论分析的基础上, 对三脉冲飞秒激光作用下核壳结构CdSe/ZnS量子点量子阱中1s e 1s h 激子光跃迁引起的受激光子回波效应进行了深入研究.运用有效质量近似方法求解了载流子的静态薛定谔方程,得到能量本征值和对应波函数.基于光学Bloch方程,分析了受激光子回波的参量相关性.结果显示受激光子回波信号可以通过量子点量子阱结构和尺寸的改变进行有效调节.同时,在量子尺寸限制理论的基础上讨论了结构和尺寸的变化对受激光子回波信号的具体影响.
The energies of 1s states inside and outside the quantum well of a CdSe/ZnS quantum-dot quantum well (QDQW) and the transition dipole moment between these two states have been calculated by effective mass approximation. By using the calculation results, the longitudinal and transversal relaxation times of CdSe/ZnS have been approximated. We obtain a three-pulse photon echo (TPE) signal on the basis of the two states using the optical Bloch equations. We find that there should be four echoes in TPE from our theoretical calculation. In particular, the effects of the variation in core radius and shell thickness have been studied. It has been shown from the numerical calculation that the TPE signal is strongly dependent on the size and structure of the QDQW, and is dominated by relaxation time, which is also dependent on the size and structure.