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한국자기학회 학술연구발표회 논문개요집

Emergence of New States in Low-Dimensional Quantum Magnets

Gang Su

Published Dec 1, 2010• 0 citations
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The prohibition of finite-temperature phase transition in one-dimensional (1D) Ising models and 1D/2D quantum Heisenberg models with short-range interactions fundamentally constrains the application potentials of low-dimensional magnetic materials. Recently, ultranarrow phase crossover (UNPC), which can approach a transition at a desirable finite temperature $T_0$ arbitrarily closely, was discovered in 1D decorated Ising chains and ladders. Here we present a theoretical study of similarly decorated, yet much more challenging, quantum Heisenberg ferrimagnets in a magnetic field, which features ferromagnetic backbone exchange $J$, antiferromagnetic site-decoration coupling $J_{AF}$, and different magnetic moments for the backbone and decorating spins $μ_aS_a<μ_bS_b$. We exactly solved the model in the large $J$ limit -- as a central-macrospin model -- and found two finite-temperature second-order transitions; just above $T_{c2}$ a ``half-ice, half-fire'' regime appears. Finite-$J$ weak-field results follow from an effective-field mapping, suggesting the emergence of UNPC at finite $T_0$ in 2D square lattices thanks to its exponentially strong initial magnetic susceptibility $χ_0\propto e^{4πS_a^2 J/T_0}$, though less likely in 1D chains where $χ_0\propto J/T_0$. These results may shed light on new technological applications of low-dimensional quantum spin systems and attract experimental and computational tests.

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Low dimensionality enhances quantum fluctuations, triggering novel states of quantum matter to emerge. In real materials, low dimensionality usually arises from spatially strongly anisotropic couplings. Here, we demonstrate a different mechanism: in two-dimensional systems with coupled alternating ferromagnetic (FM) and antiferromagnetic (AFM) spin-1/21/21/2 chains, an applied magnetic field may drive a dimensional reduction. Under magnetic field, the FM chains polarize and stiffen, suppressing the propagation of transverse AFM fluctuations from one chain to another, and effectively induce one-dimensional behavior at low energies. For a model describing botallackite, Cu2_22​(OH)3_33​Br, quantum Monte Carlo dynamics show that beyond a critical magnetic field, the low-energy spectrum reduces to that of a one-dimensional AFM Heisenberg spin-1/21/21/2 chain with field-dependent incommensurate two-spinon fluctuations, providing clear signatures for inelastic neutron scattering.
The 2012 Gordon Conference on Correlated Electron Systems will present cutting-edge research on emergent properties arising from strong electronic correlations. While we expect the discussion at the meeting to be wide-ranging, given the breadth of the title subject matter, we have chosen several topics to be the particular focus of the talks. These are New Developments in Single and Bilayer Graphene, Topological States of Matter, including Topological Insulators and Spin Liquids, the Interplay Between Magnetism and Unconventional Superconductivity, and Quantum Critical Phenomena in Metallic Systems. We also plan to have shorter sessions on Systems Far From Equilibrium, Low Dimensional Electron Fluids, and New Directions (which will primarily focus on new experimental methodologies and their interpretation).
The prohibition of finite-temperature phase transition in one-dimensional (1D) Ising models and 1D/2D quantum Heisenberg models with short-range interactions fundamentally constrains the application potentials of low-dimensional magnetic materials. Recently, ultranarrow phase crossover (UNPC), which can approach a transition at a desirable finite temperature T0T_0T0​ arbitrarily closely, was discovered in 1D decorated Ising chains and ladders. Here we present a theoretical study of similarly decorated, yet much more challenging, quantum Heisenberg ferrimagnets in a magnetic field, which features ferromagnetic backbone exchange JJJ, antiferromagnetic site-decoration coupling JAFJ_{AF}JAF​, and different magnetic moments for the backbone and decorating spins μaSa<μbSbμ_aS_a<μ_bS_bμa​Sa​<μb​Sb​. We exactly solved the model in the large JJJ limit -- as a central-macrospin model -- and found two finite-temperature second-order transitions; just above Tc2T_{c2}Tc2​ a ``half-ice, half-fire'' regime appears. Finite-JJJ weak-field results follow from an effective-field mapping, suggesting the emergence of UNPC at finite T0T_0T0​ in 2D square lattices thanks to its exponentially strong initial magnetic susceptibility χ0∝e4πSa2J/T0χ_0\propto e^{4πS_a^2 J/T_0}χ0​∝e4πSa2​J/T0​, though less likely in 1D chains where χ0∝J/T0χ_0\propto J/T_0χ0​∝J/T0​. These results may shed light on new technological applications of low-dimensional quantum spin systems and attract experimental and computational tests.