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Journal of Physics B Atomic Molecular and Optical Physics

Large numbers of cold positronium atoms created in laser-selected Rydberg states using resonant charge exchange

Robert McConnell, G. Gabrielse, W. Steven Kolthammer, Philip Richerme, A. Müllers, J. Walz, D. Grzonka, Marcin Zieliński, D. W. Fitzakerley, M. C. George, Eric A. Hessels, C. H. Storry, M. Weel

Published Feb 23, 2016• 14 citations
Publisher

Abstract

Abstract Lasers are used to control the production of highly excited positronium atoms (Ps*). The laser light excites Cs atoms to Rydberg states that have a large cross section for resonant charge-exchange collisions with cold trapped positrons. For each trial with 30 million trapped positrons, more than 700 000 of the created Ps* have trajectories near the axis of the apparatus, and are detected using Stark ionization. This number of Ps* is 500 times higher than realized in an earlier proof-of-principle demonstration (2004 Phys. Lett. B 597 257). A second charge exchange of these near-axis Ps* with trapped antiprotons could be used to produce cold antihydrogen, and this antihydrogen production is expected to be increased by a similar factor.

DOI
10.1088/0953-4075/49/6/064002

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arXiv:0804.0371•Physical Review A•Nov 24, 2008•58 citations
Abstract Lasers are used to control the production of highly excited positronium atoms (Ps*). The laser light excites Cs atoms to Rydberg states that have a large cross section for resonant charge-exchange collisions with cold trapped positrons. For each trial with 30 million trapped positrons, more than 700 000 of the created Ps* have trajectories near the axis of the apparatus, and are detected using Stark ionization. This number of Ps* is 500 times higher than realized in an earlier proof-of-principle demonstration (2004 Phys. Lett. B 597 257). A second charge exchange of these near-axis Ps* with trapped antiprotons could be used to produce cold antihydrogen, and this antihydrogen production is expected to be increased by a similar factor.
Lasers are used to choose the binding energies of highly excited positronium atoms (Ps*) created via charge exchange collisions. The lasers directly excite cesium (Cs) atoms to highly excited states (Cs*). These large Cs*atoms have a large cross section for resonant charge exchange collisions with trapped positrons. Highly excited Ps* is formed with a binding energy that is determined by the initial laser excitation. These Ps* should have a large cross section for resonant charge exchange collisions with trapped antiprotons—suggesting a possible new way to produce cold antihydrogen.
Laser-controlled charge exchange is a promising method for producing cold antihydrogen. Caesium atoms in Rydberg states collide with positrons and create positronium. These positronium atoms then interact with antiprotons, forming antihydrogen. Laser excitation of the caesium atoms is essential to increase the cross section of the charge-exchange collisions. This method was demonstrated in 2004 by the ATRAP collaboration by using an available copper vapour laser. For a second generation of charge-exchange experiments we have designed a new semiconductor laser system that features several improvements compared to the copper vapour laser. We describe this new laser system and show the results from the excitation of caesium atoms to Rydberg states within the strong magnetic fields in the ATRAP apparatus.
Our ATRAP collaboration has now demonstrated a second technique for antihydrogen (H̄) production. Lasers are used for the first time to control the production of H̄ atoms in our cryogenic apparatus at CERN. As suggested in ref. [2] and first reported in ref. [1], lasers excite a thermal beam of cesium (Cs) atoms to a Rydberg state. In a first charge exchange collision one of these laser‐excited Cs atoms (Cs*) and a cold e+ produces positronium (Ps). Our measurements at Harvard([3]) and at CERN([1]) confirm CTMC simulations([2]) that the laser‐selected binding energy in the Cs atom is preserved by the collision and results in Ps with the selected binding energy. A second charge exchange is between one of these Ps atoms and a trapped p̄ . H̄ is produced by this second collision and is expected to again have the same binding energy. One advantage of this technique as discussed in ref. [2] is that the H̄ produced is expected to be extremely cold, at the temperature of the trapped p̄ , allowing for possible confinement of the H̄ atoms in a magnetic trap.
An efficient method for production of cold antihydrogen $(\mathrm{H}\ifmmode\bar\else\textasciimacron\fi{})$ is proposed. Alkali-metal atoms laser excited to a Rydberg state are charge exchanged with cold trapped positrons, producing Rydberg states of positronium. In a second Rydberg-state charge exchange, the positronium atoms give up their Rydberg positrons to cold trapped antiprotons, producing Rydberg states of $\mathrm{H}\ifmmode\bar\else\textasciimacron\fi{}$. These $\mathrm{H}\ifmmode\bar\else\textasciimacron\fi{}$ atoms soon decay down to the ground state, and, because they are cold, could be trapped in a magnetic trap. The efficiency of the process results from the extremely large cross sections for Rydberg charge exchange. Classical trajectory Monte Carlo calculations indicate an $\mathrm{H}\ifmmode\bar\else\textasciimacron\fi{}$ instantaneous production rate of 106/{}^{6}/6/s.
This work reports on experiments in which antihydrogen atoms have been produced in cryogenic Penning traps from antiproton and positron plasmas by two different methods and on experiments that have been carried out subsequently in order to investigate the antihydrogen atoms. By the first method antihydrogen atoms have been formed during the process of positron cooling of antiprotons in so called nested Penning traps and detected via a field ionization method. A linear dependence of the number of detected antihydrogen atoms on the number of positrons has been found. A measurement of the state distribution has revealed that the antihydrogen atoms are formed in highly excited states. This suggests along with the high production rate that the antihydrogen atoms are formed by three-body recombination processes and subsequent collisional deexcitations. However current theory cannot yet account for the measured state distribution. Typical radii of the detected antihydrogen atoms lie in the range between 0.4 µm and 0.15 µm. The deepest bound antihydrogen atoms have radii below 0.1 µm. Antihydrogen atoms with that size have chaotic positron orbits so that for the first time antihydrogen atoms have been detected that cannot be described by the GCA-model. The kinetic energy of the weakest bound antihydrogen atoms has been measured to about 200 meV, which corresponds to an antihydrogen velocity of approximately 6200 m/s. A simple model suggests that these atoms are formed from only one deexcitation collision and methods that might lead to a decrease of the antihydrogen velocity are presented. By the second method antihydrogen atoms have been synthesized in charge-exchange processes. Lasers are used to produce a Rydberg cesium beam within the cryogenic Penning trap that collides with trapped positrons so that Rydberg positronium atoms are formed via charge-exchange reactions. Due to their charge neutrality the Rydberg positronium atoms are free to leave the positron trapping region. The Rydberg positronium atoms that collide with nearby stored antiprotons form antihydrogen atoms in charge-exchange reactions. So far, 14 +/- 4 antihydrogen atoms have been detected background-free via a field-ionization method. The antihydrogen atoms produced via the two-step charge-exchange mechanism are expected to have a temperature of 4.2 K, the temperature of the antiprotons from which they are formed. A method is proposed by which the antihydrogen temperature can be determined with an accuracy of better than 1 K from a measurement of the time delay between antihydrogen annihilation events and the laser pulse that initiates the antihydrogen production via the production of Rydberg cesium atoms. First experiments have been carried out during the last days of the 2004 beam time, but the number of detected antihydrogen annihilations has been too low for a determination of the antihydrogen temperature. Trapped antiprotons have been directly exposed to laser light delivered by a Titanium:Sapphire laser in order to investigate if the laser light causes any loss on the trapped antiprotons. Experiments have shown that no extra loss occurs for laser powers of less than 590 mW. This is an important result against the background of the future plan to confine antihydrogen atoms in a combined Penning-Ioffe trap and then to carry out laser spectroscopy on these atoms, since it reveals that laser light does not cause an increase of the pressure in the trapping region to the extend that annihilations with the background gas become noticeable. The ATRAP Collaboration plans to precisely investigate antihydrogen atoms. The ultimate goal is to test the CPT-theorem by a high precision measurement of the 1S-2S transition of antihydrogen and a comparison with the precisely known value of the corresponding transition in hydrogen. This thesis presents the achievement of the first step towards this challenging goal: the production of cold antihydrogen itself.
Antihydrogen production by charge exchange reaction between positronium (Ps) atoms and antiprotons requires an efficient excitation of Ps atoms up to high-nnn levels (Rydberg levels). In this study it is assumed that a Ps cloud is produced within a relatively strong uniform magnetic field (1T)(1\phantom{\rule{0.3em}{0ex}}\mathrm{T})(1T) and with a relatively high temperature (100K)(100\phantom{\rule{0.3em}{0ex}}\mathrm{K})(100K). Consequently, the structure of energy levels are deeply modified by Zeeman and motional Stark effects. A two-step laser light excitation, the first one from ground to n=3n=3n=3 and the second from this level to a Rydberg level, is proposed and the physics of the problem is discussed. We derive a simple formula giving the absorption probability with substantially incoherent laser pulses. A 30% population deposition in high-nnn states can be reached with feasible lasers suitably tailored in power and spectral bandwidth.