The work presented in this thesis investigates theoretically and experimentally quantum memories with atomic ensembles, which are suited for long-distance quantum communication. For this purpose laser-cooled, ultracold atomic clouds of Rubidium 87 are used as memory for nonclassical single-photon states. Base on the atom-light interface of the protocol from Duan, Lukin, Cirac, Zoller (DLCZ) for long distance quantum communication the single photons states are stored and retrieved. By the help of non-classical correlations and the quantum memory a deterministic single photon source is demonstrated. The Hong-Ou-Mandel dip between two single photons created in this way has been measured. Moreover it is reported on the realization of a long-lived quantum memory by using magnetic-field insensitive atomic states in an optical trap and that by extending the spinwave's wavelength the dephasing of the memory due to thermal motion could be suppressed. Measured storage times of over a millisecond represent a significant progress towards the realization of long distance quantum communication.
The work presented in this thesis investigates theoretically and experimentally quantum memories with atomic ensembles, which are suited for long-distance quantum communication. For this purpose laser-cooled, ultracold atomic clouds of Rubidium 87 are used as memory for nonclassical single-photon states. Base on the atom-light interface of the protocol from Duan, Lukin, Cirac, Zoller (DLCZ) for long distance quantum communication the single photons states are stored and retrieved. By the help of non-classical correlations and the quantum memory a deterministic single photon source is demonstrated. The Hong-Ou-Mandel dip between two single photons created in this way has been measured. Moreover it is reported on the realization of a long-lived quantum memory by using magnetic-field insensitive atomic states in an optical trap and that by extending the spinwave's wavelength the dephasing of the memory due to thermal motion could be suppressed. Measured storage times of over a millisecond represent a significant progress towards the realization of long distance quantum communication.
Quantum memories are an essential building block for quantum information science, and in particular for the implementation of quantum communications across long distances. A quantum memory is defined as a system capable of storing and retrieving quantum states on-demand, such as quantum bits (qubits). Atomic ensembles are good candidates for this purpose because they enables strong light-matter coupling in case of a large number of atoms. Moreover, the collective effect, enhanced in the regime of large optical depth, can lead to storage efficiency close to unity. Thus, in this thesis, a large magneto-optical trap for cesium atoms is used as a atomic medium in order to implement a quantum memory protocol based on electromagnetically induced transparency (EIT). First, the EIT phenomenon is studied through a criterion for the discrimination between the EIT and the Autler-Townes splitting models. We then report on the implementation of an EIT-based memory for photonic qubits encoded in orbital angular momentum (OAM) of light. A reversible memory for Laguerre-Gaussian modes is implemented, and we demonstrate that the optical memory preserves the handedness of the helical structure at the single-photon level. Then, a full quantum state tomography of the retrieved OAM encoded qubits is performed, giving fidelities above the classical bound. This showed that our optical memory operates in the quantum regime. Finally, we present the implementation of the so-called DLCZ protocol in our ensemble of cold atoms, enabling the generation of heralded single photons. A homodyne detection setup allows us to realize the quantum tomography of the created photonic state.
Quantum communication between two remote locations often involves remote parties sharing an entangled quantum state. At present, entanglement distribution is usually performed using photons transmitted through optical fibers. However, the absorption of light in the fiber limits the communication distances to less than 200 km, even for optimal photon telecom wavelengths. To increase this distance, the quantum repeater idea was proposed. In the quantum repeater architecture, one divides communication distance into segments of the order of the attenuation length of the photons and places quantum memory nodes at the intermediate locations. Since the photon loss between intermediate locations is low, it is possible then to establish entanglement between intermediate quantum memory nodes. Once entanglement between adjacent nodes is established, one can extend it over larger distances using entanglement swapping.\n\nThe long coherence time of a quantum memory is a crucial requirement for the quantum repeater protocol. It is obvious that the coherence time of a quantum memory should be much longer that the time it takes for light to travel between remote locations. For a communication distance l = 1000 km, the corresponding time is t = l/c = 3.3 ms. One can show that for a simple repeater protocol and realistic success probabilities of entanglement generation, the required coherence time should be on the order of many seconds, while for the more complicated protocols that involve multiplexing and several quantum memory cells per intermediate node, the required coherence time is on the order of milliseconds.\n\nIn this thesis, I describe a quantum memory based on an ensemble of rubidium atoms confined in a one-dimensional optical lattice. The use of the magnetically- insensitive clock transition and suppression of atomic motion allows us to increase coherence time of the quantum memory by two-orders of magnitude compared to previous work. I also propose a method for determining the Zeeman content of atomic samples. In addition, I demonstrate the observation of quantum evolution under continuous measurement. The long quantum memory lifetime demonstrated in this work opens the way for scalable processing of quantum information and long distance quantum communication.
The realization of a large-scale quantum network of interconnected quantum nodes is one of the most promising directions in quantum technology. Such a network distributes entanglement between remote matter qubits via single photons in optical fibers, enabling quantum repeaters and long-distance secure communication and supporting emerging applications such as distributed quantum computing and network-enhanced metrology. To realize this vision, proposed architectures require quantum nodes that provide an efficient quantum light-matter interface for entanglement generation, serve as a quantum memory allowing long-lived storage of quantum states, and have the possibility to connect to telecommunication fiber-based photonic channels. This thesis presents the development and experimental realization of a quantum network node based on a single Rb-87 atom. A single atom is confined in a tightly focused optical dipole trap, and entanglement is generated between the polarization of an emitted photon and the Zeeman state of the atom. To enable long-lived quantum storage, we coherently map the atomic qubit to a basis less sensitive to magnetic fields using Zeeman-state-selective Raman transfer, reducing magnetic field sensitivity by a factor of 500. Such hyperfine qubit control is implemented via a two-photon Raman process driven by a laser field that is amplitude modulated at the qubit splitting using a fiber-based Mach-Zehnder interferometer. With this approach, we achieve a 1/e storage lifetime of 10 ms, extending coherence by a factor of 30 compared with the initial qubit encoding. Residual dephasing arises primarily from position-dependent effective magnetic fields caused by the tightly focused optical dipole trap beam together with atomic motion, and the differential AC-Stark shifts come from the trap detuning. While the first can be fully canceled via a standing-wave dipole trap, which needs to change the trap setup. We mitigate the second effects with a spin-echo pulse, extending coherence by a factor of two. Nonetheless, the significantly longer coherence time already allows high-fidelity entanglement distribution over fiber links with a length of a few hundred kilometers. To reduce fiber attenuation for long-distance distribution, we convert the emitted 780 nm single photons to the low-loss telecom S band using difference-frequency generation in a periodically poled lithium niobate waveguide, pumped at 1607 nm to produce 1517 nm photons. By combining long-lived quantum memory with a telecom interface, we demonstrated long-distance atom-photon entanglement distribution through 50 km and 101 km of spooled fiber with fidelities of 85% and 71%, respectively, establishing a key component for scalable quantum communication. These results establish neutral atom nodes as promising building blocks for metropolitan-scale quantum networking and outline a scalable path toward repeater protocols based on multiplexing memories and Rydberg-mediated interactions.
Quantum communication deals with absolutely secure transfer of classical messages by means of quantum cryptography or faithful transfer of unknown quantum states by means of quantum teleportation between distant sites. The essential element for quantum communication is to create remote entangled pairs of high fidelity. The main difficulty to create such a distant entangled pair is that both photon loss and decoherence grow exponentially with distance. However, with the help of quantum repeater, it is demonstrated that both the entanglement sources and the time needed to create a single distant entangled pair of high fidelity could scale polynomially with the communication length. Here we propose a robust quantum repeater by extending the original Duan-Lukin-Cirac-Zoller (DLCZ) scheme based on atomic ensembles and linear optics. Our protocol entails the advantage of two photon interference, which is more robust than single photon interference used in the DLCZ scheme. In comparison with our previous proposal, the entangled memory qubits are manipulated across long distance, and local entanglement pairs are avoided. Our proposal provides an exciting possibility for realistic long distance quantum communication.
A reversible quantum memory allowing us to store and retrieve quantum information serves as a key necessity for implementing many of novel quantum information protocols. As light serves as a reliable long-range carrier of quantum information, and atoms offer the possibility of long storage times, current attempts at creating quantum memories focus on the transfer of the quantum fluctuations of light onto atomic coherences. The work in this thesis focuses on the development of a quantum memory for squeezed light using an ensemble of cold Cesium atoms stored in a magneto-optical trap. Our two major milestones were the development of a source of nonclassical light, and the development of a suitable atomic medium for storage. We first present the results of our efforts to generate a source of squeezed vacuum states resonant with the Cesium D2 line using a PPKTP nonlinear crystal inside of an optical parametric oscillator. Additionally, we characterize these squeezed states by carrying out a quantum state tomography using an iterative maximum likelihood approach. Next we look at the development of a new experiment which would allow us to use cold Cesium atoms as a storage medium in our recently developed magneto-optical trap. As this requires an array of novel tools and experimental techniques, we will discuss the development of these elements, and how they have furthered our progress towards storing quantum states onto our Cesium atoms, and eventually entangling two atomic ensembles.
A hybrid interface of solid state single-photon sources and atomic quantum memories is a long sought-after goal in photonic quantum technologies. Here we demonstrate deterministic storage and retrieval of photons from a semiconductor quantum dot in an atomic ensemble quantum memory at telecommunications wavelengths. We store single photons from an InAs quantum dot in a high-bandwidth rubidium vapour based quantum memory, with a total internal memory efficiency of (12.9±0.4)%. The signal-to-noise ratio of the retrieved photons is 18.2±0.6, limited only by detector dark counts. This demonstration paves the way to quantum technologies that rely on distributed entanglement, and is especially suited for photonic quantum networks.