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Springer eBooks

Coherence and Dephasing

William W. Parson

Published Jan 1, 2015• 1 citation
Publisher
DOI
10.1007/978-3-662-46777-0_10

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Coherence-generating power of quantum dephasing processes

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We provide a quantification of the capability of various quantum dephasing processes to generate coherence out of incoherent states. The measures defined, admitting computable expressions for any finite Hilbert-space dimension, are based on probabilistic averages and arise naturally from the viewpoint of coherence as a resource. We investigate how the capability of a dephasing process (e.g., a nonselective orthogonal measurement) to generate coherence depends on the relevant bases of the Hilbert space over which coherence is quantified and the dephasing process occurs, respectively. We extend our analysis to include those Lindblad time evolutions which, in the infinite-time limit, dephase the system under consideration and calculate their coherence-generating power as a function of time. We further identify specific families of such time evolutions that, although dephasing, have optimal (over all quantum processes) coherence-generating power for some intermediate time. Finally, we investigate the coherence-generating capability of random dephasing channels.

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Mechanism of intermolecular dephasings on time-resolved anti-Stokes Raman scattering from a molecular ensemble

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Mechanisms of intermolecular dephasings revealed in the time-resolved coherent anti-Stokes Raman scattering (CARS) spectra of a molecular ensemble are theoretically studied by deriving the microscopical expression for the scattered photon intensity averaged over the heat-bath variables. The intermolecular dephasing means the decay of the intermolecular coherence created by the pumping process, i.e., a linear combination of the vibrational Raman transitions of the molecules at different sites. The intensity of the time-resolved CARS is expressed in terms of time-development matrix elements of the intermolecular coherence. An equation of motion for the intermolecular coherence is derived by using the projection operator method. The structure of the intermolecular-dephasing constant is clarified. The intermolecular-dephasing constant consists of the sum of population decay constants and the intermolecular pure dephasing constant that originates from an elastic interaction between the relevant molecules and a common heat-bath mode. The intermolecular pure dephasing constant is expressed in terms of the intramolecular pure dephasing constants and destructive interference of the intramolecular pure dephasings between the relevant two molecules. The intermolecular-dephasing constant is expressed as the sum of the intramolecular-dephasing constants of the relevant molecules when there is no common heat-bath mode. Inhomogeneous effects on the time-resolved CARS spectra are also investigated. A degree of the structural order is introduced to qualitatively express the inhomogeneity of local structures in the molecular ensemble. The microscopic expression derived in this paper has taken into account both incoherent and coherent optical processes in the thermally distributed molecular ensemble.

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Coherent Detection of Electron Dephasing

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We show that an Aharonov-Bohm ring with asymmetric electron injection can act as a coherent detector of electron dephasing. The presence of a dephasing source in one of the two arms of a moderately-to-highly asymmetric ring changes the response of the system from total reflection to complete transmission while preserving the coherence of the electrons propagating from the ring, even for strong dephasing. We interpret this phenomenon as an implementation of an interaction-free measurement.

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Coherence and Decoherence

Sushanta Dattagupta, Sanjay Puri

Springer series in materials science•Jan 1, 2004•0 citations
We provide a quantification of the capability of various quantum dephasing processes to generate coherence out of incoherent states. The measures defined, admitting computable expressions for any finite Hilbert-space dimension, are based on probabilistic averages and arise naturally from the viewpoint of coherence as a resource. We investigate how the capability of a dephasing process (e.g., a nonselective orthogonal measurement) to generate coherence depends on the relevant bases of the Hilbert space over which coherence is quantified and the dephasing process occurs, respectively. We extend our analysis to include those Lindblad time evolutions which, in the infinite-time limit, dephase the system under consideration and calculate their coherence-generating power as a function of time. We further identify specific families of such time evolutions that, although dephasing, have optimal (over all quantum processes) coherence-generating power for some intermediate time. Finally, we investigate the coherence-generating capability of random dephasing channels.
Mechanisms of intermolecular dephasings revealed in the time-resolved coherent anti-Stokes Raman scattering (CARS) spectra of a molecular ensemble are theoretically studied by deriving the microscopical expression for the scattered photon intensity averaged over the heat-bath variables. The intermolecular dephasing means the decay of the intermolecular coherence created by the pumping process, i.e., a linear combination of the vibrational Raman transitions of the molecules at different sites. The intensity of the time-resolved CARS is expressed in terms of time-development matrix elements of the intermolecular coherence. An equation of motion for the intermolecular coherence is derived by using the projection operator method. The structure of the intermolecular-dephasing constant is clarified. The intermolecular-dephasing constant consists of the sum of population decay constants and the intermolecular pure dephasing constant that originates from an elastic interaction between the relevant molecules and a common heat-bath mode. The intermolecular pure dephasing constant is expressed in terms of the intramolecular pure dephasing constants and destructive interference of the intramolecular pure dephasings between the relevant two molecules. The intermolecular-dephasing constant is expressed as the sum of the intramolecular-dephasing constants of the relevant molecules when there is no common heat-bath mode. Inhomogeneous effects on the time-resolved CARS spectra are also investigated. A degree of the structural order is introduced to qualitatively express the inhomogeneity of local structures in the molecular ensemble. The microscopic expression derived in this paper has taken into account both incoherent and coherent optical processes in the thermally distributed molecular ensemble.